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41.
We consider the Cauchy problem for one-dimensional isentropic compressible Navier-Stokes equations with density-dependent viscosity coefficient.For regular initial data,we show that the unique strong s... 相似文献
42.
Toward two-dimensional nanometer resolution hard X-ray differential-interference-contrast imaging using modified photon sieves 总被引:2,自引:0,他引:2
In this Letter, we report a significant step forward in the design of single-optical-element optics for two-dimensional (2D) hard X-ray differential-interference-contrast (DIC) imaging based on modified photon sieves (MPSs). MPSs were obtained by a modified optic, i.e., combining two overlaid binary gratings and a photon sieve through two logical XOR operations. The superior performance of MPSs was demonstrated. Compared to Fresnel zone plates-based DIC diffractive optical elements (DOEs), which help to improve contrast only in one direction, MPSs can provide better resolution and 2D DIC imaging. Compared to normal photon sieves, MPSs are capable of imaging at a significantly higher image contrast. We anticipate that MPSs can provide a complementary and versatile high-resolution nondestructive imaging tool for ultra-large-scale integrated circuits at 45 nm node and below. 相似文献
43.
44.
The augmented cube AQ
n
is a variation of the hypercube Q
n
. This paper considers the panconnectivity of AQ
n
(n ⩾ 3) with at most 2n−5 faulty vertices and/or edges and shows that, for any two fault-free vertices u and v with distance d in AQ
n
, there exist fault-free uv-paths of every length from d + 2 to 2
n
− f − 1, where f is the number of faulty vertices in AQ
n
. The proof is based on an inductive construction. 相似文献
45.
The one-dimensional transient quantum Euler-Poisson system for semiconductors is studied in a bounded interval. The quantum correction can be interpreted as a dispersive regularization of the classical hydrodynamic equations and mechanical effects. The existence and uniqueness of local-in-time solutions are proved with lower regularity and without the restriction on the smallness of velocity, where the pressure-density is general (can be non-convex or non-monotone). 相似文献
46.
Temperature-induced chiral nematic phase changes of suspensions of poly(N,N-dimethylaminoethyl methacrylate)-grafted cellulose nanocrystals 总被引:1,自引:0,他引:1
Temperature-induced copolymers of poly(N,N-dimethylaminoethyl methacrylate)-grafted cellulose nanocrystals (PDMAEMA-grafted CNC) were synthesized by surface-initiated
atom transfer radical polymerization (ATRP). The graft copolymers were characterized by thermogravimetric analysis (TGA),
Fourier-transform infrared spectroscopy (FT-IR), and gel permeation chromatography (GPC). The size of the original CNC was
10–40 nm in width and 100–400 nm in length, as characterized by atomic force microscopy (AFM). The liquid-crystalline properties
of the graft copolymers were investigated by using polarizing optical microscopy (POM). The graft copolymers exhibited fingerprint
texture in lyotropic state. The temperature-induced fingerprint texture changes of PDMAEMA-grafted CNC aqueous suspensions
were investigated at various temperatures. With increasing temperature, the spacing of the fingerprint lines decreases. Temperature-induced
changes of PDMAEMA polymer chains result in changes of fingerprint texture. 相似文献
47.
Yiren Zhong Yujun Xie Sooyeon Hwang Qian Wang Judy J. Cha Dong Su Hailiang Wang 《Angewandte Chemie (International ed. in English)》2020,59(33):14003-14008
The energetic chemical reaction between Zn(NO3)2 and Li is used to create a solid‐state interface between Li metal and Li6.4La3Zr1.4Ta0.6O12 (LLZTO) electrolyte. This interlayer, composed of Zn, ZnLix alloy, Li3N, Li2O, and other species, possesses strong affinities with both Li metal and LLZTO and affords highly efficient conductive pathways for Li+ transport through the interface. The unique structure and properties of the interlayer lead to Li metal anodes with longer cycle life, higher efficiency, and better safety compared to the current best Li metal electrodes operating in liquid electrolytes while retaining comparable capacity, rate, and overpotential. All‐solid‐state Li||Li cells can operate at very demanding current–capacity conditions of 4 mA cm?2–8 mAh cm?2. Thousands of hours of continuous cycling are achieved at Coulombic efficiency >99.5 % without dendrite formation or side reactions with the electrolyte. 相似文献
48.
Qiuwei Shi Yiren Zhong Min Wu Prof. Hongzhi Wang Prof. Hailiang Wang 《Angewandte Chemie (International ed. in English)》2018,57(29):9069-9072
Developing Na metal anodes that can be deeply cycled with high efficiency for a long time is a prerequisite for rechargeable Na metal batteries to be practically useful despite their notable advantages in theoretical energy density and potential low cost. Their high chemical reactivity with the electrolyte and tendency for dendrite formation are two major issues limiting the reversibility of Na metal electrodes. In this work, we introduce for the first time potassium bis(trifluoromethylsulfonyl)imide (KTFSI) as a bifunctional electrolyte additive to stabilize Na metal electrodes, in which the TFSI? anions decompose into lithium nitride and oxynitrides to render a desirable solid electrolyte interphase layer while the K+ cations preferentially adsorb onto Na protrusions and provide electrostatic shielding to suppress dendritic deposition. Through the cooperation of the cations and anions, we have realized Na metal electrodes that can be deeply cycled at a capacity of 10 mAh cm?2 for hundreds of hours. 相似文献
49.
Introducing Fe2+ into Nickel–Iron Layered Double Hydroxide: Local Structure Modulated Water Oxidation Activity 下载免费PDF全文
Zhao Cai Daojin Zhou Maoyu Wang Seong‐Min Bak Yueshen Wu Zishan Wu Yang Tian Xuya Xiong Dr. Yaping Li Dr. Wen Liu Prof. Samira Siahrostami Dr. Yun Kuang Prof. Xiao‐Qing Yang Dr. Haohong Duan Prof. Zhenxing Feng Prof. Hailiang Wang Prof. Xiaoming Sun 《Angewandte Chemie (International ed. in English)》2018,57(30):9392-9396
Exploring materials with regulated local structures and understanding how the atomic motifs govern the reactivity and durability of catalysts are a critical challenge for designing advanced catalysts. Herein we report the tuning of the local atomic structure of nickel–iron layered double hydroxides (NiFe‐LDHs) by partially substituting Ni2+ with Fe2+ to introduce Fe‐O‐Fe moieties. These Fe2+‐containing NiFe‐LDHs exhibit enhanced oxygen evolution reaction (OER) activity with an ultralow overpotential of 195 mV at the current density of 10 mA cm?2, which is among the best OER catalytic performance to date. In‐situ X‐ray absorption, Raman, and electrochemical analysis jointly reveal that the Fe‐O‐Fe motifs could stabilize high‐valent metal sites at low overpotentials, thereby enhancing the OER activity. These results reveal the importance of tuning the local atomic structure for designing high efficiency electrocatalysts. 相似文献
50.