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Shrivats Semwal Dr. Joyanta Choudhury 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2017,129(20):5648-5652
Disclosed here is a molecular switch which responds to acid-base stimuli and serves as a bi-state catalyst for two different reactions. The two states of the switch serve as a highly active and poorly active catalyst for two catalytic reactions (namely a hydrogenation and a dehydrogenative coupling) but in a complementary manner. The system was used in an assisted tandem catalysis set-up involving dehydrogenative coupling of an amine and then hydrogenation of the resulting imine product by switching between the respective states of the catalyst. 相似文献
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