掺杂在GaAs材料中Be受主能级之间的跃迁

通过远红外吸收谱、光致发光光谱和拉曼散射光谱,对均匀掺杂在GaAs材料中Be受主能级之间的跃迁进行了研究.实验中使用的GaAs:Be样品是通过分子束外延设备,生长在半绝缘(100) GaAs衬底之上的外延单层.在4.2 K温度下,对样品分别进行了远红外吸收光谱、光致发光光谱、Raman光谱的实验测量.在远红外吸收光谱中,清楚地观察到了从Be受主1S_(3/2)Γ_8基态到它的三个激发态2P_(3/2)Γ_8, 2P5/2Γ_8和2P5/2Γ_7之间的奇宇称跃迁吸收峰.跃迁能量与先前文献中报道的符合得很好.从光致发光光谱中,观察到了Be受主从1S_(3/2)Γ_8基态到2S_(3/2)Γ_8激发态的两空穴跃迁的发光峰,从而间接地找到了两能级之间的跃迁能量.在Raman光谱中,清楚地分辨出来了Be受主从1S_(3/2)Γ_8基态到2S_(3/2)Γ_8激发态偶宇称跃迁的拉曼散射峰,直接得到了两能级间的跃迁能量.对比发现,分别直接和间接得到的1S_(3/2)Γ8基态到2S_(3/2)Γ8激发态跃迁能量结果是一致的.     

量子限制效应对δ掺杂GaAs/AlAs多量子阱中铍受主态寿命的影响

采用远红外时间分辨光谱，研究了量子限制效应对δ掺杂在GaAs/AlAs多量子阱中铍（Be）受主态寿命的影响.在低温下的远红外吸收谱中，清楚地观察到了三条主要吸收线，它们分别来源于铍受主从基态到它的三个奇宇称激发态的跃迁.实验结果表明：随着量子限制效应的增强，受主激发态寿命而减少，实验测得体材料中Be受主2p激发态的寿命是350 ps，而阱宽10 nm的多量子阱中的寿命是55 ps.量子限制效应对布里渊区折叠声学声子模的影响增强了受主带内空穴与声学声子相互作用，从而加快了受主带内空穴的弛豫过程. 关键词： 量子限制效应 受主态寿命 时间分辨光谱 δ掺杂')" href="#">δ掺杂     

Intra-acceptor hole relaxation in Be δ-doped GaAs/AlAs multiple quantum wells

This paper studies the dynamics of intra-acceptor hole relaxation in Be δ-doped GaAs/AlAs multiple quantum wells(MQW) with doping at the centre by time-resolved pump-probe spectroscopy using a picosecond free electron laser for infrared experiments.Low temperature far-infrared absorption measurements clearly show three principal absorption lines due to transitions of the Be acceptor from the ground state to the first three odd-parity excited states respectively.The pump-probe experiments are performed at different temperatures and different pump pulse wavelengths.The hole relaxation time from 2p excited state to 1s ground state in MQW is found to be much shorter than that in bulk GaAs,and shown to be independent of temperature but strongly dependent on wavelength.The zone-folded acoustic phonon emission and slower decay of the wavefunctions of impurity states are suggested to account for the reduction of the 2p excited state lifetime in MQW.The wavelength dependence of the 2p lifetime is attributed to the diffusion of the Be atom δ-layer in quantum wells.     

量子限制受主远红外电致发光器件的制备与测量

采用分子束外延技术生长GaAs/AlAs三量子阱,并在中间的GaAs阱中δ-掺杂浅受主杂质Be原子,制作出量子限制受主远红外Teraherz原型电致发光器件.实验上测量得到4.5 K时器件的电致发光谱（EL）和电传输特性（I-V曲线）.在EL发射谱中清楚地观察到222 cm^-1处宽的尖峰,这来源于Be受主奇宇称激发态到其基态的辐射跃迁,而非辐射弛豫过程则使发射谱的信号很弱.另外在I-V曲线中072和186 V的位置出现两个共振隧道贯穿现象,分别对应于中间δ-掺杂量子阱受主能级1s_3/2(Γ₆+Γ₇)到左边非掺GaAs量子阱中HH带,及右边非掺杂GaAs量子阱中HH重空穴带到中间掺杂GaAs量子阱中Be受主杂质原子奇宇称激发态2p_5/2(Γ₆+Γ₇)能级的共振隧穿.     

量子限制受主远红外电致发光器件的制备与测量

采用分子束外延技术生长GaAs/AlAs三量子阱,并在中间的GaAs阱中δ-掺杂浅受主杂质Be原子,制作出量子限制受主远红外Teraherz原型电致发光器件.实验上测量得到4.5 K时器件的电致发光谱（EL）和电传输特性（I-V曲线）.在EL发射谱中清楚地观察到222 cm^-1处宽的尖峰,这来源于Be受主奇宇称激发态到其基态的辐射跃迁,而非辐射弛豫过程则使发射谱的信号很弱.另外在I-V曲线中072和186 V的位置出现两个共振隧道贯穿现象,分别对应于中间δ-掺杂量子阱受主能级1s_3/2(Γ₆+Γ₇)到左边非掺GaAs量子阱中HH带,及右边非掺杂GaAs量子阱中HH重空穴带到中间掺杂GaAs量子阱中Be受主杂质原子奇宇称激发态2p_5/2(Γ₆+Γ₇)能级的共振隧穿. 关键词： 量子限制效应 电致发光 共振隧穿效应 δ-掺杂GaAs/AlAs三量子阱