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Marotta E Lapolla A Fedele D Senesi A Reitano R Witt M Seraglia R Traldi P 《Journal of mass spectrometry : JMS》2003,38(2):196-205
The Maillard reaction occurring between sugars and amino groups is important in living systems. When amino groups belonging to protein chains are involved, the Maillard reaction has been invoked as responsible for protein cross-linking and the production of 'toxic' compounds. The reaction leads to the production of a heterogeneous group of substances, usually called advanced glycation end products (AGEs). Classical analytical approaches, such as spectroscopic (ultraviolet, fluorescence) and mass spectrometric (matrix-assisted laser desorption/ionization, liquid chromatography/electrospray ionization mass spectrometry) methods, have shown that the digestion mixture is highly complex. However, there are clear differences between the digestion mixtures of glycated and unglycated human serum albumin (HSA). In the former case, possible glycated peptides belonging to the AGE peptide class may be identified. Tandem mass spectrometric experiments on selected species seemed to be promising as regards structural information, but it was thought of interest to undertake the present investigation, based on liquid chromatography/electrospray ionization Fourier transform mass spectrometry, in order to obtain definitive results on their elemental composition. Using this approach, about 20 glycated peptides were detected and their possible structures were postulated by examining the known sequence of HSA. 相似文献
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Harald Grosse Fedele Lizzi Harold Steinacker 《General Relativity and Gravitation》2011,43(9):2531-2539
We argue that some features of the standard model, in particular the fermion assignment and symmetry breaking, can be obtained in matrix model which describes noncommutative gauge theory as well as gravity in an emergent way. The mechanism is based on the presence of some extra (matrix) dimensions. These extra dimensions are different from the usual ones which give to a noncommutative geometry of the Grönewold-Moyal type, and are reminiscent of the Connes-Lott model, although the action is very different. 相似文献
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Sergio De NicolaRenato Fedele Margarita A. Man'koVladimir I. Man'ko 《Physics letters. A》2011,375(6):961-965
A novel approach, based on Fresnel tomography, to determine the entropy of two-dimensional optical Laguerre-Gaussian beams is presented and discussed. Numerical evaluations of the entropy distribution in the phase space associated with Laguerre-Gauss modes are presented. It is shown that the concept of Fresnel entropy provides a general criterion for studying and characterizing the vorticity of Laguerre-Gauss modes. 相似文献
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R. Fedele H. Schamel 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,27(3):313-320
An investigation to deepen the connection between the family of nonlinear Schr?dinger equations and the one of Korteweg-de
Vries equations is carried out within the context of the Madelung's fluid picture. In particular, under suitable hypothesis
for the current velocity, it is proven that the cubic nonlinear Schr?dinger equation, whose solution is a complex wave function,
can be put in correspondence with the standard Korteweg-de Vries equation, is such a way that the soliton solutions of the
latter are the squared modulus of the envelope soliton solution of the former. Under suitable physical hypothesis for the
current velocity, this correspondence allows us to find envelope soliton solutions of the cubic nonlinear Schr?dinger equation,
starting from the soliton solutions of the associated Korteweg-de Vries equation. In particular, in the case of constant current
velocities, the solitary waves have the amplitude independent of the envelope velocity (which coincides with the constant
current velocity). They are bright or dark envelope solitons and have a phase linearly depending both on space and on time coordinates. In the case of an arbitrarily
large stationary-profile perturbation of the current velocity, envelope solitons are grey or dark and they relate the velocity u0 with the amplitude; in fact, they exist for a limited range of velocities and have a phase nonlinearly depending on the combined
variable x-u0 s (s being a time-like variable). This novel method in solving the nonlinear Schr?dinger equation starting from the Korteweg-de
Vries equation give new insights and represents an alternative key of reading of the dark/grey envelope solitons based on the fluid language. Moreover, a comparison between the solutions found in the
present paper and the ones already known in literature is also presented.
Received 20 February 2002 and Received in final form 22 April 2002 Published online 6 June 2002 相似文献
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Laura Fedele Francesco Pernechele Sergio Bobbo Mauro Scattolini Roman Stryjek 《Fluid Phase Equilibria》2009
In this paper, solubility measurements of CO2 in pure pentaerythritol tetraoctanoate (PEC8) between 273 and 343 K are presented. The experiments were performed according to the static, synthetic method. The data are represented using the Peng–Robinson equation of state with the Huron–Vidal mixing rules and the UNIQUAC equation for the excess Gibbs Energy (gE) at infinite pressure. This system shows immiscibility in liquid phase, with lower critical end point (LCEP) at T = 268 ± 0.1 K and xCO2=0.98±0.001 and upper critical end point (UCEP) at the critical point of pure CO2. 相似文献
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