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Investigation of the growth process of Si nanowires using the vapour-liquid-solid mechanism 下载免费PDF全文
Silicon nanowires have been grown by the thermal decomposition of silane via the vapour-liquid-solid (VLS) mechanism. Three different stages of VLS growth (eutectic alloy formation, crystal nucleation and unidirectional growth) were studied separately using a scanning electron microscope and a high-resolution transmission electron microscope. Very short silicon nanowires prepared under particular conditions provide direct evidence of the VLS mechanism on a nanometre scale. Our results will be very helpful for the controllable synthesis of Si nanowires. 相似文献
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An increase of work function (0.3 eV) is achieved by irradiating poly(3,4-ethylenedioxythiophene):poly(styrene sul- fonate) (PEDOT:PSS) film in vacuum with 254-nm ultraviolet (UV) light. The mechanism for such an improvement is investigated by photoelectron yield spectroscopy, X-ray photo electron energy spectrum, and field emission technique. Sur- face oxidation and composition change are found as the reasons for work function increase. The UV-treated PEDOT:PSS film is used as the hole injection layer in a hole-only device. Hole injection is improved by UV-treated PEDOT:PSS film without baring the enlargement of film resistance. Our result demonstrates that UV treatment is more suitable for modifying the injection barrier than UV ozone exposure. 相似文献
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In field emission under a non-dc voltage, a displacement current is inevitable due to charging the cathode–anode condenser. Under an often-used square voltage pulse, in which the voltage rises from zero to a certain value abruptly, the charging current in the circuit is very large at the rising and falling edges. This large charging current makes measurement of the actual emissive current from the cathode difficult, constitutes a threat to the components in the circuit and causes attenuation of the emissive current within the pulse. To alleviate these drawbacks, trapezoid voltage pulses, whose rising edges are extended dramatically in comparison with square voltage pulses, are employed to extract the field emission. Under a trapezoid voltage pulse, the charging current is clearly lowered as expected. Furthermore, the heat generated by the charging current under the trapezoid voltage pulse is much smaller than that under the square voltage pulse. Hence the emissive current does not show any attenuation within the pulse. Finally, the average emissive currents are found to decrease with the repetition frequency of the pulses. 相似文献
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Amorphous silicon nanowires were prepared by heating an Si substrate at high temperatures using an Ni (or Au) catalyst.The nanowires have a diameter of 10-40nm and a length of up to several tens of micrometres.Unlike the well-known vapour-liquid-solid mechanism,a solid-liquid-solid mechanism appeared to control the nanowire growth.The heating process had a strong influence on the growth of silicon nanowires.It was found that ambient gas was necessary to grow nanowires.This method can be used to prepare other kinds of nanowires. 相似文献
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