This article presents vertically coupled, rectangular complementary split-ring resonator-shaped quad-band double-negative (DNG) metamaterial unit cells, that is, having both negative permittivity and permeability, which redirect negative refractive and also are not found in nature. The metamaterial is fabricated on magnesium zinc ferrite-based flexible microwave substrates, and the flexible substrates are chosen with two different concentrations of magnesium (Mg) denoted by Mg
30 and Mg
50 for 30% and 50% of Mg, which possess dielectric constants of 4.32 and 3.15 and loss tangents of 0.003 and 0.005, respectively. The proposed metamaterials are demonstrated by utilizing the CST microwave simulator, and their effective parameters are extracted according to the Nicolson-Ross-Wire method. With Mg
30, the prepared, flexible metamaterial shows measured resonances at 3.70 GHz, 7 GHz, 8.60 GHz, and 9.78 GHz, whereas with Mg
50 it shows the measured resonances at 4.10 GHz, 7.70 GHz, 9.33 GHz, and 10.62 GHz. Very good effective medium ratios (EMR) along with DNG properties are obtained, namely 6.5 and 5.85 for Mg
30 and Mg
50, respectively, with a physical dimension of 12.5 × 9.5 mm
2 for both of the unit cells
. Also, the electric field, magnetic field, and surface current distribution at different resonances and the polarization insensitivity at different polarization angles were observed. Thus, the designed new flexible substrate microwave materials based on DNG metamaterials are potential candidates for S-, C- and X-band applications, as well as for flexible microwave technologies.
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