Cumulant functions in optical coherence theory

Cumulant functions are introduced to describe the statistical state of a radiation field. These functions are simply related to the optical coherence functions but have some interesting features. It is shown that if the cumulant functions of all orders greater than some numberN ₀ vanish then they also vanish for all orders greater than 2. Thermal field is the only field having this property. This property holds whether the field is described by a classical stochastic process or by a quantum density operator. Further the particular operator ordering used in defining these cumulant functions for the quantized field affects only the second order cumulant function. To describe the statistical state of a vector field such as partially polarized or unpolarized radiation, one would need to introduce cumulant tensors.     

Gas phase activation energy for unimolecular dissociation of biomolecular ions determined by focused RAdiation for gaseous multiphoton ENergy transfer (FRAGMENT)

We present a novel approach for the determination of activation energy for the unimolecular dissociation of a large (>50 atoms) ion, based on measurement of the unimolecular dissociation rate constant as a function of continuous-wave CO(2) laser intensity. Following a short ( approximately 1 s) induction period, CO(2) laser irradiation produces an essentially blackbody internal energy distribution, whose 'temperature' varies inversely with laser intensity. The only currently available method for measuring such activation energies is blackbody infrared radiative dissociation (BIRD). Compared with BIRD, FRAGMENT: (a) eliminates the need to heat the surrounding ion trap and vacuum chamber to each of several temperatures (each requiring hours for temperature equilibration); (b) offers a three-fold wider range of effective blackbody temperature; and (c) extends the range of applications to include initially cold ions (e.g., gas-phase H/D exchange). Our FRAGMENT-determined activation energy for dissociation of protonated bradykinin, 1.2 +/- 0.1 eV, agrees within experimental error to the value, 1.3 +/- 0.1 eV, previously reported by Williams et al. from BIRD experiments. Copyright 1999 John Wiley & Sons, Ltd.     

Scattering and active acoustic control from a submerged spherical shell

This paper is concerned with the scattering from a submerged (heavy fluid) bilaminate spherical shell composed of an outer layer of steel, and an inner layer of radially polarized piezoelectric material. The methodology used includes separation formulas for the stresses and displacements, which in turn are used (coupled with spherical harmonics) to reduce the governing equations to linear systems of ordinary differential equations. This technique uses the full equations of elasticity rather than any of the various thin-shell approximations in determining the axisymmetric scattering from a shell, normal modes of vibration for the shell, as well as voltages necessary for annihilation of a scattered pressure due to insonification of the shell by an incident plane wave.     

Acoustic cloaking using layered pentamode materials

While receiving less attention in the literature than electromagnetic cloaking, theoretical efforts to define and create acoustic cloaks based upon mimicking coordinate transformations through use of metamaterials is of interest. The present work extends recent analysis of Norris [Proc. R. Soc. London, Ser. A 464, 2411-2434 (2008)] by considering a range of cloaks, from those comprised of fluid layers which are isotropic in bulk moduli with anisotropic density to those having anisotropic bulk moduli and isotropic density. In all but pure inertial varieties, fluid layers comprising the cloaks are pentamode materials governed by a special scalar acoustic equation for pseudopressure derived by Norris. In most cases presented, material properties of the fluid/pentamode layers are based upon target values specified by continuously varying properties resulting from theoretical coordinate transformations geared to minimize scattered pressure limited by realistic goals. The present work analyzes such cloaks for the specific case of plane wave scattering from an acoustically hard sphere. An initial exploration of the parameter space defining such cloaks (for example, material properties of its constituent layers, and operating frequency) is undertaken with a view toward "optimal" design.     

Decoupling approximations for structural acoustic interactions

The model problem of acoustic scattering by a baffled membrane is formally cast as a dual integral equation. A class of approximations are made to the equation's kernel and each gives rise to an analytically solvable problem. Each of these approximate problems corresponds to an existing physical theory which was derived in a complete by different manner. The present method of analysis systematically deduces these theories, suggests potentially useful new ones, and indicates where more theoretical studies are required.     

铌酸锶钡薄膜的微结构与电光性能的研究

本文叙述了使用溶胶凝胶法在MgO(0 0 1)的衬底上制备铌酸锶钡薄膜的过程 ,膜层厚度可达 5 μm。通过X射线衍射、摇摆曲线、扫描、拉曼散射光谱等方法研究了薄膜的微结构性能 ,实验发现 ,铌酸锶钡薄膜具有了较好的 (0 0 1)方向的优先取向性能 ,并且随着薄膜厚度的增加 ,其晶体取向性也会随之不断改进。熔石英的透明衬底上生长的SBN薄膜具有较大的电致双折射效应 ,其有效电光系数能够高达 6 6 2× 10 -11m/V。     

A modal Pritchard approximation for computing array element mutual impedance.

An investigation into the applicability and accuracy of Pritchard's approximation for closely packed transducer arrays is undertaken. A new, "modal" Pritchard approximation is developed, based upon normal modes of the acoustic medium, and is tested for arrays of acoustically hard spheres to ascertain its accuracy in determining the mutual acoustic radiation impedance between array elements. For ka approximately 1, it is found that the modal Pritchard approximation works quite well in approximating the mutual radiation impedance of a two-element array, even for relatively close spacing; but for arrays of three or more scatterers in close proximity the approximation may have relatively large errors. The effect of neglecting inter-element scattering is analyzed for the monopole-to-monopole scattering of various configurations of a three-element array and a sixteen-element double line array.     

Broadband optimization of a pentamode-layered spherical acoustic waveguide

Transformational acoustics offers the theoretical possibility of cloaking obstacles within fluids, provided metamaterials having continuously varying bulk moduli and densities can be found or constructed. Realistically, materials with the proper, continuously varying anisotropies do not presently exist. Discretely layered cloaks having constant material parameters within each layer are a viable alternative, but due to their discrete nature, may become ineffective outside of narrow frequency ranges. Because of such limitations, there is interest in finding discretely layered systems that can be effective in as wide as possible bandwidth without the need for unrealizable material properties within each layer. The present work introduces a novel methodology for finding optimal material parameters for use in such layered cloaks. In principle, the technique could be applied to any acoustic or electromagnetic scattering problem, but for purposes of demonstration, this paper considers a fluid-loaded acoustically hard sphere with a cloak that comprised layered pentamodes, whose material properties are constrained to lie within reasonable ranges relative to the density and bulk modulus of water.