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71.
Kausar A Nagano H Kuwahara Y Ogata T Kurihara S 《Chemistry (Weinheim an der Bergstrasse, Germany)》2011,17(2):508-515
In this paper the photocontrolled manipulation of solid materials on the surface of a liquid crystalline thin film is described. Three different types of films namely cholesteric liquid crystal (ChLC), compensated nematic liquid crystal (NLC) and nematic LC were used. The rotational and translational manipulation of the microscale solid object was induced by irradiation of light and mode of manipulation (either translational or rotational) was changed by changing the isomer of the azobenzene compound used to make the film. Rotational motion of the object was observed on the ChLC and compensated NLC films containing chirally pure azobenzene compound. The direction of rotational motion was controlled either by changing the optical isomer of the chiral azobenzene or by changing the irradiating light (from ultraviolet to visible). When racemic mixture of the chiral azobenzene compound was used, a translational motion of the object was observed. Even though the direction of the translational motion can be controlled by controlling irradiation position, more facile and precise manipulation of the objects was possible by spatially controlled irradiation of Ar(+) laser and diode UV laser. 相似文献
72.
Koichi Kan Jinfeng Yang Kimihiro Norizawa Takafumi Kondoh Yoichi Yoshida Atsushi Ogata 《Radiation Physics and Chemistry》2011,80(12):1323-1326
A novel method to generate high-power THz radiation is proposed. If a beam with a bunch length on the order of 100 fs is injected into an electron–hole plasma of a semiconductor with a plasma frequency on the order of THz, THz wake fields are coherently generated. If the beam moves on the axis of a hollow tube covered by a metal, the frequency spectrum of the radiation is composed of discrete components. Monochromatic radiation is obtained by making only the lowest frequency component coherent. 相似文献
73.
74.
Total synthesis of the proposed structure 2 for phomopsin B was achieved by using an intramolecular olefin metathesis as a key step. The spectral data, however, did not match with those of the natural product reported. Re-examination of the reported NMR data led to the structural revision of phomopsin B to known dothiorelone A 18. The R configuration of dothiorelone A was determined by total synthesis through a cross-metathesis with a chiral olefin 19. 相似文献
75.
76.
We consider a model describing finitely many free Fermi gas reservoirs coupled by local interactions and prove the Green–Kubo
formulas and the Onsager reciprocity relations for heat and charge fluxes generated by temperature and chemical potential
differentials.
Submitted: September 2, 2006. Accepted: November 21, 2006. 相似文献
77.
We study linear response theory in the general framework of algebraic quantum statistical mechanics and prove the Green-Kubo formula and the Onsager reciprocity relations for heat fluxes generated by temperature differentials. Our derivation is axiomatic and the key assumptions concern ergodic properties of non-equilibrium steady states. 相似文献
78.
Ogata A. Nakajima K. Kozawa T. Yoshida Y. 《IEEE transactions on plasma science. IEEE Nuclear and Plasma Sciences Society》1996,24(2):453-459
A conceptual design of a linac for pulse radiolysis is presented based on laser wakefield acceleration. Pulse radiolysis spectroscopically studies the initial stage of chemical reactions induced by electron beams. Single-bunched beams with a bunch-length on the order of a femtosecond are ideal for this purpose. The present design gives pure 20 pC single-bunches with an RMS bunch length of less than 10 fs. It accelerates and compresses only the head part of a high-current beam from a photocathode. Some practical problems concerning the design are also presented 相似文献
79.
80.