啁啾脉冲频域干涉测量技术的扰动重构理论模拟研究

利用啁啾脉冲的频域干涉测量技术,可实现对超快光学瞬态过程的单发诊断,此方法的时间分辨率和单发时间测量范围分别与啁啾脉冲的谱宽和脉冲宽度及光谱仪的工作性能有关。当两束线性啁啾脉冲进入光谱仪后,相同的频谱成分会发生干涉形成频谱干涉条纹,如果其中一束脉冲受到外界扰动的影响,可根据干涉条纹的形状重构出扰动的具体形式。理论研究和数值模拟了由频谱干涉图重构外界附加扰动的过程,模拟结果显示重构出的扰动同附加的真实扰动符合得较好;在频谱记录面有限的情况下,重构出的扰动信号带有强烈的振荡,通过平滑处理有效地抑制了振荡。     

Ultrafast third-order optical nonlinearities in DMSO

The third-order optical nonlinearities of dimethyl sulfoxide(DMSO) are investigated using the optical Kerr effect(OKE) and Z-scan techniques with femtosecond pulses.We are able to fit the OKE signal theoretically by convolving the autocorrelation of the incident pulse intensity profile with the impulse responses of the samples,illustrating the instantaneous nonlinear response of DMSO.We verify that the purely electronic cloud distortion causes the observed signal for DMSO.The Z-scan technique is used to estimate the third-order susceptibility of DMSO,which is about a quarter of that for CS2 and mainly comes from the nonlinear refraction with an intensity of less than 140 GW/cm2.