铷离子-铷原子混合阱飞行时间谱的拟合和仿真模拟

离子-原子混合阱是研究带电粒子-中性粒子低温反应的理想平台,直接甄别反应产物最准确的方法是带电粒子飞行时间谱,飞行时间谱峰的强度、位置(飞行时间)和宽度给出了相应带电粒子的强度和动能(温度)等信息.本文通过分析和模拟铷离子-原子混合阱中的飞行时间谱,获得了不同荷质比的离子绝对强度和温度等信息.具体说,首先使用Gumbel型极值分布函数飞行时间谱的谱峰,获得谱峰强度、位置和宽度等信息.然后对实验建模得到耦合的原子数和总带点离子的速率方程,用这些速率方程拟合实验数据,并结合实验测量到的绝对原子数,获得绝对的离子数强度.由此提供了一种标定探测器(本文使用的是微通道板)的方法.改变电离激光的波长和强度得到的标定因子是一致的,表明了这种方法的可靠性.此外,利用COMSOL Multiphysics模拟实验的飞行时间谱,仿真模拟结果表明离子动能大,谱峰宽度窄.本文对飞行时间谱的强度和宽度分析为冷原子光电离过程的离子-原子反应碰撞和带电粒子温度弛豫奠定了基础.     

在时域实验研究扩散诱导的Ramsey压窄

基于Duan-Lukin-Cirac-Zoller(DLCZ)方案,在时域上研究了扩散诱导的Ramsey压窄.以87Rb热原子系综为研究对象,观测到缓冲气体,激光束尺寸和镀石蜡Rb池均可以导致Ramsey压窄现象.实验结果和文献中重复相互作用模型预期的一致.     

Momentum Transfer Dependence of Two Types of the Broad Enhancement Phenomena： CO Spectra in the Valence Energy Region

Partial generalized oscillator strength densities of CO molecules related to the excitation of a 5σ or 1π electron are calculated by using multi-scattering self-consistent-field methods.Momentum transfer dependence of two types of the broad enhancement phenomena above the threshold with one-electron character,i.e. shape resonance and non-resonance enhancement,is studied.Our calculations show that the energy position of a non-resonance enhancement is related to the momentum transfer K.Therefore,electron impact based experiments can be used to identify the two types of the broad enhancement phenomena.     

氮气在100 eV以下的绝对振子强度密度

在入射电子能量为2500 eV、能量分辨为100 meV的条件下，得到了氮气在100 eV以下的绝对光学振子强度密度和广义振子强度密度；得到了23 eV和31.4 eV两个超激发态的绝对广义振子强度、并讨论了它们的动量转移依赖特性。     

氪的贝特面

用高分辨快电子能量损失谱方法, 在入射电子能量2.5 keV、激发能范围8-88 eV、动量转移范围0.056-3.56 ato. unit的条件下, 测量了氪的贝特面, 并进一步分析了贝特面的特性.     

氧分子的价壳层光学振子强度研究

在入射电子能量为1500eV、平均散射角为0°、能量分辨为60meV条件下，得到了氧分子在5.7—28.5eV能量区间的光学振子强度密度谱，获得了氧分子E³Σ^-_ｕ的ν′=0，1，2和2³Π_ｕ的ν′=0，1各振动能级的绝对光学振子强度，同时检验了我们的Bethe-Born转换因子外推到低能端的可靠性．将所得结果与前人的工作进行了比     

氢分子分立区和连续区(11.0—19.0 eV)的光学振子强度研究

利用通道规律,并考虑了转动分布对跃迁峰型的影响,对测量得到的绝对氢分子光吸收谱进行了分析．文中逐个确定了11.0—15.0 eV各振动态的振子强度,并得到了B′¹Σ⁺_u的解离强度．同时,利用多重散射Xα自洽场方法计算了氢分子分立区和连续区（11.0—19.0 eV）的光吸收谱．通过计算值和实验绝对测量值的比较可以说明,在自洽层次,文中理论计算值已能较好地说明本实验. 关键词：     

An all-optical phase detector by amplitude modulation of the local field in a Rydberg atom-based mixer

Recently, a Rydberg atom-based mixer was developed to measure the phase of a radio frequency (RF) field. The phase of the signal RF (SIG RF) field is down-converted directly to the phase of a beat signal created by the presence of a local RF (LO RF) field. In this study, we propose that the Rydberg atom-based mixer can be converted to an all-optical phase detector by amplitude modulation (AM) of the LO RF field; that is, the phase of the SIG RF field is related to both the amplitude and phase of the beat signal. When the AM frequency of the LO RF field is the same as the frequency of the beat signal, the beat signal will further interfere with the AM of the LO RF field inside the atom, and then the amplitude of the beat signal is related to the phase of the SIG RF field. The amplitude of the beat signal and the phase of the SIG RF field show a linear relationship within the range of 0 to π/2 when the phase of the AM is set with a difference π/4 from the phase of the LO RF field. The minimum phase resolution can be as small as 0.6° by optimizing the experimental conditions according to a simple theoretical model. This study will expand and contribute to the development of RF measurement devices based on Rydberg atoms.     

基于冷里德堡原子电磁感应透明的微波电场测量

在磁光阱中利用冷原子温度低,多普勒展宽小的优势获得了窄线宽的里德堡电磁感应透明(EIT)谱峰,结合Autler-Townes分裂效应(EIT-AT分裂)分别测量了多个频率的微波电场强度.结果显示,EIT-AT分裂间距与微波电场强度呈很好的线性关系,EIT-AT分裂方法可测量的微波电场强度线性区的下限可达222μV/cm,这个下限比传统热原子蒸汽池中EIT-AT分裂线性区的下限5 mV/cm提高了大约22倍,这对极弱微波电场的绝对校准非常有帮助.我们进一步利用EIT共振处探测光透过率的变化测量微波电场强度,对应的最小测量值可以小于1μV/cm,相应的灵敏度可达到1μV·cm^-1.Hz^-1/2.这些结果展示了冷原子样品在微波电场测量及其绝对校准方面的优势.     

Decay pathways of superexcited states of nitrous oxide

The ionization and ionic dissociation of the superexcited state of N20 are studied by using electron energy loss spectroscopy and positive ion time-of-flight mass spectroscopy at different momentum transfers; that is, 0 and 0.23 a.u. （atomic unit） . The transitions at 13.8 eV and 14.0 eV are reassigned as 3pπ（000） and 3pσ（000） converging to A^2∑＋, respectively. The competition between the main decay pathways of superexcited states at different momentum transfers is revealed. It is found that 3dσ converging to C^2∑＋ mainly decays into N2O^＋ while 4dσ can decay into both N2^O＋ and NO^＋.