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采用短碳链的表面活性剂溴代十二烷基三甲基溴化铵为模板剂,合成了具有较大粒径和超小孔径分布的单分散树枝状介孔二氧化硅纳米球(记为DMSNs-C12).通过扫描电子显微镜(SEM)、透射电子显微镜(TEM)、X射线衍射能谱(XRD)、傅里叶变换红外光谱(FT-IR)、以及氮气吸附脱附曲线对制备的DMSNs-C12进行了形貌、晶体结构、化学组成、孔体积、比表面积等分析.结果表明:与传统的、以溴代十六烷基三甲基溴化铵为模板剂制备的单分散树枝状二氧化硅纳米球相比(DMSNs-C16),DMSNs-C12颗粒尺寸明显增大,褶皱结构消失,孔道尺寸急剧减小.原因是随着碳链减小,表面活性剂相互斥力减弱,影响微乳液形成,最终导致结构差异. 相似文献
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ＩｎｔｒｏｄｕｃｔｉｏｎＴｈｅｏｉｌｆｏｒｍａｔｉｏｎｉｎｓｅｄｉｍｅｎｔｂａｓｉｎｓ ,ｉｔｓｄｉｓｐｌａｃｅｍｅｎｔ,ｔｒａｎｓｐｏｒｔａｎｄａｃｃｕｍｕｌａｔｉｏｎ ,ａｎｄｔｈｅｆｉｎａｌｆｏｒｍａｔｉｏｎｏｆｏｉｌｄｅｐｏｓｉｔｓｈａｖｅｂｅｅｎｏｎｅｏｆｔｈｅｋｅｙｐｒｏｂｌｅｍｓｉｎｔｈｅｅｘｐｌｏｒａｔｉｏｎｏｆｏｉｌ＿ｇａｓｒｅｓｏｕｒｃｅｓ.Ｈｏｗｈａｓｏｉｌｂｅｅｎａｃｃｕｍｕｌａｔｅｄｉｎｔｈｅｐｒｅｓｅｎｔｌｏｏｐａｃｃｏｒｄｉｎｇｔｏｔｈｅｍｅｃｈａｎｉｃｓｏｆｉｍｍｉｓｃ… 相似文献
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Numerical simulation of careful parallel arithmetic of oil resources migration-accumulation of Tanhai Region (three-layer) was done. Careful parallel operator splitting-up implicit iterative scheme, parallel arithmetic program, parallel arithmetic information and alternating-direction mesh subdivision were put forward.Parallel arithmetic and analysis of different CPU combinations were done. This numerical simulation test and the actual conditions are basically coincident. The convergence estimation of the model problem has successfully solved the difficult problem in the fields of permeation fluid mechanics, computational mathematics and petroleum geology. 相似文献
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For the system of multilayer dynamics of fluids in porous media, the second order upwind finite difference fractional steps schemes applicable to parallel arithmetic are put forward. Some techniques, such as calculus of variations, energy method, multiplicative commutation rule of difference operators, decomposition of high order difference operators and prior estimates are adopted. Optimal order estimates are derived to determine the error in the second order approximate solution. These methods have already been applied to the numerical simulation of migration-accumulation of oil resources. 相似文献
5.
From such actual conditions as the effects of characteristics of miltilayer petroleum geology and permeation fluid mechanics, a new numerical model is put forward and coupling splitting-up implicit interactive scheme is formed. For the actual situation of Dongying hollow ( four-layer ) and Tanhai region ( three-layer ) of Shengli Petroleum Field, the numerical simulation test results and the actual conditions are coincident. 相似文献
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陈熙;韩玉玖;张纪生 《力学与实践》1980,2(1)
实际燃烧装置的喷雾炬内,燃料滴的直径约为几十到几百微米.目前积累的大量有关液滴燃烧的实验资料,大多是用悬挂滴法与多孔球法获得的,所用液滴直径为一到十几毫米,比实际喷雾中的滴径大的多.因而,燃烧过程中自然对流的影响较大,而化学动力学因素的影响较小.研究压力对燃料滴燃烧速度的影响,可以用改变环境介质压力的办法,在宽广的数 相似文献
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The research of the miscible oil and water displacement problem with moving boundary values is of great value to the history of oil-gas transport and accumulation in the basin evolution as well as to the rational evaluation in prospecting and exploiting oil-gas resources. The mathematical model can be described as a coupled system of nonlinear partial differential equations with moving boundary values. For the twodimensional bounded region, the upwind finite difference schemes are proposed. Some techniques, such as the calculus of variations, the change of variables, and the theory of a priori estimates, are used. The optimal orderl2-norm estimates are derived for the errors in the approximate solutions. The research is important both theoretically and practically for the model analysis in the field, the model numerical method, and the software development. 相似文献
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非溶剂致相分离法作为制备聚偏氟乙烯（PVDF）膜一种常用的方法已得到广泛推广，但因影响其成膜因素诸多，至今没有一种较好的协同效果．作者介绍了不同溶剂、聚合物的浓度、添加剂的种类和浓度、凝胶浴的组成和温度、蒸发时间及后处理等制膜条件对膜的影响，以期为优化制膜工艺提供参考． 相似文献
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多层油资源运移聚集并行数值模拟,其功能是重建油气盆地的运移聚集演化史,对于油资源的评价,确度油藏位置,估计油藏贮量均具有重要的价值.从生产实际出发,提出数学模型,构造大规模精细并行计算的耦合算子分裂隐式迭代格式,设计了并行计算程序和并行计算的信息传递和交替方向网格剖分方法.并对不同的网格步长进行了并行计算和分析.对滩海地区进行精细数值模拟,计算结果在油田位置等方面和实际情况相吻合.对模型问题(非线型性耦合问题)进行数值分析,得到最佳阶L2误差估计,解决了这一计算渗流力学和石油地质的困难问题. 相似文献
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