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Single-molecule electron spin resonance |
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| Authors: | C. von Borczyskowski J. Köhler W. E. Moerner M. Orrit J. Wrachtrup |
| Affiliation: | 1. Optical Spectroscopy and Molecular Physics and Centre for Nanostructured Materials and Analytics, Chemnitz University of Technology, Strasse der Nationen 62, 09107, Chemnitz, Germany 2. Experimental Physics IV, University of Bayreuth, Bayreuth, Germany 3. Department of Chemistry, Stanford University, Stanford, California, USA 4. Molecular Nanooptics and Spins, Huygens Laboratory, Leiden University, Leiden, The Netherlands 5. Physikalisches Institut, Universit?t, Stuttgart, Germany |
| Abstract: | In 1993, two collaborations independently achieved the first optical detection of a single electron spin, using paramagnetic resonance of the triplet state of a single molecule. We review the context of this work and the main later results and give a brief outlook for future experiments based on the detection and manipulation of single spins by optical methods. |
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