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Keiki Kishikawa Yuki Furukawa Tomohiro Watanabe Michinari Kohri Tatsuo Taniguchi Shigeo Kohmoto 《Liquid crystals》2017,44(6):956-968
Novel C2-symmetric chiral dopant derivatives, namely, N-substituted (2R, 3R)-2,3-bis(4-(4-octyloxyphenyl)benzoyloxy)succinimides1a-h, were synthesised, and the effects of the N-substituent and imide-carbonyl groups on the helical twisting powers (HTPs) were investigated in two nematic liquid crystalline compounds, 4-n-pentyl-4?-cyanobiphenyl (5CB) and N-(4-ethoxybenzylidene)-4-n-butylaniline (EBBA). As a result, it was clarified that the bulkiness of the N-substituents has a significant correlation with the HTPs, and the imide-carbonyl group interacts strongly with the cyano group of 5CB to give high HTPs in the nematic phases. However, it is assumed that the imide-carbonyl groups of the dopants do not have strong electrostatic attractive interactions with EBBA molecules in the nematic phase to afford the moderate HTPs. 相似文献
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Michinari Kohri Madoka Sato Fumina Abo Takumi Inada Masakatsu Kasuya Tatsuo Taniguchi Takayuki Nakahira 《European Polymer Journal》2011,47(12):2351-2360
Polystyrene particles bearing ATRP initiating groups, obtained by emulsifier-free emulsion polymerization of styrene (St) and 2-chloropropyloxyethyl methacrylate (CPEM), were subjected to surface-initiated activator generated by electron transfer for atom transfer radical polymerization (AGET ATRP) using glycomonomers, i.e., 4-vinylbenzenesulfonamidoethyl 1-thio-β-d-glucopyranoside (1) and 4-vinylbenzenesulfonamidoethyl 1-thio-β-d-lactoside (2). The glycopolymer-grafted polystyrene particles obtained Gp1 and Gp2 were shown to have hydrated graft layers of 15–65 nm in thickness on the cores of 370 nm in diameter. Gp1 and Gp2 coagulated in the presence of concanavalin A (Con A) and that of peanut agglutinin (PNA), respectively, showing highly specific response toward lectins. 相似文献
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Tatsuo Taniguchi Fumiyasu Murakami Masakatsu Kasuya Takashi Kojima Michinari Kohri Kyoichi Saito Takayuki Nakahira 《Colloid and polymer science》2013,291(1):215-222
Organic/inorganic hybrids were prepared by catalytic hydrolysis and subsequent polycondensation of tetra-n-butyl titanate (TnBT) in shell layers grafted on core particles. The core particles were synthesized by emulsifier-free emulsion polymerization of styrene, N-n-butyl-N-2-methacryloyloxyethyl-N,N-dimethylammonium bromide (C4DMAEMA), and 2-chloropropionyloxyethyl methacrylate using 2,2′-azobis(2-amidinopropane) dihydrochloride as an initiator. The core diameters were controlled in the range of 70–550 nm by adjusting a C4DMAEMA feed concentration. The core–shell particles were prepared by surface-initiated activator generated electron transfer–atom transfer radical polymerization of 2-(N,N-dimethylamino)ethyl methacrylate (DMAEMA). The sizes of core–shell particles were found to increase monotonically with an increase in a DMAEMA concentration. The hybrid particles were fabricated by adding TnBT into a water/ethanol dispersion of core–shell particles. The amounts of titania deposited increased in proportion to the grafted amounts of poly[2-(N,N-dimethylamino)ethyl methacrylate] on the core particles. The X-ray diffraction measurement revealed that the hollow titania particles obtained by heat treatment of hybrids have an anatase crystallographic phase. 相似文献
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Kohri H Ahn DS Ahn JK Akimune H Asano Y Chang WC Date' S Ejiri H Fukui S Fujimura H Fujiwara M Hasegawa S Hicks K Hotta T Imai K Ishikawa T Iwata T Kawai H Kim ZY Kino K Kumagai N Makino S Mart T Matsuda T Matsumura T Matsuoka N Mibe T Miyabe M Miyachi Y Morita M Muramatsu N Nakano T Niiyama M Nomachi M Ohashi Y Ohkuma H Ooba T Oshuev DS Rangacharyulu C Sakaguchi A Sasaki T Shagin PM Shiino Y Shimizu A Shimizu H Sugaya Y Sumihama M Toi Y Toyokawa H Wakai A Wang CW Wang SC Yonehara K Yorita T 《Physical review letters》2006,97(8):082003
Differential cross sections and photon-beam asymmetries have been measured for the gamma n --> K+ Sigma- and gamma p --> K+Sigma0 reactions separately using liquid deuterium and hydrogen targets with incident linearly polarized photon beams of E gamma = 1.5-2.4 GeV at 0.6 < cos ThetacmK< 1. The cross section ratio of sigma K+ Sigma-/sigma K+ Sigma0, expected to be 2 on the basis of the isospin 1/2 exchange, is found to be close to 1. For the K+ Sigma- reaction, large positive asymmetries are observed, indicating the dominance of K* exchange. The large difference between the asymmetries for the K+ Sigma- and K+ Sigma0 reactions cannot be explained by simple theoretical considerations based on Regge model calculations. 相似文献
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Mibe T Chang WC Nakano T Ahn DS Ahn JK Akimune H Asano Y Daté S Ejiri H Fujimura H Fujiwara M Hicks K Hotta T Imai K Ishikawa T Iwata T Kawai H Kim ZY Kino K Kohri H Kumagai N Makino S Matsuda T Matsumura T Matsuoka N Miwa K Miyabe M Miyachi Y Morita M Muramatsu N Niiyama M Nomachi M Ohashi Y Ooba T Ohkuma H Oshuev DS Rangacharyulu C Sakaguchi A Sasaki T Shagin PM Shiino Y Shimizu H Sugaya Y Sumihama M Titov AI Toi Y Toyokawa H Wakai A Wang CW Wang SC Yonehara K Yorita T Yoshimura M Yosoi M 《Physical review letters》2005,95(18):182001
Photoproduction of a phi meson on protons was studied by means of linearly polarized photons at forward angles in the low-energy region from threshold to Egamma = 2.37 GeV. The differential cross sections at t = -|t|min do not increase smoothly as Egamma increases but show a local maximum at around 2.0 GeV. The angular distributions demonstrate that phi mesons are photoproduced predominantly by helicity-conserving processes, and the local maximum is not likely due to unnatural-parity processes. 相似文献
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The solid dispersion of mebendazole was prepared with polyethylene glycol (PEG) to enhance the dissolution rate of mebendazole, an agent for the chemotherapy of human echinococcosis. The dissolution rate of the solid dispersion increased compared with the physical mixture, and also increased with the incorporation of an increasing amount of PEG-6000. An extensive improvement of the dissolution rate was observed when the ratio of the solid dispersion of mebendazole to PEG-6000 was more than 1: 2. Furthermore, greater bioavailability in rabbits was obtained after oral administration of the solid dispersion compared with the physical mixture. 相似文献
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Nakayama S Yamagata T Akimune H Daito I Fujimura H Fujita Y Fujiwara M Fushimi K Inomata T Kohri H Koori N Takahisa K Tamii A Tanaka M Toyokawa H 《Physical review letters》2000,84(2):262-265
We consider a billiard model of a self-bound, interacting three-body system in two spatial dimensions. Numerical studies show that the classical dynamics is chaotic. The corresponding quantum system displays spectral fluctuations that exhibit small deviations from random matrix theory predictions. These can be understood in terms of a new type of scarring caused by a one-parameter family of orbits inside the collinear manifold. 相似文献