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1.
Improving the up-conversion luminescence efficiency of rare-earth ions via the multi-photon absorption process is crucial in several related application areas. In this work, we theoretically propose a feasible scheme to enhance the resonance-mediated two-photon absorption in Er~(3+) ions by shaping the femtosecond laser field with a rectangle phase modulation. Our theoretical results show that the resonance-mediated two-photon absorption can be decomposed into the on-resonant and near-resonant parts, and the on-resonant part mainly comes from the contribution of laser central frequency components, while the near-resonant part mainly results from the excitation of low and high laser frequency components.So, the rectangle phase modulation can induce a constructive interference between the two parts by properly designing the modulation depth and width, and finally realizes the resonance-mediated two-photon absorption enhancement. Moreover, our results also show that the enhancement efficiency of resonance-mediated two-photon absorption depends on the laser pulse width(or laser spectral bandwidth), final state transition frequency, and intermediate and final state absorption bandwidths. The enhancement efficiency modulation can be attributed to the relative weight manipulation of on-resonant and near-resonant two-photon absorption in the whole excitation process. This study presents a clear physical insight for the quantum control of resonance-mediated two-photon absorption in the rare-earth ions, and there will be an important significance for improving the up-conversion luminescence efficiency of rare-earthions.  相似文献   
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Femtosecond laser-induced resonance-enhanced multiphoton-ionization photoelectron spectroscopy (REMPI-PS) is faced with two drawbacks of low spectral resolution and poor selective excitation due to the broad spectral bandwidth. We propose a scheme to obtain a high-resolution selective excitation of (2+1) REMPI-PS by com- bining 7r and cosinusoidal phase modulation. Our theoretical results indicate that the (2+1) REMPI-PS signals related to neighboring excited states can be differentiated from their indistinguishable photoelectron spectra by the 7r phase modulation, and then their selective excitation can be realized by supplementally adding the cosi- nusoidal phase modulation. Furthermore, the physical mechanism of the high-resolution selective excitation of (2+1) REMPI-PS is explained by considering the two-photon power spectrum.  相似文献   
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飞秒激光作用下全向高反膜破坏的激发过程   总被引:1,自引:0,他引:1       下载免费PDF全文
设计和制备了全向高反膜SiO2/TiO2,研究了它在不同脉冲宽度、不同脉冲能量的飞秒激光作用下的破坏阈值和烧蚀深度.利用发展的抽运-探针方法,研究了抽运脉冲作用下材料中导带电子的超快激发和能量沉积过程,建立并求解了飞秒激光激发材料和材料的激发对抽运光自身反作用的耦合动力学模型.模型较好地揭示了材料破坏的激发过程. 关键词: 飞秒激光 全向高反膜 激发过程 破坏机制  相似文献   
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We report single-shot damage threshold as a function of pulse duration (50-900 fs) for MgF2/ZnS 800-nm omnidirectional-reflection film, interference filter, and gold film. The results indicate that the damage with ultrashort pulse is nonthermal, which is different from that with long pulse. Additionally, the ablation crater depths of 45°  相似文献   
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飞秒激光脉冲作用下氧化镁的烧蚀及其超快动力学过程   总被引:3,自引:2,他引:1  
研究了双面抛光氧化镁单晶(111)表面800 nm飞秒激光单脉冲烧蚀阈值和激光脉宽的依赖关系.利用泵浦-探针技术,测量不同能量和脉宽作用下飞秒激光烧蚀的时间分辨反射率的演化.通过扫描电镜观察其烧蚀形貌,发现大量的沿氧化镁[100]晶向开裂的裂纹.讨论了表面裂纹的形成机理,并解释了飞秒激光烧蚀氧化镁的超快动力学过程.  相似文献   
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The study on femtosecond laser-material interaction,especially the topics of laser ablation theorem and ul-trafast dynamics in the process[1-9], has been a veryrich subject in the last few decades. The spotlightsare confined to metal[4,5,9], transparent material[7], IVsemiconductors[2], and III-V compounds[3,6,8], ratherthan the II-VI compounds[10]. ZnSe is an importantluminescent II-VI semiconductor material, with a bandgap of 2.7 eV. Its transmission range is 0.5—22 μm, andit is cons…  相似文献   
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超短脉冲照射下氟化锂的烧蚀机理及其超快动力学研究   总被引:7,自引:0,他引:7  
研究了超短脉冲激光照射下LiF晶体的破坏机理及其超快动力学过程,利用扫描电镜和原子力显微镜等测试手段,观测了飞秒激光照射下LiF晶体的烧蚀形貌。利用烧蚀面积与激光脉冲能量的对数关系确定了LiF晶体的破坏阈值,并利用非线性玻璃棒展宽脉宽,得到了800nm激光作用下LiF破坏阈值对激光脉宽(50~1000fs)的依赖关系;利用抽运一探针超快探测平台,探测了LiF烧蚀过程中反射率的变化。采用雪崩击穿模型,并根据晶体材料反射率与材料的介电常量的依赖关系,通过数值计算,模拟了材料烧蚀阈值与脉宽的依赖关系及材料激发过程中反射率的变化关系。结果表明,理论结果与实验结果符合较好。讨论了飞秒激光照射下LiF晶体中导带电子数密度的变化规律,并解释了相应的实验结果。  相似文献   
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李霞  冯东海  何红燕  贾天卿  单璐繁  孙真荣  徐至展 《物理学报》2012,61(19):197801-197801
在水相合成CdTe以及CdTe/CdS核壳结构量子点基础上, 利用基于抽运-探测技术的瞬态差分透射技术研究了CdTe量子点以及不同CdS壳层厚度的CdTe/CdS量子点的最低激子能态的超快激发与弛豫动力学. 研究表明:相比于CdTe,CdTe/CdS量子点的电子空穴由于空间分离,其所需的激发时间要长于电子空穴空间重叠态所需要的激发时间.随着壳层厚度的增加, 量子点表面的钝化有效地减少了表面态相关弛豫机理,并延长相对应的弛豫时间.  相似文献   
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