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991.
Carolina Toloza Porras Dagmar R. D'hooge Marie‐Franoise Reyniers Guy B. Marin 《Macromolecular theory and simulations》2013,22(2):136-149
The potential of initiators for continuous activator regeneration atom transfer radical polymerization (ICAR ATRP) for the synthesis of well‐defined poly(n‐butyl acrylate) is analyzed by means of simulations. The kinetic model accounts for reactivity differences between secondary and tertiary macrospecies and considers the possible influence of diffusional limitations. CuBr2 is used as transition metal salt and the commercially available N,N,N′,N″,N″‐pentamethyldiethylenetriamine as ligand. For targeted chain lengths (TCLs) up to 1000, the ICAR ATRP can be performed relatively quickly, and with ppm levels of ATRP catalyst. For moderate TCLs, slightly higher ppm levels are required if excellent control over chain length is also desired. In all cases, limited loss of end‐group functionality (EGF) results.
992.
In this paper, explicitly considering the influences of an epidemic outbreak on human travel, a time-varying human mobility pattern is introduced to model the time variation of global human travel. The impacts of the pattern on epidemic dynamics in heterogeneous metapopulation networks, wherein each node represents a subpopulation with any number of individuals, are investigated by using a mean-field approach. The results show that the pattern does not alter the epidemic threshold, but can slightly lower the final average density of infected individuals as a whole. More importantly, we also find that the pattern produces different impacts on nodes with different degree, and that there exists a critical degree kc. For nodes with degree smaller than kc, the pattern produces a positive impact on epidemic mitigation; conversely, for nodes with degree larger than kc, the pattern produces a negative impact on epidemic mitigation. 相似文献
993.
White matter maturation in the brains of Long Evans shaker myelin mutant rats by ex-vivo QSI and DTI
The brains of Long Evans shaker (les) rats, a model of dysmyelination, and their age- matched controls were studied by ex-vivo q-space diffusion imaging (QSI) and diffusion tensor imaging (DTI). The QSI and DTI indices were computed from the same acquisition. The les and the control brains were studied at different stages of maturation and disease progression. The mean displacement, the probability for zero displacement and kurtosis were computed from QSI data while the fractional anisotropy (FA) and the eigenvalues were computed from DTI. It was found that all QSI indices detect the les pathology, at all stages of maturation, while only some of the DTI indices could detect the les pathology. The QSI mean displacement was larger in the les group as compared with their age-matched controls while the probability for zero displacement and the kurtosis were both lower all indicating higher degree of restriction in the control brains. Since all the DTI eigenvalues were higher in the les brains as compared to controls, the less efficient DTI measure for discerning the les pathology was found to be the FA. Clearly, the most sensitive DTI parameter to the les pathology is λ3, i.e. the minimal diffusivity. Since the QSI and DTI data were obtained from the same acquisition, despite the somewhat higher SNR of the QSI data compared to the DTI data, it seems that the higher diagnostic capacity of the QSI data in this experimental model of dysmyelination, originates mainly from the higher diffusing weighting of the QSI data. 相似文献
994.
Diffusion-weighted MRI images acquired at b-value greater than 1000 s mm− 2 measure the diffusion of a restricted pool of water molecules. High b-value images are accompanied by a reduction in signal-to-noise ratio (SNR) due to the application of large diffusion gradients. By fitting the diffusion tensor model to data acquired at incremental b-value intervals, we determined the effect of SNR on tensor parameters in normal human brains, in vivo. In addition, we also investigated the impact of field strength on the diffusion tensor model. Data were acquired at 1.5 and 3 T, at b-values 0, 1000, 2000 and 3000 s mm− 2 in twenty diffusion-sensitised directions. Fractional anisotropy (FA), mean diffusivity (MD) and principal eigenvector coherence (κ) were calculated from diffusion tensors fitted between datasets with b-values 0–1000, 0–2000, 0–3000, 1000–2000 and 2000–3000 s mm− 2. Field strength and b-value effects on diffusion parameters were analysed in white and grey matter regions of interest. Decreases in FA, κ and MD were found with increasing b-value in white matter. Univariate analysis showed a significant increase in FA with increasing field strength in highly organised white matter. These results suggest there are significant differences in diffusion parameters at 1.5 and 3 T and that the optimal results, in terms of the highest values of FA in white matter, are obtained at 3 T with a maximum b = 1000 s mm− 2. 相似文献
995.
Abrupt changes in the near-band-edge luminescence of n-type undoped GaAs after implantation with 400 keV Zn ions and vacuum annealing at 580°C are reported. The good agreement of the spectral position, half-width and temperature dependence of the emission obtained after implantation and annealing with that of melt-doped GaAs: Zn indicates that implanted Zn ions have been incorporated at Ga lattice sites. The larger number of Zn substitutions obtained when bombardment is made on the Ga face than for an equivalent fluence on the As face demonstrates the existence of a polar implant effect. 相似文献
996.
This article deals with the critical curve of a fast diffusive polytropic filtration system coupled at the boundary condition. By constructing the self-similar supersolution and subsolution, we obtain the critical global existence curve. The critical curve of Fujita type is conjectured with the aid of some new results. 相似文献
997.
998.
Xuechen Wang 《Applicable analysis》2013,92(4):752-775
A diffusive predator–prey system with Ivlev-type functional response subject to Neumann boundary conditions is considered. Hopf and steady-state bifurcation analysis are carried out in detail. First, the stability of the positive equilibrium and the existence of spatially homogeneous and inhomogeneous periodic solutions are investigated by analysing the distribution of the eigenvalues. The direction and stability of Hopf bifurcation are determined by the normal form theory and the centre manifold reduction for partial functional differential equations and then steady-state bifurcation is studied. Finally, some numerical simulations are carried out for illustrating the theoretical results. 相似文献
999.
1000.
E. Patricio 《Applicable analysis》2013,92(1-4):113-126
A class of method with a free parameter(s) is considered for the solution of the diffusion–convection equation. This class is obtained using interpolation function approach and so, some classic methods appears when s take specific values. In order to obtain a non–oscillatory numerical solution some restrictions will be placed on s. Choosing two suitable methods of that class, an algorithm will be established and computational requirements will be considered 相似文献