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991.
992.
993.
A cobalt porphyrin equipped with two different but geometrically complementary pyridine ligands self-assembles to form an unusually stable complex with approximately 12 porphyrin monomers arranged in a macrocyclic array. 相似文献
994.
James B. Gerken Claire Badger Christopher Bisbee Sasha Gardner Yan Qi Víctor Durà Vilà John D. Roberts 《Journal of Physical Organic Chemistry》2008,21(3):193-197
Conformational preferences of glutaric, 3‐hydroxyglutaric and 3‐methylglutaric acid, and their mono‐ and dianions have been investigated with the aid of NMR spectroscopy. In contrast to succinic acid, glutaric acid displays essentially statistical conformational equilibria in polar and non‐polar solutions of high and low hydrogen‐bonding ability with no clear evidence for intramolecular hydrogen‐bonding interactions. The acid ionization constant ratios, K 1/K2, in D2O and DMSO of glutaric, 3‐hydroxyglutaric, and 3‐methylglutaric acids also indicate that intramolecular interactions are much less important than, or indeed insignificant, for shorter‐chain acids. FTIR studies on 3‐methylglutaric acid indicate some preference for either association with solvent or dimerization, depending on the solvent, rather than intramolecular hydrogen bonding. Copyright © 2008 John Wiley & Sons, Ltd. 相似文献
995.
The relationship between cosmological solutionsof five-dimensional Space-Time-Matter (STM) theory anda Generalized Scalar-Tensor (GST) theory is investigatedin which the cosmological term Lambda depends not only on a scalar field but also onits time derivative
.Identification of these solutions allows us to solve forthe functional form of the cosmological term, and mayhave relevance for the early Universe. 相似文献
996.
The question of the cause of inertial reaction forces and the validity of Mach's principle are investigated. A recent claim that the cause of inertial reaction forces can be attributed to an interaction of the electrical charge of elementary particles with the hypothetical quantum mechanical zero-point fluctuation electromagnetic field is shown to be untenable. It fails to correspond to reality because the coupling of electric charge to the electromagnetic field cannot be made to mimic plausibly the universal coupling of gravity and inertia to the stress-energy-momentum (i.e., matter) tensor. The gravitational explanation of the origin of inertial forces is then briefly laid out, and various important features of it explored in the last half-century are addressed. 相似文献
997.
998.
Sam V. Nablo James C. Wood Jr. Marc F. Desrosiers Vitaly Yu. Nagy 《Radiation Physics and Chemistry》1998,52(1-6):479-485
A small capacity (100 g.s−1) pilot system is described for presentation of powders and fine aggregates at high velocity, to an electron beam. Electron beam dose rate is continuously monitored in real time, while the thickness of the fluidized bed used to pneumatically transport the product can be monitored and controlled using beta-gauge techniques. Using electron paramagnetic resonance (EPR) techniques, alanine power mixed with the product is used for precise determination of dose delivered to the powder stream. Thin film dosimeters transported in the bed are also used for dose determination. Results with a variety of products are presented using both dose rate and velocity as the independent variables. Lethality data for the bioburdens present in several powdered foodstuffs are discussed. 相似文献
999.
This paper deals with the problem “Can a noisy orbit be tracked by a real orbit?” In particular, we will study the one-parameter family of tent maps and the one-parameter family of quadratic maps. We writeg μ for eitherf μ orF μ withf μ (x)=μx forx≦1/2 andf μ (x)=μ(1?x) forx≧1/2, andF μ (x)=μx(1?x). For a given μ we will say:g μ permits increased parameter shadowing if for each δ x >0 there exists someδ μ >0 and some δ f >0 such that every δ f -pseudog μ -orbit starting in some invariant interval can be δ x -shadowed by a realg α -orbit with α=μ+δ μ . We show thatg μ typically permits increased parameter shadowing. 相似文献
1000.
Asynchronous Transfer Mode (ATM) has been adopted by the CCITT as the transport mode in which Broadband ISDN will be based. In this paper, we formulate the problem of routing cells in an ATM network as an optimization problem. The objective is to minimize the largest cell loss probability among all links. The constraints correspond to a multicommodity network flow problem with gains. An algorithm to determine a global optimal flow assignment is presented. The minimax routing algorithm was implemented and tested on several sample networks. The computational experiments show that the algorithm is computationally efficient.Supported by NSF grant NCR 92-23148. 相似文献