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Prof. Dr. Yasutomo Segawa Takehisa Maekawa Prof. Dr. Kenichiro Itami 《Angewandte Chemie (International ed. in English)》2015,54(1):66-81
Activation of aromatic C? H bonds by a transition metal catalyst has received significant attention in the synthetic chemistry community. In recent years, rapid and site‐selective extension of π‐electron systems by C–H activation has emerged as an ideal methodology for preparing organic materials with extended π‐systems. This Review focuses on recently reported π‐extending C–H activation reactions directed toward new optoelectronic conjugated materials. 相似文献
3.
In this paper, we report on an experimental technique for the simultaneous measurement of temperature and three components of velocity in a three-dimensional thermal flow using scanning liquid-crystal thermometry and stereo velocimetry. The temperature is measured by the color image analysis of the liquid-crystal particles suspended in a fluid, while the three velocity components are measured by stereo particle image velocimetry (stereo PIV) with the aid of tracer particles. The measurement is carried out by scanning the light-sheet plane while capturing the sequential color images of the liquid crystals and tracer particles. This measurement allows the reconstruction of the three-dimensional distribution of temperature and full velocity field simultaneously. The present experimental technique is applied to the horizontal fluid layer of a turbulent Rayleigh-Bérnard convection and the three-dimensional structures of thermal plumes are evaluated. The experimental results indicate that the structures of plumes are often correlated with the vertical velocity of the fluid, but they behave randomly in space, influenced by the large-scale turbulence evident in the middle of the fluid layer. 相似文献
4.
Feedback control of vortex shedding from a circular cylinder in a uniform flow at moderate Reynolds numbers is studied experimentally with the cylinder subjected to feedback cylinder oscillations in cross-flow direction. The cylinder oscillation is digitally phase shifted with respect to the shedding vortex and is controlled by velocity feedback from the shear layer of the cylinder wake. Possible attenuation of vortex shedding is demonstrated by hot-wire measurements of the flow field and its mechanisms are studied by simultaneous data sampling and flow visualization with the smoke wire method and a laser-sheet illumination technique. Measurement results reveal substantial reduction in the fluctuating reference velocity at the optimum phase control. Flow visualization study indicates that the shear layer roll-up and the eventual vortex formation are dynamically attenuated under the control which results in a modification of the near wake.List of symbols
A
amplitude of cylinder oscillation
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D
cylinder diameter
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E
u
power spectrum function for fluctuating velocity u
-
frequency
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R
radius of circular cylinder
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t
time
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u
streamwise mean velocity
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u
streamwise fluctuating velocity
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U
streamwise mean velocity of main flow
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u
r
mean reference velocity
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u
r
fluctuating reference velocity
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u
rf
fluctuating reference velocity after filtering
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y
c
cylinder displacement
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x, y, z
coordinates from the cylinder center (Fig. 1)
-
feedback coefficient
-
phase lag
The authors would like to express thanks to Professor K. Nagaya for his advice for designing electromagnetic actuators in the present experiments. 相似文献
5.
A graph with at least vertices is said to be distance -extendable if, for any matching of with edges in which the edges lie at distance at least pairwise, there exists a perfect matching of containing . In this paper we prove that every 5-connected triangulation on the projective plane of even order is distance 3 7-extendable and distance 4 -extendable for any . 相似文献
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Fujisawa Kiyoshi Okano Mitsuki Martín-Pastor Manuel López-Sánchez Rubén Elguero José Alkorta Ibon 《Structural chemistry》2021,32(1):215-224
Structural Chemistry - Experimental multinuclear determination of the chemical shifts, especially 15N and 109Ag, of five silver(I) trinuclear pyrazolate complexes, (PzAg)3, coupled with ZORA... 相似文献
8.
Abstract The pulse-echo-overlap method was used to measure the longitudinal and transverse wave velocities in single-crystal (100) and (111) samples of InSb up to 3 GPa at room temperature. The peculiar variations of the elastic constants were observed near the covalent-metallic transition. 相似文献
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