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Spectra of single tetra-tert-butylterrylene chromophore molecules embedded in an amorphous polyisobutylene matrix as microprobes were recorded. The individual temperature dependences of the spectral linewidths for the same single molecules (SMs) in a broad temperature interval (1.6 < T < 40 K) have been measured. This enabled us to separate the contributions of tunneling two-level systems and quasilocalized low-frequency vibrational modes (LFMs) to the observed linewidths. The analysis of the T dependences yields the values of LFM frequencies and SM-LFM coupling constants for the LFMs in the local environment of a given chromophore. Pronounced distributions of the observed parameters of LFMs were found. This result can be regarded as the first direct experimental proof of the localized nature of LFMs in glasses. 相似文献
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Optics and Spectroscopy - Experiments carried out in recent years using single-molecule spectroscopy to study the low-temperature dynamics of some molecular solid-state media with a disordered... 相似文献
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The subject of investigation is multiple-beam Bragg diffraction of light, i.e., the formation of a highly effective multiple-beam field representing a superposition of equidistant monochromatic acoustic waves with determinate phases and amplitudes using a nonaxial TeO2 deflector. It is shown theoretically and experimentally that the anisotropic character of interaction considerably changes the basic parameters of multiple-beam diffraction (compared with the isotropic case): the net diffraction efficiency grows to 100%, and the frequency band expands noticeably. A modulator splitting the initial laser radiation into five beams of equal intensity with a net efficiency approaching 100% is designed. 相似文献
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V. N. Bagratashvili Yu. G. Vainer V. S. Doljikov S. F. Koliakov A. A. Makarov L. P. Malyavkin E. A. Ryabov E. G. Silkis V. D. Titov 《Applied Physics A: Materials Science & Processing》1980,22(1):101-105
The method of spectroscopy of spontaneous Raman scattering (RS) with time resolution has been applied for the first time to
diagnose the process of multiphoton ir molecular excitation (MPE). Some aspects of RS diagnostics of MPE processes are being
analyzed. It has been shown experimentally on SF6 and CF3I molecules that it is possible to study such important characteristics of excitation process as the fraction of molecules
involved in the process of excitation, vibrational energy distribution of molecules, stochastization of inner molecular energy. 相似文献
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The optical dynamics of a doped amorphous system, tetra-tert-butylterrylene in amorphous polyisobutylene, has been experimentally studied by the spectra of single impurity molecules measured at temperatures of 2, 4.5, 7, and 15 K. The study of the temporal evolution of the fluorescence excitation spectra of the molecules under consideration made it possible to unambiguously establish the individual identity of the spectra of particular molecules and to analyze their multiplet structure. Repeated scanning of a selected spectral range with subsequent summation of the data made it possible to considerably reduce the errors that arise upon single scanning of the spectra of single molecules. The majority of the spectral trails detected were in agreement with the model of two-level systems. Jumps of spectral lines due to transitions in such systems were observed at all temperatures. 相似文献
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A. Ya. Vainer K. M. Dyumaev A. M. Kovalenko A. V. Vishnyakov K. I. Zelikson Sh. N. Sukharskaya 《Doklady Chemistry》2017,477(1):235-238
A new strategy was proposed for the synthesis of fluorene-containing indole polyphenols, based on the Suzuki–Miyaura reaction of hexabrominated symmetric indole trimer with the monoboryl N,N'-di[9,9'-bis(3',5'-dimethoxybenzyl)fluoren-2'-yl]aniline derivative and subsequent chemical transformations. The prepared compound was applicable for the development of a promising positive resist for electron-beam nanolithography capable of forming patterns with a 12 nm resolution. 相似文献