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1.
Laurens Kooijman Dr. Matthias Schuster Christian Baumann Simon Jurt Dr. Frank Löhr Dr. Boris Fürtig Prof. Dr. Peter Güntert Prof. Dr. Oliver Zerbe 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2020,132(47):21151-21158
To achieve efficient proton pumping in the light-driven proton pump bacteriorhodopsin (bR), the protein must be tightly coupled to the retinal to rapidly convert retinal isomerization into protein structural rearrangements. Methyl group dynamics of bR embedded in lipid nanodiscs were determined in the dark-adapted state, and were found to be mostly well ordered at the cytosolic side. Methyl groups in the M145A mutant of bR, which displays only 10 % residual proton pumping activity, are less well ordered, suggesting a link between side-chain dynamics on the cytosolic side of the bR cavity and proton pumping activity. In addition, slow conformational exchange, attributed to low frequency motions of aromatic rings, was indirectly observed for residues on the extracellular side of the bR cavity. This may be related to reorganization of the water network. These observations provide a detailed picture of previously undescribed equilibrium dynamics on different time scales for ground-state bR. 相似文献
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3.
A. V. Anisimov A. A. Grishkyan Kh. A. Gaisina E. A. Viktorova 《Chemistry of Heterocyclic Compounds》1994,30(4):420-421
1-Allyloxy-2-allylthio-4-methylbenzene rearranges in NN-diethylaniline at 215°C with migration of allyloxy and allylthio groups to form 2,4-dimethyl-6-allyl-7-hydroxy-2,3dihydrobenzothiophene.M. V. Lomonosov State University, Moscow 119899. Translated from Khimiya Geterotsiklicheskikh Soedinenii, No. 4, pp. 480–482, 1994. Original article submitted March 5, 1994. 相似文献
4.
In two dimensional electron systems with Coulomb or dipolar interactions, a direct transition, whether first or second order, from a liquid to a crystalline state is forbidden. As a result, between these phases there must be other (micro-emulsion) phases which can be viewed as a meso-scale mixture of the liquid and crystalline phases. We investigate the transport properties of these new electronic phases and present arguments that they are responsible for the various transport anomalies that have been seen in experiments on the strongly correlated 2DEG in high mobility semiconductor devices with low electron densities. 相似文献
5.
S. I. Anisimov V. V. Zhakhovskii N. A. Inogamov K. Nishihara A. M. Oparin Yu. V. Petrov 《JETP Letters》2003,77(11):606-610
Molecular-dynamics (MD) simulation of the destruction of a crystal film heated by a femtosecond laser pulse was carried out. Heating is assumed to be instantaneous, because there is no time for the material to be displaced during the pulse. Film destruction is caused by the interaction of unloading waves. It can be considered as a model of a more complex process of splitting out of a thin surface layer from a massive target in the case where the layer remains solid after heating. It was found that the crystal order is broken due to the stretching strains and to the strong anisotropy of residual stress, resulting in a bipartition of the layer separating from the target. The lattice stretching and the formation of anisotropic stresses are due to the expansion of a heated lattice. 相似文献
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Set-Valued and Variational Analysis - 相似文献
7.
A. Yu. Anisimov 《Physics of Atomic Nuclei》2004,67(3):640-647
We provide a detailed numerical study of the influence of thermal effects on the original picture of the Affleck-Dine baryogenesis. These effects are found to modify the results greatly in some cases. We estimate the baryon/entropy ratio and provide numerical results on the typical behavior of the charge as a function of the strength of the potential and other parameters. 相似文献
8.
Boris Goldfarb 《Topology and its Applications》2004,140(2-3):267-294
New compactifications of symmetric spaces of noncompact type X are constructed using the asymptotic geometry of the Borel–Serre enlargement. The controlled K-theory associated to these compactifications is used to prove the integral Novikov conjecture for arithmetic groups. 相似文献
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10.
Letters in Mathematical Physics - 相似文献