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Encapsulation of Functional Organic Compounds in Nanoglass for Optically Anisotropic Coatings 下载免费PDF全文
Matthias Stöter Dr. Bernhard Biersack Dr. Sabine Rosenfeldt Markus J. Leitl Dr. Hussein Kalo Prof. Dr. Rainer Schobert Prof. Dr. Hartmut Yersin Prof. Geoffrey A. Ozin Prof. Dr. Stephan Förster Prof. Dr. Josef Breu 《Angewandte Chemie (International ed. in English)》2015,54(16):4963-4967
A novel approach is presented for the encapsulation of organic functional molecules between two sheets of 1 nm thin silicate layers, which like glass are transparent and chemically stable. An ordered heterostructure with organic interlayers strictly alternating with osmotically swelling sodium interlayers can be spontaneously delaminated into double stacks with the organic interlayers sandwiched between two silicate layers. The double stacks show high aspect ratios of >1000 (typical lateral extension 5000 nm, thickness 4.5 nm). This newly developed technique can be used to mask hydrophobic functional molecules and render them completely dispersible in water. The combination of the structural anisotropy of the silicate layers and a preferred orientation of molecules confined in the interlayer space allows polymer nanocomposite films to be cast with a well‐defined orientation of the encapsulated molecules, thus rendering the optical properties of the nanocoatings anisotropic. 相似文献
3.
The axisymmetric buckling (delamination) of a circular disk (plate) with a penny-shaped crack is analyzed using a continuum
model, piecewise-homogeneous model, and the three-dimensional linearized theory of stability. The FEM is used. The analysis
is carried out using various singular and ordinary finite elements. The numerical results obtained indicate that it is not
necessary to use singular finite elements to solve the problem
Published in Prikladnaya Mekhanika, Vol. 43, No. 9, pp. 120–129, September 2007. 相似文献
4.
将层板横截面分为含裂纹区与不含裂纹区,在每一区内,根据夏变函数理论与特征函数展开法,得到了各自区内满足所有支配方程、裂纹表面边界条件与层间连续条件的位移与应力的特征展开式,然后利用分区广义变分原理满足裂纹表面边界以外的边界条件以及两区之间的交界条件,并由此求得奇异场控制量(广义应力强度因子)。 相似文献
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Study on failure process of delaminated stiffened composite plates under compression 总被引:4,自引:0,他引:4
Failure behavior of the delaminated stiffened composite plates under compression is studied by the finite element method,
based on a Global-Local variational model. A virtual crack closure technique and a self-adaptive grid moving scheme are proposed
to predict the delamination growth process. The contact effect along the delamination front is considered. The numerical results
show that the influences of the distribution and location of the stiffeners, the configuration and size of the delamination,
the boundary condition and the contact upon the failure behavior of the plates are significant.
The project supported by the National Natural Science Foundation of China (59975014) 相似文献
8.
《Composite Interfaces》2013,20(5):469-478
The effect of carbon fiber textile for flexural reinforcement to deteriorated reinforced concrete floor slab is tested in laboratory by cutting out six specimens from existing structure aged more than 70 years. The repair method between concrete and carbon fiber textile is used as experimental parameter. From the test results, deformation, bond characteristic of carbon fiber textile and the applicability of carbon fiber textiles to flexural reinforcement of floor slabs are discussed. 相似文献
9.
《Composite Interfaces》2013,20(5):337-349
The lamination of composite elements such as sheets or fibres made from ceramic powders represents a cheap and easy way of making tough ceramics. The fabrication and failure behaviour of such layered structures is described. It is shown that crack growth along the interfaces is dominated by dynamic effects due to the storage of excess elastic energy and that effects of loading state, in the silicon carbide/graphite system at least, appear to be relatively unimportant. Crack deflection at interfaces is also discussed and it is shown that observations made in these systems are not consistent with existing theories. Various possibilities are investigated. 相似文献
10.
Ugur Gven 《Acta Mechanica Solida Sinica》2011,24(6):506-509
In this work a bi-material beam exhibiting partly bilinear behaviour under a uniform temperature change is analyzed. The essence of solution is based on the approach of Timoshenko’s mechanics of materials. The main aim of the present analysis is to understand the effect of the bilinear behaviour on the peeling moment. This theoretical mechanics model mentioned here can give us useful insights to improve the resistance against the delamination. 相似文献