A self-powered and sensitive terahertz photodetection based on PdSe2

With the rapid development of terahertz technology, terahertz detectors are expected to play a key role in diverse areas such as homeland security and imaging, materials diagnostics, biology, medical sciences, and communication. Whereas self-powered, rapid response, and room temperature terahertz photodetectors are confronted with huge challenges. Here, we report a novel rapid response and self-powered terahertz photothermoelectronic (PTE) photodetector based on a low-dimensional material: palladium selenide (PdSe₂). An order of magnitude performance enhancement was observed in photodetection based on PdSe₂/graphene heterojunction that resulted from the integration of graphene and enhanced the Seebeck effect. Under 0.1-THz and 0.3-THz irradiations, the device displays a stable and repeatable photoresponse at room temperature without bias. Furthermore, rapid rise (5.0 μs) and decay (5.4 μs) times are recorded under 0.1-THz irradiation. Our results demonstrate the promising prospect of the detector based on PdSe₂ in terms of air-stable, suitable sensitivity and speed, which may have great application in terahertz detection.     

CO_2激光烧结合成负热膨胀材料Sc_2(MO_4)_3(M=W,Mo)及其拉曼光谱

用CO2激光烧结合成了负热膨胀材料Sc2(WO4)3和Sc2(MoO4)3.实验表明,激光合成负热膨胀材料Sc2(WO4)3和Sc2(MoO4)3属于快速合成技术,合成一个样品的时间仅需几秒到十几秒,具有快速凝固的特征;X射线衍射和拉曼光谱分析表明,所合成的材料为正交相结构,且具有较高的纯度;变温拉曼光谱分析表明,所合成的材料在室温以上没有相变,但可能有微弱的吸水性;在对Sc2O3,Mo O3,WO3,Sc2(MoO4)3和Sc2(WO4)3拉曼光谱分析的基础上,给出了激光光子能量及原料和合成产物的声子能级图,分析了激光烧结合成的机理.激光光子能量转化为激发声子的能量是光热转化的主要通道,原料在熔池中反应并快速凝固形成最终产物.     

利用非规整膜系实现宽角度入射减偏振、减反射薄膜的研究

利用非均匀膜系理论对宽角度入射减偏振、减反射薄膜进行优化设计,分析了在宽角度入射的情况下,偏振光产生透过率不同的原因,选取了Na3AlF6、Ta2O5和Al2O3三种不同折射率材料,采用BK7作为基底,模拟设计了光谱区在500～560 nm波段、入射角为0~70°之间的多层减偏振、减反射薄膜,设计结果表明,薄膜的透过率得到大幅度提高.     

First-Principles Study of Electronic Properties in PbS（1^-00） with Vacancy Defect

Electronic properties of both Pb and S vacancy defects in PbS（1^-00） have been studied using the first-principles density functional theory （DFT） calculations with the plane-wave pseudopotentials. It is found that the density of states （DOS） near the top of the valence band and the bottom of the conduction band is significantly modified by these defects. Our calculation indicates that in the case of S vacancy defects the Fermi energy shifts to the conduction band making it as an n-type PbS （donor）. However, in the case of Pb vacancy, because of the appreciable change of the DOS, the system acts as a p-type PbS （accepter）. In addition, the structural relaxation shows that the defect leads to outward relaxation of the nearest-neighbouring atoms and inward relaxation of the next-nearest neighbouring atoms.     

缺陷对二维四方光子晶体透射光谱的影响

利用转移矩阵法研究了二维四方光子晶体中缺陷对透射光谱的影响。结果表明缺陷对TE波的影响比对TM波的影响明显,缺陷层填充比对禁带宽度影响很大,TE波禁带在填充比r/a=0.33时最宽,第一禁带的最低频率随着填充比的增加向低频移动。     

极化诱导的内建电场对Mn δ掺杂的GaN/AlGaN量子阱居里温度的调制

采用传输矩阵方法分析极化诱导的内建电场对Mn δ掺杂的GaN/Al_xGa_1-xN量子阱居里温度(T_C)的调制作用.通过解薛定谔方程计算出在不同的内建电场条件下半导体量子阱局域态内的基态空穴能级和波函数分布情况，并在此基础上确定量子阱内Mn δ掺杂情况下T_C随内建电场的变化趋势，分析了不同量子阱结构引起的内建电场分布变化及其对T_C的影响.在耦合双量子阱中通过调节左右阱的不对称性可以得到T_C近3倍的增长. 关键词： GaN 量子阱 内建电场 居里温度     

First Principles Study on the Magnetism of Rectangular Nanosilicenes

We present first-principle calculations on the magnetism in finite rectangular nanosilicenes(RNSs). An antiferromagnetic(AFM) state at two zigzag edges is found when the RNSs approach a critical size. This AFM state originates from the localized p_z orbits of Si atoms at the edges, similar to those in the infinitely long zigzag-edged silicon nanoribbons. The smallest RNS that can maintain the AFM phase as the ground state is identified. It is also found that aluminum dopants can regulate the distribution of the spin density and the energy difference between AFM and FM states.     

CO$lt;sub$gt;2$lt;/sub$gt;激光烧结合成负热膨胀材料Sc$lt;sub$gt;2$lt;/sub$gt;($lt;i$gt;M$lt;/i$gt;O$lt;sub$gt;4$lt;/sub$gt;)$lt;sub$gt;3$lt;/sub$gt;($lt;i$gt;M$lt;/i$gt;=W,Mo)及其拉曼光谱

用CO₂激光烧结合成了负热膨胀材料Sc₂(WO₄)₃和Sc₂(MoO₄)₃. 实验表明, 激光合成负热膨胀材料Sc₂(WO₄)₃和Sc₂(MoO₄)₃属于快速合成技术, 合成一个样品的时间仅需几秒到十几秒, 具有快速凝固的特征; X射线衍射和拉曼光谱分析表明, 所合成的材料为正交相结构, 且具有较高的纯度; 变温拉曼光谱分析表明, 所合成的材料在室温以上没有相变, 但可能有微弱的吸水性; 在对Sc₂O₃, MoO₃, WO₃, Sc₂(MoO₄)₃和Sc₂(WO₄)₃拉曼光谱分析的基础上, 给出了激光光子能量及原料和合成产物的声子能级图, 分析了激光烧结合成的机理. 激光光子能量转化为激发声子的能量是光热转化的主要通道, 原料在熔池中反应并快速凝固形成最终产物. 关键词： 负热膨胀材料 合成 激光烧结 拉曼光谱     

磁场诱导的单离子各向异性反铁磁链的比热

利用改进的Schwinger玻色子平均场理论,研究了横向外加磁场下自旋为1的单粒子各向异性海森堡反铁磁链的热力学性质.发现在外加磁场下预示这一体系中存在Luttinger液体相—完全极化相相变的比热奇性,并给出了相应的相图.研究还发现,单粒子各向异性对比热的影响较小,这和纵向场的结果完全不同.以上结果对整自旋的反铁磁链具有普适性,对实验研究具有指导性. 关键词： 反铁磁链 热力学性质 Schwinger 玻色子