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1.
Employing nanocrystals (NCs) as building blocks of porous aerogel network structures allows the conversion of NC materials into macroscopic solid structures while conserving their unique nanoscopic properties. Understanding the interplay of the network formation and its influence on these properties like size-dependent emission is a key to apply techniques for the fabrication of novel nanocrystal aerogels. In this work, CdSe/CdS dot/rod NCs possessing two different CdSe core sizes were synthesized and converted into porous aerogel network structures. Temperature-dependent steady-state and time-resolved photoluminescence measurements were performed to expand the understanding of the optical and electronic properties of these network structures generated from these two different building blocks and correlate their optical with the structural properties. These investigations reveal the influence of network formation and aerogel production on the network-forming nanocrystals. Based on the two investigated NC building blocks and their aerogel networks, mixed network structures with various ratios of the two building blocks were produced and likewise optically characterized. Since the different building blocks show diverse optical response, this technique presents a straightforward way to color-tune the resulting networks simply by choosing the building block ratio in connection with their quantum yield.  相似文献   
2.
Fluid Dynamics - Steady-state subsonic flows of nonequilibrium air plasma past a cylindrical body with plane face and heat transfer are investigated under the conditions characteristic of testing...  相似文献   
3.
Massoumi  Sina  Challamel  Noël  Lerbet  Jean  Wautier  Antoine  Nicot  François  Darve  Félix 《Meccanica》2022,57(8):2043-2066
Meccanica - This study is an attempt towards a better understanding of the length scale effects on the bending response of the granular beams. To this aim, a unidimensional discrete granular chain...  相似文献   
4.
Russian Physics Journal - Using the methods of modern physical materials science, the structural phase state, the defect substructure and the fracture surface of low-carbon alloy steel welds formed...  相似文献   
5.
This work describes the basic principles of Total-reflection X-Ray Fluorescence (TXRF) spectrometry and some of its most outstanding applications for investigating metal traces, mainly in biological and biomedical samples. TXRF is an analytical technique that combines the versatility of elemental analysis by X-ray energy dispersion with a low detection limit in the order of picograms of absolute mass or a few ppb (μg L−1) as concentration. The microanalytical capacity of TXRF allows the study of small sample quantities. The TXRF can perform qualitative and mass ratio analyses of the elements present in a sample of only a few hundred nanograms. These properties are of great importance in the research of metal traces in biological systems, as they allow fast, precise, and accurate characterisation of the elemental fingerprint at trace level. Its successful application in studies of the coordination kinetics of new platinum-based antitumor drugs with DNA, its application in the study profile of the metal in healthy and cancerous human tissues, or even its application in the study of the processes of metal diffusion through cell membranes are just a few examples of TXRF capabilities in the biomedical sciences. This brief review's main objective is to provide an overview of the physical principles and possibilities of TXRF spectrometry. It also highlights some of the most outstanding applications that have been developed so far, mainly in the biological field, so that the reader can evaluate their potential applications.  相似文献   
6.
Carbyne is an infinitely long linear chain of carbon atoms with sp1 hybridization and the truly one-dimensional allotrope of carbon. While obtaining freestanding carbyne is still an open challenge, the study of confined carbyne, linear chains of carbon encapsulated in carbon nanotubes, provides a pathway to explore carbyne and its remarkable properties in a well-defined environment. In this review, we discuss the basics and recent advances in studying single confined carbyne chains by Raman spectroscopy, which is their primary spectroscopic characterization method. We highlight where single carbyne chain studies are needed to advance our understanding of confined carbyne as a material system and provide an overview of the open questions that need to be addressed and of those aspects currently under debate.  相似文献   
7.
Journal of Thermal Analysis and Calorimetry - The paper focuses on the analytical analysis of the propagation of a normal shock wave in an adiabatic gas flow with nanoparticles. A modified...  相似文献   
8.
Physics of Atomic Nuclei - Data on the production of positively charged particles emitted at an angle of 40 $${}^{\circ}$$ (in the laboratory frame) with transverse momenta of up to 2.7 GeV $$/c$$...  相似文献   
9.
Russian Physics Journal - Aiming at problems of low probability of interception and poor anti-jamming performance of the multi-output radar, the numerical simulation based on a chaos optimization...  相似文献   
10.
Russian Physics Journal - The interaction mechanisms of low-energy long-duration (~1 ms) laser pulses with dispersed particles in air are considered. The basic equations describing the mechanisms...  相似文献   
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