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C. Xia 《Journal of Molecular Spectroscopy》2005,229(1):39-46
The CO-stretching vibration-rotation spectra of CO-H2S, CO-D2S, and CO-HDS complexes have been studied in the 2150 cm−1 region using a supersonic slit-jet expansion and a tunable diode laser spectrometer. The spectra were analyzed with the help of very recent microwave pure rotational studies of the same complexes. Two bands were assigned for each of the symmetric hydrogen sulfide isotopes, corresponding to the two nuclear spin modifications, para and ortho. The band origins were blue shifted, relative to the free CO molecule, by about 3.8 cm−1 for CO-H2S and 4.3 cm−1 for CO-D2S. These are considerably smaller shifts than exhibited by the related CO-water complexes, indicating that the intermolecular forces in CO-H2S are weaker and more isotropic. 相似文献
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Zheng Su 《Journal of Molecular Spectroscopy》2005,232(1):112-114
Rotational transitions of the propylene oxide-20Ne and propylene oxide-22Ne molecular adducts have been measured, in the frequency region from 4 to 18 GHz, using a pulsed jet Fourier Transform microwave spectrometer. The transition frequencies were used to refine the rotational and distortion spectroscopic constants obtained from the previous free jet millimetre wave measurements of the complex. No splittings due to the methyl group internal rotation were detected. 相似文献
76.
考虑双层碳纳米管的层间范德华力,采用连续介质力学的波动理论,建立了双层碳纳米管中周向导波传播模型,研究周向导波的频散现象.通过与单层碳纳米管结果的比较表明,双层碳纳米管中周向导波的传播表现出更为明显的频散特性,出现更多的模态干涉现象,并发现在某些特殊频率处出现成对模态的消失与新启现象. 相似文献
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We analyze a modified van der Pol–Duffing electronic circuit, modeled by a tridimensional autonomous system of differential equations with Z2-symmetry. Linear codimension-one and two bifurcations of equilibria give rise to several dynamical behaviours, including periodic, homoclinic and heteroclinic orbits. The local analysis provides, in first approximation, the different bifurcation sets. These local results are used as a guide to apply the adequate numerical methods to obtain a global understanding of the bifurcation sets. The study of the normal form of the Hopf bifurcation shows the presence of cusps of saddle-node bifurcations of periodic orbits. The existence of a codimension-four Hopf bifurcation is also pointed out. In the case of the Takens–Bogdanov bifurcation, several degenerate situations of codimension-three are analyzed in both homoclinic and heteroclinic cases. The existence of a Hopf–Shil'nikov singularity is also shown. 相似文献
79.
The response of a system of two nonlinearly coupled van der Poloscillators to a principal parametric excitation in the presence ofone-to-one internal resonance is investigated. The asymptoticperturbation method is applied to derive the slow flow equationsgoverning the modulation of the amplitudes and the phases of the twooscillators. These equations are used to determine steady-stateresponses, corresponding to a periodic motion for the starting system(synchronisation), and parametric excitation-response andfrequency-response curves. Energy considerations are used to studyexistence and characteristics of limit cycles of the slow flowequations. A limit cycle corresponds to a two-period amplitude- andphase-modulated motion for the van der Pol oscillators. Two-periodmodulated motion is also possible for very low values of the parametricexcitation and an approximate analytic solution is constructed for thiscase. If the parametric excitation increases, the oscillation period ofthe modulations becomes infinite and an infinite-period bifurcationsoccur. Analytical results are checked with numerical simulations. 相似文献
80.
参数激励耦合系统的复杂动力学行为分析 总被引:3,自引:0,他引:3
分析了耦合van der Pol振子参数共振条件下的复杂动力学行为.基于平均方程,得到了参数平面上的转迁集,这些转迁集将参数平面划分为不同的区域,在各个不同的区域对应于系统不同的解.随着参数的变化,从平衡点分岔出两类不同的周期解,根据不同的分岔特性,这两类周期解失稳后,将产生概周期解或3—D环面解,它们都会随参数的变化进一步导致混吨.发现在系统的混沌区域中,其混吨吸引子随参数的变化会突然发生变化,分解为两个对称的混吨吸引子.值得注意的是,系统首先是由于2—D环面解破裂产生混吨,该混吨吸引子破裂后演变为新的混吨吸引子,却由倒倍周期分岔走向3—D环面解,也即存在两条通向混沌的道路:倍周期分岔和环面破裂,而这两种道路产生的混吨吸引子在一定参数条件下会相互转换. 相似文献