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1.
《Current Applied Physics》2020,20(2):244-248
We theoretically demonstrate a broadband mode converter and multiplexer based on plasmonic waveguides loaded with structured dielectrics. The proposed device can realize conversions between a fundamental TM0 mode and a first order TM1 mode, as well as (de)multiplex them with another TM0 mode. Our design exhibits as wide as 400 nm bandwidth and as short as 6~7 μm coupling length. This work has potential application in high density photonic integrated devices for both computing and communication applications.  相似文献   
2.
In this paper we have proposed a technique based on image analysis of the surface plasmon excitation at the metal-dielectric interface of inside silver coated fused silica capillary glass tube. Chemical deposition technique has been used for the deposition of silver. Angular interrogation in Kretschmann-like configuration is realized by non-radial transverse illumination of this cylindrical dielectric-metal-dielectric (C-DMD) structure with a He–Ne laser source. Here the uniform film deposition of the inside surface of the capillary is not that crucial except within the transversely illuminated working area concerned. Moreover, the proposed technique has been validated experimentally for sensing different aqueous dielectric samples inserted inside the tube.  相似文献   
3.
We study light propagation in nanoscale periodic structures composed of dielectric and metal in the visible range. We demonstrate that diffraction curves of nonuniform waveguide arrays can be tailored by varying the geometric and dielectric features of the waveguides. The results obtained from a proper formulation of coupled mode theory for nonuniform arrays are validated through numerical solution of Maxwell equations in frequency domain.  相似文献   
4.
Two different hybrid materials composed of gold nanoparticles (AuNPs) supported on either commercial niobium oxide HY 340 or mesoporous niobium oxide catalyzed the Friedel-Crafts alkylation of anisole by benzyl chloride. Excitation of the surface plasmon of the supported AuNPs allowed the reaction to occur at lower temperatures by acting as an alternative heat source. The localized heating produced via plasmon excitation permitted the acid catalyzed reaction to occur - at the Lewis acid sites on the Nb2O5 support - at 80 °C while thermal-dark reactions using a conventional heat source, required temperatures of 120 °C or higher. The catalytic activity of the tested hybrid materials decreased with storage time. However, the deactivation showed to be reversible upon lyophilisation indicating that the nature of the deactivation could be due to water adsorption.  相似文献   
5.
This tutorial provides a broad perspective on the synthesis, characterization, and size-dependent dynamics of nanoscale materials. Synthetic strategies include bottom-up, top-down, and hybrid strategies in gas and condensed phases. Advances in imaging and structure analysis provide the spatial information to correlate dynamic phenomena to structure in complex nanocomposites. Excited-state dynamics can change with material dimensions due to changes in the properties of the host and due to unique nanoscale phenomena such as plasmon resonance in metals and quantum confinement in semiconductors.  相似文献   
6.
Thin film tandem solar cells made of amorphous and microcrystalline silicon provide renewable energy at the benefit of low material consumption. As a drawback, these materials do not posses the high carrier mobilities of their crystalline counterpart which limits the feasible material thickness. For maintaining the light absorption as high as possible, photon management is required. Here we show that metallic nanodiscs that sustain localized plasmon polaritons can increase the efficiency of such solar cells if they are incorporated into the dielectric intermediate reflector separating the top and the bottom cell. We provide quantitative estimates for the possible absorption enhancement of optimized bi-periodic nanodiscs that are feasible for fabrication. Emphasis is also put on discussing the impact of obliquely incident sun light on the solar cell performance.  相似文献   
7.
Jin Li  Yundong Zhang  Hanyang Li  Chengbao Yao  Ping Yuan 《Optik》2013,124(24):6772-6775
The paper proposes the metal–insulator–metal (MIM) waveguides with different tooth-shapes (rectangle-tooth and triangle-tooth) and calculates the corresponding power spectrums by discrete Fourier transform. The finite difference time domain (FDTD) simulation results show that the spectrum transformations reveal the significant differences in the two structures with the same tooth-depth, such as amplitudes, amplitudes difference and spacing of the two peaks. The study will be useful in waveform modulation in the communication wavelength. Furthermore, the spectrum may also be used to detect different nanostructures based on the corresponding transformations.  相似文献   
8.
Surface electromagnetic waves are characterized by the intrinsic spin‐orbit interaction which results in the fascinating spin‐momentum locking. Therefore, directional coupling of light to surface waves can be achieved through chiral nanoantennas. Here, we show that dielectric nanoantenna provides chiral response with strong spectral dependence due to the interference of electric and magnetic dipole momenta when placed in the vicinity of the metal‐air interface. Remarkably, chiral behaviour in the proposed scheme does not require elliptical polarization of the pump beam or the geometric chirality of the nanoantenna. We show that the proposed ultracompact and simple dielectric nanoantenna allows for both directional launching of surface plasmon polaritons on a thin gold film and their demultiplexing with a high spectral resolution.  相似文献   
9.
等离激元效应在光催化体系中的集成为实现广谱光吸收提供了一个新的途径,然而等离激元热电子的较低迁移率和不确定扩散方向使得其光催化效率仍较低.等离激元金属与n型半导体接触后,其界面间会形成肖特基结.在特定波长太阳光照射下,等离激元金属将其表面等离子体能量聚集在表面自由电子上,进而产生热电子.当这些热电子具有的能量高于肖特基势垒时,热电子便可注入到半导体导带上.与此同时,半导体上的电子可以通过肖特基接触发生回流,与金属上的空穴复合,进而降低半导体-等离激元金属复合材料的光催化性能.因此,为了提高光催化效率,如何调控等离激元热电子迁移和充分利用等离激元效应是一个重要挑战.本文尝试将"表面异质结"与肖特基结相结合的复合结构,得以有效地调控等离激元热电子的迁移.在该复合结构中,金纳米颗粒和铂纳米颗粒分别作为等离激元吸光单元和助催化剂,集成在TiO_2纳米片表面.其中"表面异质结"是由TiO_2纳米片的两种不同表面晶面所构成,我们选择由{001}和{101}两组晶面组成的TiO_2纳米片作为半导体衬底.该结构中的{001}晶面导带能级高于{101}导带能级,因而电子由高能级的{001}流向低能级的{101}晶面,可以用来引导等离激元热电子从可见光响应的金纳米颗粒向TiO_2进行高效转移.通过巯基丙酸的桥联作用,将等离激元Au纳米颗粒锚定在TiO_2纳米片的{001}晶面上,获得Au-TiO_2{001}样品.另一方面,利用TiO_2纳米片自身光生电荷导向性光沉积,得到与{101}晶面结合形成的Au-TiO_2{101}样品.我们对两组样品进行光电流和光催化产氢实验对比,确认在"表面异质结"诱导下Au-TiO_2{001}样品中Au产生的光生热电子可以更好地注入到TiO_2纳米片导带上.我们进一步通过光沉积Pt纳米颗粒来判定光生电子所能到达的区域,验证了以上结论.与此同时,肖特基结由铂纳米颗粒与TiO_2纳米片所形成,可以促使电子由TiO_2向铂纳米颗粒进行转移,而避免发生向金纳米颗粒的反向迁移,从而在Au-TiO_2体系中实现高效的单向载流子转移.基于该设计,等离激元光催化剂实现了明显改善的全谱光催化产氢性能.本文为全谱光催化的复合结构理性设计提供了一个新的思路.  相似文献   
10.
Photoluminescence of a conjugated polymer in the presence of surface plasmons on metallic nanoparticles is studied. A layered device structure was constructed that enabled control over nanoparticle diameter and separation between the polymer and nanoparticles layers. The dependence of the surface plasmon evanescent field and energy transfer has been investigated with the largest enhancement in photoluminescence observed at a 40 nm distance separation between the fluorophore and the surface plasmon. A spectrum of surface plasmon resonances ranging from the emission to the absorption energies of the conjugated polymer revealed largest enhancements when the resonance was tuned to the conjugated polymer emission energy. At peak photoluminescence the maximum photoluminescent enhancement was found to be 5.6 times of the photoluminescence of the control structure and the total integrated enhancement was 5.9 times.  相似文献   
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