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Pr^3+掺杂的LaF3纳米微晶/氟氧化物玻璃陶瓷的4f5d能级光谱性质 总被引:1,自引:0,他引:1
用同步辐射的真空紫外(VUV)和紫外(UV)作为激发源研究了Pr^3 (0.1%)掺杂的LaF3纳米微晶,氟氧化物玻璃陶瓷的4f5d能级光谱性质。样品中存在两种不同的Pr^3 -LaF3微晶中的Pr^3 最低的4f5d能级在^1S0能级之上,玻璃中的却在^S0能级之下,通过VUV和UV激发光谱得出这两种Pr^3 最低的4f5d能级的位置。当用181nm光激发样品时,在发射光谱中同时观察到了微晶中Pr^3 4f^2→4f^2的窄谱带发射和玻璃中4f5d→4f^2的宽谱带发射。在20K时观察到了LaF3纳米微晶中作为Pr^3 光子级联发射(PCE)第二步的^3P0→H4的跃迁,室温下却没有观察到,文中详细讨论了产生这种现象的原因。 相似文献
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为计算中高频半空间结构频带振动下声辐射问题,推导了基于能量源的半空间频率均方声压法(Frequency Averaged Quadratic Pressure,FAQP),并提出了改进的半空间FAQP法,克服了半空间FAQP法在失效频率下解不唯一的问题。频率带宽为4 Hz的刚性壁面作用下的脉动球和与自由表面相接触的脉动半球的声辐射数值计算,验证了改进的半空间FAQP法对解决失效频率下解不唯一问题的有效性。同时,刚性壁面作用下的脉动球和与自由表面相接触的脉动半球声辐射数值计算结果均表明,在1/3倍频程下,改进的半空间FAQP法与常规边界元方法相比,具有更高的计算精度,更适用于中高频计算。 相似文献
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用共沉淀法制备出不同掺杂浓度的钇铝石榴石(Y3Al5O12,YAG):Pr3+粉末.在不同温度下用同步辐射的真空紫外光(VUV)作为激发光 源测量了其发射和激发光谱.对YAG:Pr3+被VUV激发后的发光过程进行了分析, 并估算了YAG:Pr3+的声子能量、黄昆因子S及Stokes位移.当用170nm光激发样 品时,可能存在自陷激子和通过自陷激子能量传递引发的3P0发射 ,这种跃迁途径不同于用240nm和289nm两个波长激发后的跃迁途径;对Pr3+在Y AG中的4f5d能级进行了研究,从而对其4f5d组态有了一个较清晰的认识.
关键词:
3+')" href="#">YAG:Pr3+
同步辐射
4f5d能级
VUV 相似文献
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用共沉淀法制备出不同掺杂浓度的钇铝石榴石(Y3Al5O12,YAG):Pr3+粉末.在不同温度下用同步辐射的真空紫外光(VUV)作为激发光源测量了其发射和激发光谱.对YAG:Pr3+被VUV激发后的发光过程进行了分析,并估算了YAG:Pr3+的声子能量、黄昆因子S及Stokes位移.当用170nm光激发样品时,可能存在自陷激子和通过自陷激子能量传递引发的3P0发射,这种跃迁途径不同于用240nm和289nm两个波长激发后的跃迁途径;对Pr3+在YAG中的4f5d能级进行了研究,从而对其4f5d组态有了一个较清晰的认识. 相似文献
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Pr3+掺杂的LaF3纳米微晶/氟氧化物玻璃陶瓷的VUV光谱 总被引:1,自引:0,他引:1
The vacuum ultraviolet (VUV) spectroscopic properties of praseodymium (Pr3+, 1at%) doped LaF3 nanocrystals/glass at room temperature and 20 K are reported. Two types of Pr3+ ions, those in LaF3 nanocrystals and those in the glass host, were excited to 4f 5d band by VUV using synchrotron radiation as an excitation source, and emissions of 1S0 → 1D2 (336 nm), 1S0 → 1I6 (397 nm ) of Pr3+ in the nanocrystals and emissions of 4f 5d → 3HJ, 3FJ of Pr3+ in the glass appeared at the same time. But unlike in the bulk sample crystals, emission of 3P0 → 3HJ, 3FJ as the second step of the quantum splitting (QS) of Pr3+ in the LaF3 nanocrystals was not observed at room temperature, which could be explained that Pr3+ ions in the glass absorbed the energy of 3P0→ 3H4 of Pr3+ in the nanocrystals. Two types of excitation spectra monitoring different emissions were also measured, so it could be observed that the lowest energy of 4f 5d band of Pr3+ in the nanocrystals was about 53 500 cm-1 (186 nm) and in the glass about 33 800 cm-1(295 nm), respectively. These emission and excitation spectra were contrasted to those of bulk sample crystals LaF3∶Pr3+. 相似文献
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