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1.
Nanocomposite ZrCN films consisting of nanocrystalline ZrCN grains embedded in nitrogen-doped amorphous carbon film are deposited by filtered cathodic vacuum arc technology under different bias voltages ranging from 50to 400 V.The influence of bias voltage on the characterization and the mechanical properties of the ZrCN films are investigated by x-ray diffraction,x-ray photoelectron spectroscopy,scanning electron microscopy,transmission electron microscopy,Raman spectroscopy and nano-indentation.The bias voltage has a subtle effect on the ZrCN grain size,which is around 9.5 nm and keeps almost constant.A slight increase of the bias voltage induces a relatively high sp~3 fraction about 40%in N-doped amorphous C films but leads to the graphitization of the films under a higher voltage.The best mechanical property of the ZrCN film with the hardness of 41 GPa is obtained under the bias voltage of 200 V,indicating the positive effect of slight increase of ion bombardment on the hardness of the films.  相似文献   
2.
Nitrogen-doped TiO2 nanotubes(TNTs)were prepared by ion implantation and anodic oxidation.The prepared samples were applied in photocatalytic(PC)oxidation of methyl blue,rhodamine B,and bisphenol A under light irradiation.To explore the influence of doped ions on the band and electronic structure of TiO2,computer simulations were performed using the VASP code implementing spin-polarized density functional theory(DFT).Both substitutional and interstitial nitrogen atoms were considered.The experimental and computational results propose that the electronic structure of TiO2 was modified because of the emergence of impurity states in the band gap by introducing nitrogen into the lattice,leading to the absorption of visible light.The synergy effects of tubular structures and doped nitrogen ions were responsible for highly efficient and stable PC activities induced by visible and ultraviolet(UV)light.  相似文献   
3.
Herein we report a prototypical electronic substrate specifically designed to serve the weakly interacting massive particles(WIMPs)detectors at the China Dark Matter Experiment(CDEX).Because the bulky high-purity germanium(HPGe)detectors operate under liquid-nitrogen temperatures and ultralow radiation backgrounds,the desired electronic substrates must maintain high adhesivity across different layers in such cold environment and be free from any radioactive nuclides.To conquer these challenges,for the first time,we employed polytetrafluoroethylene((C2F4)n)foil as the base substrate,in conjunction with ion implantation and deposition techniques using an independently developed device at Beijing Normal University for surface modification prior to electroplating.The remarkable peeling strengths of 0.88±0.06 N/mm for as-prepared sample and 0.75±0.05 N/mm for that after 2.5-days of soaking inside the liquid nitrogen were observed,while the regular standards commonly require 0.4 N/mm^0.6 N/mm for electronic substrates.  相似文献   
4.
结合N-back任务范式和持续操作测试(CPT)任务范式,设计出模拟认知性VDT持续监控作业的实验.根据实验数据:分别对脑力负荷评估指标体系中的6个评估指标在20个作业时间段的均值进行方差分析,差异显著;训练非线性自回归神经网络模型(NAR),对不同作业时间段脑力负荷在评估指标上发生的变化进行动态预测;再结合认知性VDT持续监控作业人因可靠性评估模型对人因可靠性概率进行预测.研究结果表明:该方法可动态预测不同时间段作业者的人因可靠性,实现认知性VDT持续监控作业任务的动态分配,提高系统可靠性.  相似文献   
5.
The nickel-base alloy is one of the leading candidate materials for generation IV nuclear reactor pressure vessel.To evaluate its stability of helium damage and retention,helium ions with different energy of 80 keV and 180 keV were introduced by ion implantation to a certain dose(peak displacement damage 1-10 dpa).Then thermal desorption spectroscopy(TDS)of helium atoms was performed to discuss the helium desorption characteristic and trapping sites.The desorption peaks shift to a lower temperature with increasing dpa for both 80 keV and 180 keV irradiation,reflecting the reduced diffusion activation energy and faster diffusion within the alloy.The main release peak temperature of 180 keV helium injection is relatively higher than that of 80 keV at the same influence,which is because the irradiation damage of 180 keV,helium formation and entrapment occur deeper.The broadening of the spectra corresponds to different helium trapping sites(He-vacancies,grain boundary)and desorption mechanisms(different Hen Vm size).The helium retention amount of 80 keV is lower than that of 180 keV,and a saturation limit associated with the irradiation of 80 keV has been reached.The relatively low helium retention proves the better resistance to helium bubbles formation and helium brittleness.  相似文献   
6.
利用基于密度泛函理论的线性缀加平面波(LAPW)法, 计算未掺杂和掺杂钨和钒的锐钛矿TiO2晶体的能带和电子态密度. 计算结果表明, 钨和钒的掺杂能够使锐钛矿TiO2的能带明显变窄.  相似文献   
7.
To understand the evolution of defects in SiC during irradiation and the influence of temperature,in situ luminescence measurements of 6H-SiC crystal samples were carried out by ion beam induced luminescence(IBIL)measurement under2 MeV H^+ at 100 K,150 K,200 K,250 K,and 300 K.A wide band(400-1000 nm)was found in the spectra at all temperatures,and the intensity of the IBIL spectra was highest at 150 K among the five temperatures.A small peak from 400 nm to 500 nm was only observed at 100 K,related with the D1 defect as a donor-acceptor pair(D-A)recombination.For further understanding the luminescent centers and their evolution,the orange band(1.79 eV)and the green band(2.14 eV)in the energy spectrum were analyzed by Gaussian decomposition,maybe due to the donor-deep defect/conduction band-deep defect transitions and Ti related bound excition,respectively.Finally,a single exponential fit showed that when the temperature exceeded 150 K,the two luminescence centers’resistance to radiation was reduced.  相似文献   
8.
开展了11组南海钙质砂和福建石英砂的分离式霍普金森压杆(SHPB)实验,试样相对密实度为90%,厚度分别为10、30和50 mm,得到了冲击荷载下钙质砂和石英砂的应变率时程曲线、应变时程曲线和应力应变关系。实验结果表明:通过严格装样技术可以减小实验设备产生的误差,改变试样厚度、子弹长度、整形器等是实现钙质砂应力平衡和恒应变率的主要手段。在相同的密实度和加载条件下,钙质砂的体积模量和剪切模量约为石英砂的10%,压缩强度和抗剪强度约为石英砂的30%。冲击荷载作用下钙质砂的动态力学性能与石英砂存在较大的差异,因此不能将已有石英砂的研究结果直接用于钙质砂。  相似文献   
9.
The electronic density of states and band structures of doped and un-doped anatase TiO2 were studied by the Linearized Augmented Plane Wave method based on the density functional theory. The calculation shows that the band structures of TiO2 crystals doped with transition metal atoms become narrower. Interesting, an excursion towards high energy level with increasing atomic number in the same element period could be observed after doping with transition metal atoms.  相似文献   
10.
Ag/Cu-doped titania nanotubes (Ag/TiNT, Cu/TiNT) are prepared by a metal vapor vacuum arc implanter. A scanning electronic microscope is employed for microstruetural characterization. The photo-current performance of doped titania nanotubes under UV and visible light is tested by an electrochemical workstation CS300UA, the results show that the absorption edge of both Ag/TiNT and Cu/TiNT samples shifts to the visible light region and the band gap becomes narrower. Ag/TiNT possesses better photo-current ability than Cu/TiNT under UV and visible light. Titania doped with Ag and Cu metal ions is also studied based on the linearized augmented planewave method implemented by WIEN2k package, the result becomes better with the experimental performance.  相似文献   
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