Coherent anti-Stokes resonance Raman scattering of excited molecules |
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| Authors: | J. Herrmann M. Landmann |
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| Affiliation: | Department of Physics, University of Jena, Jena, German Democratic Republic |
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| Abstract: | A theoretical investigation of the coherent anti-Stokes resonance Raman scattering (CARRS) of excited molecules is given. The calculation of the anti-Stokes intensity predicts the simultaneous appearance of the vibrational frequencies of the ground and the excited electronic state in the CARRS spectra. The line shape of these spectra and the optimum conditions for the anti-Stokes amplification are discussed. |
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