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宁凯杰  张庆礼  周鹏宇  杨华军  许兰  孙敦陆  殷绍唐 《物理学报》2012,61(12):128102-128102
采用提拉法成功生长尺寸为φ30 mm× 75 mm的15at.%Yb3+:Gd2SiO5单晶, 并用Reitveld全谱拟合方法确定了其晶格常数、原子坐标和温度因子等参数. 用吸收光谱计算了Yb3+离子2F7/22F5/2能级跃迁的振子强度、谱线强度、跃迁概率、 能级寿命和积分发射截面等光谱参数, 并根据激光性能评估得出结论: 表明该晶体具有较大的阈值特性, 有望采用大功率激光二极管泵浦实现可调谐或超快激光输出.  相似文献
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用提拉法生长了新型激光晶体5at%Yb3+:YNbO4,测量了它的吸收和光致发光光谱,计算了它的吸收和发射截面,并对其激光性能进行了评估.Yb3+:YNbO4的吸收半峰全宽为17nm,吸收峰位于933,955,974和1003nm,相应的吸收截面分别为0.73×10^-20,1.85×10^-20,0.86×10^-20。和0.44×10^-20cm2;最大吸收截面值为Yb3+:YAG的两倍.光致发光谱的发射带的中心位置处于1020nm附近,相应的半高宽为41nm,是Yb3+:YAG的3倍;Yb3+:YNbO4在955,974,1005,1021和1030nm处都有着较大的发射截面,截面值分别为0.69×10^-20,0.86×10^-20,1.81×10^-20,1.11×10^-20和0.57×10^-20cm2,最大发射截面值与Yb3+:YAG相当.Yb3+:YNbO4晶体的宽发射带有利于实现相应波长的超短脉冲和可调谐激光输出,表明它是在这些领域非常有希望的全固态工作物质.  相似文献
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The crystal structural parameters of Nd 3+-doped rare earth orthotantalate Gd x Lu 1 x TaO 4(x = 0.85) are determined by applying the Rietveld refinement to its X-ray diffraction,and its emission and excitation spectra at 77 K are analysed.The relativistic model of ab initio self-consistent DV-Xα method,which is applied to the cluster NdO 8 in Gd x Lu 1 x TaO 4,and the effective Hamiltonian model are used to investigate its spin-orbit and crystal-field parameters.The free-ions and crystal-field parameters are fitted to the experimental energy levels at 77 K with a root-mean-square deviation of 14.92 cm 1.According to the crystal-field calculations,96 levels of Nd 3+ are assigned.Finally,the fitting results of free-ions and crystal-field parameters are compared with those already reported for Nd 3+:YAlO 3.The results indicate that the free-ion parameters are similar to those of the Nd3+ in Gdx Lu1-x TaO4 and YAlO 3 hosts,and the crystal-field interaction of Nd3+ in Gdx Lu1-x TaO4 is stronger than that in YAlO 3.  相似文献
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The crystal structural parameters of Nd 3+-doped rare earth orthotantalate Gd x Lu 1 x TaO 4(x = 0.85) are determined by applying the Rietveld refinement to its X-ray diffraction,and its emission and excitation spectra at 77 K are analysed.The relativistic model of ab initio self-consistent DV-Xα method,which is applied to the cluster NdO 8 in Gd x Lu 1 x TaO 4,and the effective Hamiltonian model are used to investigate its spin-orbit and crystal-field parameters.The free-ions and crystal-field parameters are fitted to the experimental energy levels at 77 K with a root-mean-square deviation of 14.92 cm 1.According to the crystal-field calculations,96 levels of Nd 3+ are assigned.Finally,the fitting results of free-ions and crystal-field parameters are compared with those already reported for Nd 3+:YAlO 3.The results indicate that the free-ion parameters are similar to those of the Nd3+ in Gdx Lu1-x TaO4 and YAlO 3 hosts,and the crystal-field interaction of Nd3+ in Gdx Lu1-x TaO4 is stronger than that in YAlO 3.  相似文献
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