High-resolution emission spectroscopy of CO2 collisionally excited by N2. Rotational distribution |
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| Authors: | SP Venkateshan SV Ryali JB Fenn |
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| Institution: | Department of Chemical Engineering, Yale University, New Haven, Connecticut 06520, USA |
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| Abstract: | We obtained, for the first time, high-resolution rotational distribution of CO2 collisionally excited by N2. The rotational distribution is non-Boltzmann, and the initial results suggest that surprisingly large impact parameter collisions contribute substantially to the collisional excitation, even though small impact parameter collisions are more effective, as expected. |
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