Stahl

Ohne Zusammenfassung     

Evidence for complex magnetic order in U2Zn17: A μ+ SR studySR study

μ⁺ SR-measurements in transversally applied magnetic fields of 2000 G and 4000 G on heavy-electron single crystal U₂Zn₁₇ are presented. They reveal that at least two types of interstitial sites are occupied by the positive muons. One of these sites (1/3, 2/3, 5/6) could be identified via induced local dipolar fields which aboveT _N=9.7 K can exactly be derived from the magnetic susceptibility. The corresponding component of the μ⁺-signal exhibits a steplike decrease by about 40% atT _N which is caused by the onset of a very broad distribution of static internal magnetic fields (ΔB≈1000 G) with zero average. Such a field distribution is in distinct contrast to dipolar-field calculations performed for the simple antiferromagnetic structure deduced from neutron diffraction. The remaining 60% of the muons contributing to this component belowT _N are subject to a narrow static field distribution (ΔB≈1 G). The induced dipolar fields at the site (1/3, 2/3, 5/6) are temperature-independent belowT _N. A weak dipolar coupling to the U-moments renders similar observations for muons occupying the second type of interstitial impossible.     

Pharmazeutische Pr?parate

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Bestimmung von Sauerstoff in Stahl

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Longitudinal field quenching studies in KCl and KBr — Evidence for a precursor muonium state

The repolarization of μ⁺ in a longitudinal field as a function of field strength has been measured at various temperatures in KCl and KBr single crystals. The data at room temperature in KCl are essentially in agreement with Ivanteret al. /1/ and Nishiyamaet al. /5/. The obtained quenching curves can be reasonably fitted by assuming that the long lived muonium state, seen directly in transverse field experiments by Kieflet al. /4/, is preceded by another short lived muonium state with reduced hf-coupling. It is also necessary to allow for electron spin exchange in the precursor state. The model fits yield the hyperfine frequency of the precursor state, its chemical lifetime and an electron spin flip rate. It is speculated that the precursor state and the temperature dependence of the fitted parameters reflect the early history of the μ⁺ in its terminal spur.     

μSR in UAs

UAs has the NaCl structure and undergoes a first order transition into a type I (single k) antiferromagnetic state at 123 K, followed by a second first order transition at 62 K into a type IA (double k) antiferromagnetic structure. μSR spectra of a powder sample were taken in zero and transverse fields up to 0.3 T. They cover the paramagnetic and the two antiferromagnetic states. The most significant features of our data are: i) a first increase of relaxation rate below T=180 K; ii) a sudden jump in both, relaxation rate and frequency shift at T=123 K, together with a small decrease in initial asymmetry (≈15%); iii) no μ⁺ spin rotation in zero field in the type I state; iv) an overlay, of 3 spectra in the type IA state. Two of these spectra show spin rotation in zero field. Their frequencies are clearly temperature dependent. In a transverse field of 5 and 10 mT the external field adds nearly fully to the internal field. Work supported in part by the Bundesministerium fur Forschung und Technologie, Federal Republic Germany.