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流动CO2-H2O系统中白云岩的溶解研究使用了旋转盘和催化剂技术.实验在与CO2分压分别为30~105Pa达到平衡的H2O-CO2溶液中进行,结果表明远离平衡时的白云岩溶解速率R与旋速w有关.实验结果可用经过改进的扩散边界层(DBL)理论模型获得解释.此外,在溶液中加入能加速CO2转换反应的碳酸酐酶催化剂,促进了白云岩的溶解.发现不同CO2分压条件下存在着较大的差异.从这些实验观测可以得出结论:改进的DBL理论模型能以满意的精度预测远离平衡时不同CO2分压条件下的白云岩溶解速率及其变化机理. 相似文献
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本文证明了:用单纯形法迭代求解Kell和Minty例(式(1)的线性规划问题)时,如果用最大增量法确定入基变量,则从其任一顶点出发,迭代次数不超过n次. 相似文献
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本文提出了一组应力函数,采用边界配置方法计算了含中心裂纹不同截面形状柱体扭转时的应力强度因子。有关椭圆截面柱体的算例表明,本文方法具有良好的精度。同时,文中给出了圆、椭圆和矩形等不同截面柱体的计算结果。 相似文献
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Kinetics and rate-limiting mechanisms of dolomite dissolution at various CO_2 partial pressures 总被引:1,自引:0,他引:1
Techniques of rotating-disk and catalyst were used in investigating the kinetics of dolomite dissolution in flowing CO2-H2O system. Experiments run in the solutions equilibrated with various CO2 partial pressures (PCO2) from 30 to 100000 Pa. It shows that dissolution rates of
dolomite are related with rotating speeds at conditions far from equilibrium. This was explained by modified diffusion boundary layer (DBL) model. In addition, the dissolution rates increase after addition of carbonic anhydrase (CA) to solutions, where the CA catalyzes CO2 conversion. However, great differences occur among various CO2 partial pressures. The experimental observations give a conclusion that the modified DBL model enables one to predict dissolution rates and their behaviour at various PCO2 with satisfactory precision at least far from equilibrium. 相似文献
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