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1.
By partially doping Pb to effectively suppress the superstructure in single-layered cuprate Bi_2Sr_2CuO_(6+δ)(Pb-Bi2201) and annealing them in vacuum or in high pressure oxygen atmosphere, a series of high quality Pb-Bi2201 single crystals are obtained with T_c covering from 17 K to non-superconducting in the overdoped region. High resolution angle resolved photoemission spectroscopy measurements are carried out on these samples to investigate the evolution of the Fermi surface topology with doping in the normal state. Clear and complete Fermi surfaces are observed and quantitatively analyzed in all of these overdoped Pb-Bi2201 samples. A Lifshitz transition from holelike Fermi surface to electron-like Fermi surface with increasing doping is observed at a doping level of ~0.35. This transition coincides with the change that the sample undergoes superconducting-to-non-superconducting states.Our results reveal the emergence of an electron-like Fermi surface and the existence of a Lifshitz transition in heavily overdoped Bi2201 samples. This provides important information in understanding the connection between the disappearance of superconductivity and the Lifshitz transition in the overdoped region.  相似文献   
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The detailed information of the electronic structure is the key to understanding the nature of charge density wave(CDW) order and its relationship with superconducting order in the microscopic level. In this paper, we present a high resolution laser-based angle-resolved photoemission spectroscopy(ARPES) study on the three-dimensional(3 D) hole-like Fermi surface around the Brillouin zone center in a prototypical quasi-one-dimensional CDW and superconducting system ZrTe_3. Double Fermi surface sheets are clearly resolved for the 3 D hole-like Fermi surface around the zone center. The3 D Fermi surface shows a pronounced shrinking with increasing temperature. In particular, the quasiparticle scattering rate along the 3 D Fermi surface experiences an anomaly near the charge density wave transition temperature of ZrTe_3(~ 63 K). The signature of electron–phonon coupling is observed with a dispersion kink at ~ 20 me V; the strength of the electron–phonon coupling around the 3 D Fermi surface is rather weak. These results indicate that the 3 D Fermi surface is also closely connected to the charge-density-wave transition and suggest a more global impact on the entire electronic structure induced by the CDW phase transition in ZrTe_3.  相似文献   
4.
刘国东 《物理学进展》2011,24(2):163-194
本文较详细地评述了高温超导体角分辨光电子能谱研究的所有主要方面的成就及最新进展。所涉及的主题有:角分辨光电子能谱基础知识,费米面的角分辨光电子能谱研究,超导能隙及对称性研究,赝能隙问题的角分辨光电子能谱研究,高温超导体的角分辨光电子能谱谱线形分析,近节点区域准粒子的色散行为,双层能带劈裂。所涉及的材料不仅有最广泛研究的Bi2212,还包括Bi2201,Bi2223,La_214,Y 123乃至电子型掺杂的超导体。所引用的文献特别注意了从新一代高能量、动量分辨的能量分析器得到的系统、深入的工作。  相似文献   
5.
赵林  刘国东  周兴江 《物理学报》2018,67(20):207413-207413
铜氧化物超导体和铁基超导体是人类相继发现的两类高温超导家族,它们的高温超导机理是凝聚态物理领域中长期争论但悬而未决的重大问题.对铁基超导体广泛而深入的研究,以及与铜氧化物高温超导体的对比,对于发展新的量子固体理论、解决高温超导机理、探索新的超导体以及超导实际应用都具有重要意义.固体材料的宏观物性由其微观电子结构所决定,揭示高温超导材料的微观电子结构是理解高温超导电性的前提和基础.由于角分辨光电子能谱技术具有独特的同时对能量、动量甚至自旋的分辨能力,已成为探测材料微观电子结构的最直接、最有力的实验手段,在高温超导体的研究中发挥了重要作用.本文综述了在不同体系铁基超导体中费米面拓扑结构、超导能隙大小和对称性、轨道三维性和选择性、电子耦合模式等的揭示和发现,为甄别和提出铁基超导新理论、解决高温超导机理问题提供重要依据.  相似文献   
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High quality Pb-doped Bi2Sr2Cu06+δ (Pb-Bi2201) single crystals are grown by the traveling solvent floating zone technique, with dimensions as large as - 50 min× - 5.0 min ×- 2 mm. The Pb-Bi2201 single crystals with different doping levels are obtained by the annealing process which covers a wide doping range of the overdoped region. We describe in detail the growth and annealing procedures and the characterization and physical property measurements of the Pb-Bi2201 crystals. The availability of these crystals provides a good opportunity to experimentally investigate high-To cuprate superconductors, particularly in the overdoped region.  相似文献   
7.
在小型常压固定床反应器中研究了不同离子浸渍改性对纳米ZSM-5固体酸催化剂上丁烷和丁烯转化的影响.结果表明,混和碳四中异丁烷比正丁烷易转化,丁烯异构体的转化与其在原料中的含量有关.在贫烯烃原料中,丁烯倾向于生成.在富丁烯原料中,丁烯倾向于转化.但在两种情况下,产物中各丁烯含量大体上按异丁烯、顺反-丁烯-2和丁烯-1顺序递减.采用锌离子改性时异丁烷转化率提高、正丁烷转化率降低.锌离子改性有利于芳烃选择性,但是副产物甲烷和乙烷的产率也较高;铁离子改性对丁烷和丁烯的转化影响不大,但能减少甲烷和乙烷的生成,并提高芳烃选择性;与锌改性相比,锌钠双离子改性降低了异丁烷、正丁烷和丁烯-1的转化率,减少了芳烃产率,但能明显促进丙烯和丁烯的生成.上述结果为碳四液化气综合利用提供了有益信息.  相似文献   
8.
High resolution photoemission measurements are carried out on non-superconducting LaFeAsO parent com- pound and various superconducting RFeAs(O1-ZFx) (R=La, Ce and Pr) compounds. It is found that the parent LaFeAsO compound shows a metallic character. By extensive measurements, several common features are identified in the electronic structure of these Fe-based compounds: (1) 0.2 eV feature in the valence band, (2) a universal 13-16 meV feature, (3) near EF spectral weight suppression with decreasing temperature. These uni- versal features can provide important information about band structure, superconducting gap and pseudogap in these Fe-based materials.  相似文献   
9.
在低温下,通过混合石墨粉,补体3抗血清,溶胶-凝胶而制备了一种基于啼-凝胶技术的可更新的安培分析免疫传感器。该传感器坚固,多孔,拥有一个更新的表面,在辣根过氧化物酶标记的补体3的协助下,通过竞争性的免疫分析来确定人血清中补体3的含量。以邻-氨酚作为底物,-150mV作为工作电位,响应电流与补体3的浓度在1.17-35.1μg/mL范围内呈线性关系,检出限为0.56μg/mL。分析血清样本结果表明所制备的传感器在临床分析中是可行的。  相似文献   
10.
Hongtao Yan 《中国物理 B》2022,31(8):87401-087401
The pseudogap state is one of the most enigmatic characteristics in the anomalous normal state properties of the high temperature cuprate superconductors. A central issue is to reveal whether there is a symmetry breaking and which symmetries are broken across the pseudogap transition. By performing high resolution laser-based angle-resolved photoemission measurements on the optimally-doped Bi2Sr1.6La0.4CuO6+δ superconductor, we report the observations of the particle-hole symmetry conservation in both the superconducting state and the pseudogap state along the entire Fermi surface. These results provide key insights in understanding the nature of the pseudogap and its relation with high temperature superconductivity.  相似文献   
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