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1.
Russian Physics Journal - 相似文献
2.
Some features of software implementation of the Pulay scaling procedure are considered. The advantages of the single value decomposition method for maintaining well-conditionality of the scale factor determination problem are demonstrated. The necessity of using a rational number of scale factors is shown. The possibility of obtaining transferable scale factors with the Pulay method and thus predict the vibrational spectra of related compounds is emphasized. 相似文献
3.
Dmitry Panchenko 《Random Structures and Algorithms》2004,24(1):65-74
Using Talagrand's concentration inequality on the discrete cube {0, 1}m we show that given a real‐valued function Z(x) on {0, 1}m that satisfies certain monotonicity conditions one can control the deviations of Z(x) above its median by a local Lipschitz norm of Z at the point x. As one application, we obtain a deviation inequality for the number of k‐cycles in a random graph. © 2003 Wiley Periodicals, Inc. Random Struct. Alg., 2004 相似文献
4.
Lasing and discharge in mixtures of SF6 with hydrogen and hydrocarbons are investigated. If the chemical reaction is initiated by a self-sustained discharge (a generator
with both an inductive and capacitive energy storage can be used), the maximum lasing efficiency is attained at high values
of the ratio E/p (where E is the electric field intensity and p is the pressure in the mixture) if shaped electrodes and preionization of the discharge gap are employed. For the first time,
the lasing efficiency obtained in a nonchain HF laser is as high as 10% of the energy deposit and 4.5% of the stored energy
for a specific radiation energy of ≈140 J/(l atm). At high efficiencies, the emission spectrum of the nonchain HF laser significantly
broadens and cascade lasing at P(3-2) → P(2-1) → P(1-0) vibrational transitions for several rotational lines is realized. 相似文献
5.
E. N. Abdullin N. G. Ivanov B. M. Kovalchuk I. N. Konovalov V. F. Losev A. N. Panchenko Yu. N. Panchenko V. S. Skakun V. F. Tarasenko A. G. Yastremsky 《Laser Physics》2006,16(1):104-115
Two-high power excimer laser systems with square (25 × 25 cm) and circular (with a diameter of 40 cm) cross sections of the
output laser beam are described. The first (second) system consists of four (five) excimer lasers. The experimental results
on the generation of the high-quality high-power laser pulses are presented. Laser beams with a pulse duration of 1–250 ns,
a divergence of 0.01 mrad, a spectral line width of 0.01 cm−1, and a pulse energy of up to 330 J are obtained.
Original Text ? Astro, Ltd., 2006. 相似文献
6.
S. N. Lyashchuk B. V. Panchenko A. G. Gershikov Yu. G. Skrypnik V. P. Bezrodnyi 《Theoretical and Experimental Chemistry》1991,27(2):146-151
Combined methods of quantum chemistry and molecular mechanics have been used to investigate the structure and energetics of formation of sulfene, and also N-methanesulfonylpyridinium and oxypyridinium halides, which are intermediates in catalytic alkanesulfonylation reactions. The potential energy surface of ion-ion interactions of N-methanesulfonylpyridinium halides has been analyzed. The results have been applied in identifying kinetically indistinguishable mechanisms of general basic and nucleophilic catalysis in processes of alkanesulfonylation of phenols.Institute of Physical Organic Chemistry and Coal Tar Chemistry, Academy of Sciences of the Ukrainian SSR, Donetsk. Donetsk University. Translated from Teoreticheskaya i Eksperimental'naya Khimiya, Vol. 27, No. 2, pp. 159–165, March–April, 1991. Original article submitted November 9, 1989. 相似文献
7.
Savos'kin M. V. Yaroshenko A. P. Mochalin V. N. Panchenko B. V. 《Russian Journal of Applied Chemistry》2003,76(6):906-908
Sorption of industrial oil by expanded graphite prepared from residual graphite hydrosylfate at 300-900°C was studied. The sorption isotherms of both neat oil and oil from its aqueous suspension were measured. The sorption capacity for oil was studied as influenced by the specific surface area and specific volume of expanded graphite sorbent. 相似文献
8.
Yurii N. Panchenko Sergei V. Krasnoshchiokov Philip George Charles W. Bock 《Structural chemistry》1992,3(1):15-26
The results of complete geometry optimizations of the high energy stable gauche,Trans,trans- and gauche,Cis,trans- rotamers of hexa-1,3,5-trienes are reported at the RHF/6-31G//RHF/B-31G level. The angles of rotation around one of the single C-C bonds are found to be 33.7° and 45.5°, respectively. The corresponding harmonic force fields of these molecules are also reported at this level and corrected using scale factors transferred from buta 1,3-diene. Aspecial scale factor was used for the central C=C double bond stretching coordinate to take into account vibronic coupling. The theoretical vibrational frequencies, calculated with the scaled quantum mechanical (SQM) force fields, allow a complete interpretation of the experimental vibrational spectra of these molecules.Preliminary results were reported at the Austin XII Symposium on Molecular Structure, Austin, TX, February 28 through March 3, 1988, S 18, p. 111 (USA) and at the XIXth European Congress on Molecular Spectroscopy, Dresden, September 4 through September 8, 1989, p. 226 (GDR). 相似文献
9.
Falko Böttger‐Hiller Patrick Kempe Dr. Gerhard Cox Dr. Alexander Panchenko Dr. Nicole Janssen Dr. Albrecht Petzold Prof. Dr. Thomas Thurn‐Albrecht Lars Borchardt Dr. Marcus Rose Prof. Dr. Stefan Kaskel Colin Georgi Prof. Dr. Heinrich Lang Prof. Dr. Stefan Spange 《Angewandte Chemie (International ed. in English)》2013,52(23):6088-6091
10.