High-Resolution Selective Excitation of Resonance-Enhanced Multiphoton-Ionization Photoelectron Spectroscopy by Shaping Femtosecond Laser Pulses

Femtosecond laser-induced resonance-enhanced multiphoton-ionization photoelectron spectroscopy （REMPI-PS） is faced with two drawbacks of low spectral resolution and poor selective excitation due to the broad spectral bandwidth. We propose a scheme to obtain a high-resolution selective excitation of （2＋1） REMPI-PS by com- bining 7r and cosinusoidal phase modulation. Our theoretical results indicate that the （2＋1） REMPI-PS signals related to neighboring excited states can be differentiated from their indistinguishable photoelectron spectra by the 7r phase modulation, and then their selective excitation can be realized by supplementally adding the cosi- nusoidal phase modulation. Furthermore, the physical mechanism of the high-resolution selective excitation of （2＋1） REMPI-PS is explained by considering the two-photon power spectrum.     

飞秒激光作用下全向高反膜破坏的激发过程

设计和制备了全向高反膜SiO₂/TiO₂，研究了它在不同脉冲宽度、不同脉冲能量的飞秒激光作用下的破坏阈值和烧蚀深度.利用发展的抽运-探针方法，研究了抽运脉冲作用下材料中导带电子的超快激发和能量沉积过程，建立并求解了飞秒激光激发材料和材料的激发对抽运光自身反作用的耦合动力学模型.模型较好地揭示了材料破坏的激发过程. 关键词： 飞秒激光 全向高反膜 激发过程 破坏机制     

Femtosecond laser-induced breakdown of multilayers and gold film

We report single-shot damage threshold as a function of pulse duration (50-900 fs) for MgF2/ZnS 800-nm omnidirectional-reflection film, interference filter, and gold film. The results indicate that the damage with ultrashort pulse is nonthermal, which is different from that with long pulse. Additionally, the ablation crater depths of 45°     

飞秒激光烧蚀石英玻璃的实验与理论研究

实验研究了800nm飞秒激光作用下石英玻璃的破坏机理和烧蚀规律，给出了破坏阈值与脉冲宽度的关系.发展了雪崩击穿模型，计算了材料的烧蚀阈值与脉冲宽度的依赖关系，烧蚀深度、烧蚀体积与脉冲能量的依赖关系，研究了导带电子的扩散对材料中激光能量的沉积、分布，以及材料的破坏阈值和烧蚀规律的影响. 关键词： 飞秒激光脉冲 破坏机理 石英玻璃 电子扩散     

抽运激光在光靶中的局域及其对X射线激光特性的影响

新型X射线靶设计为:由SiO2和TiO2组成具有12个周期的一维光子晶体,在它的中间嵌入光靶材料层作为缺陷层,SiO2,TiO2和光靶层的光学厚度分别为λ4、λ4和λ2,λ为抽运激光波长.与普通平板光靶相比,当抽运光垂直照射到这种光靶时,靶层内部的光强将提高2个数量级,所以抽运激光的阈值强度将降低2个数量级,这有利于X射线激光的小型化.在同样的抽运激光照射下,X射线激光的强度将提高4个数量级,转换效率也将提高约4个数量级.由于平均电离度随抽运激光强度的提高而提高,所以采用这种光靶有利于使X射线激光向短波长推进. 关键词： X射线激光 光子晶体 光波局域     

飞秒激光脉冲作用下氧化镁的烧蚀及其超快动力学过程

研究了双面抛光氧化镁单晶（111）表面800 nm飞秒激光单脉冲烧蚀阈值和激光脉宽的依赖关系.利用泵浦-探针技术，测量不同能量和脉宽作用下飞秒激光烧蚀的时间分辨反射率的演化.通过扫描电镜观察其烧蚀形貌，发现大量的沿氧化镁［100］晶向开裂的裂纹.讨论了表面裂纹的形成机理，并解释了飞秒激光烧蚀氧化镁的超快动力学过程.     

Simulating resonance-mediated two-photon absorption enhancement in rare-earth ions by a rectangle phase modulation

Improving the up-conversion luminescence efficiency of rare-earth ions via the multi-photon absorption process is crucial in several related application areas. In this work, we theoretically propose a feasible scheme to enhance the resonance-mediated two-photon absorption in Er~(3+) ions by shaping the femtosecond laser field with a rectangle phase modulation. Our theoretical results show that the resonance-mediated two-photon absorption can be decomposed into the on-resonant and near-resonant parts, and the on-resonant part mainly comes from the contribution of laser central frequency components, while the near-resonant part mainly results from the excitation of low and high laser frequency components.So, the rectangle phase modulation can induce a constructive interference between the two parts by properly designing the modulation depth and width, and finally realizes the resonance-mediated two-photon absorption enhancement. Moreover, our results also show that the enhancement efficiency of resonance-mediated two-photon absorption depends on the laser pulse width(or laser spectral bandwidth), final state transition frequency, and intermediate and final state absorption bandwidths. The enhancement efficiency modulation can be attributed to the relative weight manipulation of on-resonant and near-resonant two-photon absorption in the whole excitation process. This study presents a clear physical insight for the quantum control of resonance-mediated two-photon absorption in the rare-earth ions, and there will be an important significance for improving the up-conversion luminescence efficiency of rare-earthions.     

Dispersion Theory of Polaron in a Parabolic Quantum Dot at Finite Temperatures

By using the dispersion theory instead of the Fröhlich Hamiltonian, the polaron energy in a quantum dot with a parabolic confinement potential is investigated at finite temperatures. It is found that the self-trapping energy of the polaron decreases with the increasing temperature, and the temperature effect is more obvious in quantum dots with weaker confinement.     

超快电子衍射技术及其应用

时间和空间上实时观测原子运动对于自然科学研究有着非常重大的意义, 而超快电子衍射(UED)技术同时具备飞秒激光脉冲的高时间分辨特性和电子衍射技术的高空间特性, 可以为实时观测原子级分辨尺度物质的结构变化提供一种有效工具. 本文综述了超快电子衍射技术的发展历史、实验方法以及相关应用, 并且展望了超快电子衍射技术未来的发展.