Band mixing in156Gd and158Gd

A detailed investigation of the energies and intensities of the γ-rays that depopulate the low spin levels of the β- and γ-vibrational bands of¹⁵⁶Gd and the γ-vibrational band of¹⁵⁸Gd has been conducted. Both singles and γ-γ coincidence measurements were made on sources of 15-d¹⁵⁶Eu and 46-min¹⁵⁸Eu by use of large volume, high resolution Ge(Li) detectors. In addition to the γ-band at 1154.09 keV, twoK ^π=0⁺ bands were observed in¹⁵⁶Gd with band heads at 1049.45 and 1168.11 keV, respectively. The 2⁺ and 3⁺ members of the γ-vibrational band in¹⁵⁸Gd were observed at 1187.12 and 1265.43 keV, respectively, as well as a newK ^π=0⁺ band at 1195.98 keV. A first order perturbational treatment of the branching ratios was applied to both nuclei. In addition, the mixing between the ground state, the β-, and the γ-vibrational bands of¹⁵⁶Gd is considered from two approaches, but neither satisfactorily explains all the experimentalB(E2) ratios.     

Search for weak transitions in the decay of125Sb and accurate gamma intensities

The weak transitions in the decay of¹²⁵Sb have been investigated through gamma ray measurements with high resolution X-ray and with large volume Ge(Li) detectors. The 172.6, 178.8 and 198.5 keV gamma rays are confirmed, while others previously reported were not. Accurate intensities were obtained for the stronger transitions. The weighted averages of these intensities which cover the range of 116 to 670 keV are useful for calibration of Ge(Li) systems.     

Maximizing the Hilbert space for a finite number of distinguishable quantum states

Given a particular quantum computing architecture, how might one optimize its resources to maximize its computing power? We consider quantum computers with a number of distinguishable quantum states, and entangled particles shared between those states. Hilbert-space dimensionality is linked to nonclassicality and, hence, quantum computing power. We find that qutrit-based quantum computers optimize the Hilbert-space dimensionality and so are expected to be more powerful than other qudit implementations. In going beyond qudits, we identify structures with much higher Hilbert-space dimensionalities.     

Lead tetrakis(imidazolyl)borate solids: anion exchange, solvent intercalation, and self assembly of an organic anion

The coordination polymer Pb[B(Im)(4)](NO(3))(xH(2)O), constructed by using sodium tetrakis(imidazolyl)borate and lead(II) nitrate solutions, is a layered material with the metal centers facing the interlayer spacing. As in naturally occurring layered minerals, this compound can readily undergo anion exchange and reversible intercalation of solvent water in the solid state with retention of crystallinity. We observed changes in solvent intercalation by (207)Pb solid state NMR (SSNMR) and thermogravimetric analysis (TGA). Stoichiometric exchange of (15)N nitrate for nitrate and iodide for nitrate is monitored by (15)N and (207)Pb SSNMR, and single crystals of the iodide-exchanged material Pb[B(Im)(4)]I were isolated. While the iodide compound can be obtained through facile exchange from the nitrate parent compound, the organic anion benzoate is placed in the interlayer spacing for nitrate under self-assembly conditions and forms an alternating monolayer in Pb[B(Im)(4)](C(6)H(5)COO)(0.5H(2)O). The ion exchange versus self-assembly behavior correlates with the structural differences in the three compounds. In both Pb[B(Im)(4)]I and Pb[B(Im)(4)](C(6)H(5)COO)(0.5H(2)O), the lead sites act as Lewis acids for the iodide and benzoate, respectively.     

Low molecular weight organogelators for water

Mono-urea serine derivatives with low molecular weights were prepared in one step and show remarkable self-assembling and gelation properties in water.     

The Application of Nonlinear Dynamics in Nursing Research

In this article, the authors present an overview of the applications of chaos theory and nonlinear dynamics to problems of relevance not only to nurses, but to anyone dealing with human functioning and interaction. These applications have been in the areas of epidemiology, nursing management and physiological functioning. In some cases, the applications were successful in identifying information that would have been overlooked using traditional methods. In other cases, the problems of data collection and analysis, unique to nonlinear dynamics, are still being developed and tested.     

A Si(Li) detector system for conversion coefficient measurements and application to the decays of51Cr and87Y

An electron detector system with a 3 mm × 100 mm² Si(Li) detector with a cooled FET and vacuum air lock for changing sources was constructed. The absolute efficiency was measured as a function of energy for use in the measurement ofK conversion coefficients. With the Si(Li) and a Ge(Li) detector, theK conversion coefficient of the 320 keV transition in⁵¹V was measured to be 0.00156 ± 0.00008 where theK conversion coefficients of the 661 and 279 keV transitions in¹³⁷Ba and²⁰³Tl were used as standards. From absolute detection efficiency measurements, theK conversion coefficients of the 388 and 483 keV transitions in⁸⁷Sr were measured to be 0.16 ± 0.02 and 0.0024 ± 0.0003, respectively.