全文获取类型
收费全文 | 1064篇 |
免费 | 197篇 |
国内免费 | 46篇 |
专业分类
化学 | 273篇 |
晶体学 | 4篇 |
力学 | 176篇 |
综合类 | 12篇 |
数学 | 208篇 |
物理学 | 634篇 |
出版年
2024年 | 4篇 |
2023年 | 11篇 |
2022年 | 23篇 |
2021年 | 30篇 |
2020年 | 29篇 |
2019年 | 32篇 |
2018年 | 22篇 |
2017年 | 53篇 |
2016年 | 51篇 |
2015年 | 37篇 |
2014年 | 56篇 |
2013年 | 73篇 |
2012年 | 40篇 |
2011年 | 63篇 |
2010年 | 49篇 |
2009年 | 59篇 |
2008年 | 79篇 |
2007年 | 59篇 |
2006年 | 65篇 |
2005年 | 59篇 |
2004年 | 56篇 |
2003年 | 50篇 |
2002年 | 41篇 |
2001年 | 54篇 |
2000年 | 27篇 |
1999年 | 25篇 |
1998年 | 22篇 |
1997年 | 30篇 |
1996年 | 21篇 |
1995年 | 25篇 |
1994年 | 6篇 |
1993年 | 10篇 |
1992年 | 4篇 |
1991年 | 7篇 |
1990年 | 6篇 |
1989年 | 7篇 |
1988年 | 3篇 |
1987年 | 8篇 |
1986年 | 3篇 |
1985年 | 3篇 |
1984年 | 2篇 |
1981年 | 1篇 |
1979年 | 1篇 |
1977年 | 1篇 |
排序方式: 共有1307条查询结果,搜索用时 31 毫秒
1.
Dr. Joaquim Torra Dr. Felipe Viela Dr. Diego Megías Dr. Begoña Sot Prof. Cristina Flors 《Chemistry (Weinheim an der Bergstrasse, Germany)》2022,28(19):e202200026
CRANAD-2 is a fluorogenic curcumin derivative used for near-infrared detection and imaging in vivo of amyloid aggregates, which are involved in neurodegenerative diseases. We explore the performance of CRANAD-2 in two super-resolution imaging techniques, namely stimulated emission depletion (STED) and single-molecule localization microscopy (SMLM), with markedly different fluorophore requirements. By conveniently adapting the concentration of CRANAD-2, which transiently binds to amyloid fibrils, we show that it performs well in both techniques, achieving a resolution in the range of 45–55 nm. Correlation of SMLM with atomic force microscopy (AFM) validates the resolution of fine features in the reconstructed super-resolved image. The good performance and versatility of CRANAD-2 provides a powerful tool for near-infrared nanoscopic imaging of amyloids in vitro and in vivo. 相似文献
2.
Titanium dioxide (TiO2) is regarded as an important prototype photocatalytic material for several decades. The charge carrier kinetics determines the photocatalytic properties of TiO2 materials; this is found to be greatly dependent on electronic structures. It has been revealed that the intrinsic intermediate gap states (intrinsic GSs) play a significant role in charge carrier kinetics that drive the photocatalytic processes of TiO2 materials, which are not well summarized until now. Motivated by this thought, the purpose of this review focuses on physiochemical science of the intrinsic GSs of TiO2 materials and their important role in charge carrier kinetics. We first give a summary on the chemical resources of the intrinsic GSs in TiO2 and their physiochemical nature. Their general energy distribution, charge carrier population, and the associated thermodynamic properties are also elaborated from an overall viewpoint. We further carefully summarize and compare the experimental studies on the energy and the density distribution of the intrinsic GSs and discuss the associated chemical resources and charge carrier localizations. Trapping is the dominant function of intrinsic GSs in the charge carrier kinetics of TiO2 materials. The significant effect of trapping on the transport, recombination, and interfacial transfer of charge carriers are also comprehensive summarized. Furthermore, the effects of charge carrier kinetics on photocatalytic performances are also discussed to some extents. Because of the importance of intrinsic GSs in modulating charge carrier kinetics, it is expected to increase the photocatalytic activity by engineering the intrinsic GSs, not only for TiO2 materials, but also for the other semiconductor photocatalysts. 相似文献
3.
《Physics letters. A》2020,384(7):126152
Derived from quantum waves immersed in an Abelian gauge potential, the quasiperiodic Aubry-André-Harper (AAH) model is a simple yet powerful Hamiltonian to study the Anderson localization of ultracold atoms. Here, we investigate the localization properties of ultracold atoms in quasiperiodic optical lattices subject to a non-Abelian gauge potential, which are depicted by non-Abelian AAH models. We identify that the non-Abelian AAH models can bear the self-duality. We analyze the localization of such non-Abelian self-dual optical lattices, revealing a rich phase diagram driven by the non-Abelian gauge potential involved: a transition from a pure delocalization phase, then to coexistence phases, and finally to a pure localization phase. This is in stark contrast to the Abelian counterpart that does not support the coexistence phases. Our results establish the connection between localization and gauge symmetry, and thus comprise a new insight on the fundamental aspects of localization in quasiperiodic systems, from the perspective of non-Abelian gauge potential. 相似文献
4.
5.
《Physics letters. A》2019,383(29):125918
In this paper, the acoustic localization characteristics of the two-dimensional phononic crystals with slit tube defect are investigated theoretically and experimentally. In contrast to the typical formation pattern of defect states, the proposed defect states are created by replacing a slotted tube in the center of perfect phononic crystal. Compared to perfect phononic crystal, the proposed structure can effectively localize waves of specific frequencies in the point defect and improve the acoustic pressure amplification. Then the effects of the geometric parameters of the slotted tube on the acoustic localization characteristics are studied. Numerical results show that the resonant frequency and acoustic pressure amplification amplitude could be effectively modulated by the geometric parameters of the slotted tube. Experimental results are in good agreement with the simulation results. 相似文献
6.
We investigate a single-qubit state transfer protocol along a channel featuring diagonal diluted disorder. In the regime where the source and destination sites are weakly coupled to the channel, we report the possibility of transmitting quantum states with high fidelity as well as establishing end-to-end entanglement in that sort of configuration. We further discuss how the performance of the protocol depends upon the availability of extended states within the disordered channel. 相似文献
7.
8.
9.
基于头相关传递函数数据库的传统双耳声源定位方法的定位角度往往被限定在头相关传递函数数据库的离散测量点上。当头相关传递函数数据库的测量方位角间隔较大时,这类算法的性能会显著下降,这就是典型的离格问题。该文提出了基于加权宽带稀疏贝叶斯学习的离格双耳声源定位算法。首先该算法建立离格双耳信号的稀疏表示模型,然后利用双耳相干与扩散能量比特征对各个频点进行加权以降低噪声和混响的影响,最后通过加权宽带稀疏贝叶斯学习方法估计离格声源的方位角。实验结果表明,该算法在各种复杂的声学环境下都有着较高的定位精度和鲁棒性,特别是提高了离格条件下的声源定位性能。 相似文献
10.