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21.
Advances on the Determination of the Astatine Pourbaix Diagram: Predomination of AtO(OH)2− over At− in Basic Conditions 下载免费PDF全文
Dumitru‐Claudiu Sergentu Dr. David Teze Dr. Andréa Sabatié‐Gogova Dr. Cyrille Alliot Ning Guo Dr. Fadel Bassal Dr. Isidro Da Silva Prof. Dr. David Deniaud Dr. Rémi Maurice Dr. Julie Champion Dr. Nicolas Galland Dr. Gilles Montavon 《Chemistry (Weinheim an der Bergstrasse, Germany)》2016,22(9):2964-2971
It is generally assumed that astatide (At?) is the predominant astatine species in basic aqueous media. This assumption is questioned in non‐complexing and non‐reductive aqueous solutions by means of high‐pressure anion‐exchange chromatography. Contrary to what is usually believed, astatide is found to be a minor species at pH=11. A different species, which also bears a single negative charge, becomes predominant when the pH is increased beyond 7. Using competition experiments, an equilibrium constant value of 10?6.9 has been determined for the formation of this species from AtO(OH) with the exchange of one proton. The identification of this species, AtO(OH)2?, is achieved through relativistic quantum mechanical calculations, which rule out the significant formation of the AtO2? species, while leading to a hydrolysis constant of AtO(OH) in excellent agreement with experiment when the AtO(OH)2? species is considered. Beyond the completion of the Pourbaix diagram of astatine, this new information is of interest for the development of 211At radiolabeling protocols. 相似文献
22.
Considering a two-level atom interacting with the competing two-mode field, this paper investigates the entanglement between the two-level atom and the two-mode field by using the quantum reduced entropy, and that between the two-mode field by using the quantum relative entropy of entanglement. It shows that the two kinds of entanglement are dependent on the relative coupling strength of atom-field and the atomic distribution, and exhibit the periodical evolution. The maximal atom-field entanglement state can be prepared via the appropriate selection of system parameters and interaction time. 相似文献
23.
提出一种采用Kohonen网络算法进行12电极电容CT系统的图像重建的方法.该网络由输入和输出两层神经元组成,输入为12电极电容CT系统测量所得的66个电容值,输出对应管道介质的空间分布模式.该网络采用竞争算法无监督学习,实验结果证明,该网络有较强的抗噪声能力,可重建出较精确的介质分布图像 相似文献
24.
掺杂KNSBN晶体中的电子—空穴竞争 总被引:1,自引:1,他引:0
通过测量掺杂KNSBN晶体光折变光栅记录和擦除动态特性,首次分析了掺杂KNSBN晶体中的电子-空穴竞争,根据耦合波理论,指出,响应时间越快的晶体,电子-空穴竞争越激烈,因而导致净调制折射率越小,衍射效率赵低,最后,分析了空穴产生的原因,并估算有效载流子浓度为10^15/cm^3量级。 相似文献
25.
By means of Mawhin's continuation theorem of coincidence degree and Lyapunov functional, a set of easily verifiable criteria are established for the existence and global attractivity of positive periodic solutions for delay Lotka-Volterra competition patch system with stocking
26.
For nonautonomous dynamical systems, the principle of inheriting local properties by global Poincaré maps is developed. Using this method, a selection criterion for systems of close competitors is found: to gain competitive advantage, it suffices to outproduce other populations with a margin. The margin factor in question remains uniformly bounded as the number of competitors in the community grows. 相似文献
27.
具有功能反应的两斑块扩散时滞竞争系统正周期解的存在性 总被引:6,自引:0,他引:6
§ 1 IntroductionFormanyspeciesthespatialfactorsareimportantinpopulationdynamics .Thetheoreticalstudyofspatialdistributionhasbeenextensivelystudiedinmanypapers .Mostofthepreviouspapersfocusedonthecoexistenceofpopulationsmodelledbyststemsofordinarydiffere… 相似文献
28.
Hongbin Zhang 《International Journal of Infrared and Millimeter Waves》2007,28(9):713-723
A spatially independent model of vertical-cavity surface-emitting lasers (VCSELs) is derived by integrating the spatially
dependent rate equations over the cross section of the cavity of a VCSEL. The angular and radial non-uniformities of the injection
current are taken into account. The well-known LP modes of a weakly-guiding cylindrical waveguide are employed to describe
the transverse modal structure in the VCSEL cavity. This model is solved in a self-consistent way by using the 4th order Runge-Kutta
method. The dependence of transverse mode competition on the current intensity, the angular and radial non-uniformities of
the injection current, and the geometrical parameters of the electrical contact are thoroughly investigated and analyzed.
The results are useful to the optimum design of the optical transverse modal structure of VCSELs. 相似文献
29.
We have investigated the evolution of the atomic quantum entropy and the entanglement of atom-photon in the system with competing k-photon and l-photon transitions by means of fully quantum theory, and examined the effects of competing photon numbers (k and l), the relative coupling strength between the atom and the two-mode field (A/g), and the initial photon number of the field on the atomic quantum entropy and the entanglement of atom-photon. The results show that the multiphoton competing transitions or the large relative coupling strength can lead to the strong entanglement between atoms and photons. The maximal atom-photon entanglement can be prepared via the appropriate selection of system parameters and interaction time. 相似文献
30.
Houqin Su Xuncheng Huang Xuncheng Huang Xiaoning Xu 《Journal of mathematical chemistry》2008,43(3):1273-1284
A three-dimensional bio-reactor model of exploitative competition of two predator organisms with inhibition responses for
the same renewable organism with reproductive properties is considered. By constructing a modified Lyapunov function and using
LaSalle’s invariant principle, it is shown that the lower “break-even” concentration predator organism survives in the competition.
相似文献