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具有手性晶体结构的MnSb2O6其基态为螺旋磁序,对外磁场有着响应丰富的铁电性.本文通过助熔剂法制备了高质量MnSb2O6单晶.电子自旋共振谱(ESR)的结果表明其共振场具有类似铁磁材料的各向异性温度依赖关系.这一结果表明MnSb2O6基态的螺旋磁序在外磁场中形成了随磁场方向转动的圆锥磁序相(conical phase).对共振峰半高宽的进一步拟合得到一个意外小的临界指数,这表明MnSb2O6中的磁矩具有二维特征并且存在着较强的竞争相互作用. 相似文献
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Geometrical frustration in low-dimensional magnetic systems has been an intriguing research aspect, where the suppression of conventional magnetic order may lead to exotic ground states such as spin glass or spin liquid. In this work we report the synthesis and magnetism study of the monocrystalline Mn$_2$Ga$_2$S$_5$, featuring both the van der Waals structure and a bilayered triangular Mn lattice. Magnetic susceptibility reveals a significant antiferromagnetic interaction with a Curie-Weiss temperature $\theta_{\rm w}\sim-260$ K and a high spin $S=5/2$ Mn$^{2+}$ state. However, no long range magnetic order has been found down to 2 K, and a spin freezing transition is found to occur at around 12 K well below its $\theta_{\rm w}$. This yields a frustration index of $f = -\theta_{\rm w}/T_{\rm f} \approx 22$, an indication that the system is highly frustrated. The absence of a double-peak structure in magnetic specific heat compared with the $TM_2$S$_4$ compounds implies that the spin freezing behavior in Mn$_2$Ga$_2$S$_5$ is a result of the competition between exchange interactions and the 2D crystalline structure. Our results suggest that the layered Mn$_2$Ga$_2$S$_5$ would be an excellent candidate for investigating the physics of 2D magnetism and spin disordered state. 相似文献
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The double-doped La2/3+4x/3Sr1/3-4x/3Mn1-xMgxO3 samples with fixed Mn^3+/Mn^4+ ratio equal to 2/1 are investigated by means of magnetism and transport measurements. Phase separation is observed at temperature higher than T^onset c for x = 0.10 and 0.15. For x = 0.10, rather strong phase separation induces drastic magnetic random potential and results in the localization of carriers. Thus, the varlable-range hopping process dominates. For other samples, there is no or only weak phase separation above T^onset c. Thus, thermal activation mechanism is responsible for the high temperature transport behaviour. For x = 0.20 and 0.25, unexpected AFM behaviour is observed at low temperature. All these results are well understood by considering the special role of the "double-doping". 相似文献
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近年来,二维范德瓦尔斯磁性材料因为在自旋电子学的应用前景而吸引了广泛的关注.CrOCl是一种范德瓦尔斯磁性材料,理论预言其单层具有高达160 K的居里温度,因此吸引了广泛的关注。为了更好的理解这一材料的磁性,我们利用磁力显微镜研究了CrOCl变磁性相变中磁畴结构随磁场的变化。实验发现,在2K下CrOCl样品表面出现随磁场变化的方格条纹,给出了变磁性相比中反铁磁相和铁磁相竞争的图样,并通过二维快速傅里叶变换证实了CrOCl磁性的各向异性。我们的结果为后续研究CrOCl薄层的磁性提供了参考依据。 相似文献
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构造了一个新的等谱问题,利用相容性条件,推导出离散晶格方程的正族和负族。再利用迹恒等式,建立其Hamilton 结构。获得的离散方程族的达布变换、双线性化、对称、守恒率及其精确解也值得进一步研究。 相似文献
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