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71.
72.
17O solid state NMR of organic materials is developing rapidly. This article provides a snapshot of the current state of development of this field. The NMR techniques and enrichment protocols that are driving this progress are outlined. The 17O parameters derived from solid-state NMR experiments are summarized and the structural sensitivity of the approach to effects such as hydrogen bonding highlighted. The prospects and challenges for 17O solid-state NMR of biomolecules are discussed. 相似文献
73.
B. Macke B. Ségard 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2003,23(1):125-141
This paper deals with the apparent superluminal propagation of electromagnetic pulses in a linear dispersive medium. One specifically
examines the possibility that the pulse leaving the medium may be nearly identical to the incident one (low distortion) and
in significant advance of it (strongly negative group-delays). Favourable conditions are obtained in a dilute medium where
the required anomalous dispersion originates in an ensemble of narrow absorption or gain lines. Analytical expressions of
the advancement of the pulse centre-of-gravity and of the lowest order distortion are established from the transfer-function
of the medium. The experiments already achieved with arrangements involving a single absorption-line or a gain-doublet are
analysed in detail and compared. The considerable difficulties to overcome in order to attain advancements comparable to the
pulse width without important distortion are pointed out. New and promising schemes involving a narrow dip in a gain profile
or absorption-doublets are proposed.
Received 4 July 2002 / Received in final form 8 November 2002 Published online 4 February 2003
RID="a"
ID="a"e-mail: bruno.macke@univ-lille1.fr
RID="b"
ID="b"Unité Mixte de Recherche de l'Université et du CNRS (UMR 8523) 相似文献
74.
P. Karvonen T. Sonoda I. D. Moore J. Billowes A. Jokinen T. Kessler H. Penttilä A. Popov B. Tordoff J. Äystö 《The European physical journal. Special topics》2007,150(1):283-284
The ion guide technique was developed in Jyv?skyl? during the early 1980's. In the ion guide the reaction recoil products
are stopped and thermalized in high purity helium gas where they remain ionic due to high ionization potential of helium atoms.
Different designs of ion guide exist for light-ion induced fusion reactions, for heavy-ion induced fusion and for proton induced
fission. Although the IGISOL method is fast and universal it is chemically unselective and in many cases relatively inefficient.
In order to address these deficiencies in the technique, a new laser ion source project, FURIOS (Fast Universal Resonant laser
Ion
Source), commenced in 2004. In addition, resonance ionization spectroscopy has been tested off – line within a sextupole ion
beam
guide. 相似文献
75.
Zhongzhi Zhang Shuigeng Zhou Lichao Chen Jihong Guan Lujun Fang Yichao Zhang 《The European Physical Journal B - Condensed Matter and Complex Systems》2007,59(1):99-107
We propose a geometric growth model for weighted
scale-free networks, which is controlled by two tunable parameters.
We derive exactly the main characteristics of the networks, which
are partially determined by the parameters. Analytical results
indicate that the resulting networks have power-law distributions of
degree, strength, weight and betweenness, a scale-free behavior for
degree correlations, logarithmic small average path length and
diameter with network size. The obtained properties are in agreement
with empirical data observed in many real-life networks, which shows
that the presented model may provide valuable insight into the real
systems. 相似文献
76.
R. Bachelard A. Antoniazzi C. Chandre D. Fanelli X. Leoncini M. Vittot 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2007,42(1):125-132
The intensity of an electromagnetic wave interacting self-consistently
with a beam of charged particles as in a free electron laser, displays large
oscillations due to an aggregate of particles, called the macro-particle. In
this article, we propose a strategy to stabilize the intensity by re-shaping
the macro-particle. This strategy involves the study of the linear stability
(using the residue method) of selected periodic orbits of a mean-field model. As
parameters of an additional perturbation are varied, bifurcations occur in the
system which have drastic effect on the modification of the self-consistent
dynamics, and in particular, of the macro-particle. We show how to obtain an
appropriate tuning of the parameters which is able to strongly decrease the
oscillations of the intensity without reducing its mean-value. 相似文献
77.
In this work, we study long-range correlations in a “Scherzo-Duetto di Mozart” score (K-73x) for two violins. This is a fascinating piece, as the second violin part is upside down on the same sheet below the first violin, and some parts are like a palindrome. Given such ingenious structure, it is expected the existence of long-range correlations in the score structure. In order to quantify long-range correlations, we considered the music score as a sequence of integer numbers, each of them corresponding to last common denominator units of note. By using detrended fluctuation analysis (DFA), correlations are quantified by means of the scaling exponent that reflects the type of correlations for a given distance between neighbors note. The following conclusions can be drawn from the analysis: (a) For about 10-25 neighbor note distances, correlations are similar to 1/f-noise. This is an interesting finding since it has been shown that pleasant sounds for humans display a behavior similar to 1/f noise. (b) As the neighbor note distance increases, the long-range correlations decays continuously. For some score sections, the music score behaves like non-correlated (i.e., purely random) noise. Summing up, the results show that the studied Mozart's score contains a certain degree of correlation for relatively small note distances, and becomes close to non-correlated behavior for long note distances. We considered also the sequence constructed by considering the distance between the simultaneously played notes of the two violins. Interestingly, for relatively small neighbor note distances, a scaling behavior similar to that found for individual violins is also displayed. In some sense, this is an expression of the specific structure (palindromes plus upside down construction) used by Mozart in the composition of this music score. Although we focused on a particular high-art music score, our results suggest that modern methods borrowed from statistical physics can be useful for the systematic study of music composition techniques. 相似文献
78.
Xitong Liu Wei Wang Zhenqiang Fan Wanning Huang Lixing Luo Canglei Yang Prof. Dr. Jing Zhang Prof. Dr. Jianfeng Zhao Prof. Dr. Lei Zhang Prof. Dr. Wei Huang 《Chemistry (Weinheim an der Bergstrasse, Germany)》2021,27(40):10448-10455
Fullerene host-guest constructs have attracted increasing attention owing to their molecular-level hybrid arrangements. However, the usage of simple carbazolic derivatives to bind with fullerenes is rare. In this research, three novel carbazolic derivatives, containing a tunable bridging linker and carbazole units for the capturing of fullerenes, are rationally designed. Unlike the general concave-convex interactions, fullerenes could interact with the planar carbazole subunits to form 2-dimensional hexagonal/quadrilateral cocrystals with alternating stacking patterns of 1 : 1 or 1 : 2 stoichiometry, as well as the controllable fullerene packing modes. At the meanwhile, good electron-transporting performances and significant photovoltaic effects were realized when a continuous C60⋅⋅⋅C60 interaction channel existed. The results indicate that the introduction of such carbazolic system into fullerene receptor would provide new insights into novel fullerene host-guest architectures for versatile applications. 相似文献
79.
80.