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41.
M. Yoshida K. Ishii K. Ikeuchi I. Jarrige Y. Murakami J. Mizuki K. Tsutsui T. Tohyama S. Maekawa K. Kudo Y. Koike Y. Endoh 《Physica C: Superconductivity and its Applications》2010
We report a resonant inelastic X-ray scattering (RIXS) study of charge excitations in the two-leg ladder Sr14Cu24O41. RIXS spectra at 1–5 eV are found to be dependent on temperature. An intraband excitation of the ladder, which appears as a continuum intensity below the Mott gap, decreases in intensity with temperature. Because the intraband excitation is related to the dynamics of doped holes in the ladder, its decrease of the intraband excitation is attributed to the reduction of the mobile holes in the ladder at low temperature. 相似文献
42.
43.
Sueishi Y Yoshioka D Yoshioka C Yamamoto S Kotake Y 《Organic & biomolecular chemistry》2006,4(5):896-901
Using a competitive spin trapping method, relative spin trapping rates were quantified for various short-lived radicals (methyl, ethyl, and phenyl radicals). High static pressure was applied to the competitive spin-trapping system by employing high-pressure electron spin resonance (ESR) equipment. Under high pressure (490 bar), spin trapping rate constants for alkyl and phenyl radicals increased by 10 to 40%, and the increase was dependent on the structure of nitrone spin traps. A maximum increase was obtained when tert-butyl(4-pyridinylmethylene)amine N-oxide (4-POBN) was used as a spin trap. Activation volumes (DeltaDeltaV(double dagger)) for the two spin trapping reactions were calculated to be -17-(-9) cm(3) mol(-1) for the 4-POBN system. 相似文献
44.
Takao Morinari Eiji Kaneshita Tohyama Tohyama 《Physica C: Superconductivity and its Applications》2010,470(2):95-97
We propose interlayer magnetoresistance experiments which provide information about Fermi surface topology in layered multi-band systems. The interlayer magnetoresistance shows an oscillating behavior with respect to the azimuthal angle of the applied in-plane magnetic field if the Fermi surface is anisotropic. We discuss applications to LaFeAsO, a parent compound of FeAs-based superconductors. We show the results on the paramagnetic state and the antiferromagnetic state based on a mean field calculation. 相似文献
45.
46.
Naoya Yoda Kojuro Ikeda Masaru Kurihara Shunroku Tohyama Ryoji Nakanishi 《Journal of polymer science. Part A, Polymer chemistry》1967,5(9):2359-2374
New high temperature aromatic polybenzoxazinones of high molecular weight have been prepared by the cyclopolycondensation of 4,4′-diaminobiphenyl-3,3′-dicarboxylic acid (I) with aromatic dicarboxylic acid halides (II). The low temperature solution polymerization techniques afforded poly(amic acid) (III) of high molecular weight in the first step. An open-chain precursor subsequently underwent thermal cyclodehydration along the polymer chain at 200–350°C. in the second step, to give in quantitative yield a fully aromatic polybenzoxazinone (IV) of outstanding heat stability both in nitrogen and in air. The poly(amic acid) is soluble in N-methyl-2-pyrrolidone, and tough, transparent films can be cast from solution. Insoluble aromatic polybenzoxazinone films which possess excellent oxidative and thermal stability were obtained by the heat treatment of the polyamic acid. A detailed account of polymerization conditions in the low temperature solution polymerization of polybenzoxazinones is given, and the reaction mechanisms of cyclopolycondensation of poly(amic acids) and the formation of polybenzoxazinones are discussed. 相似文献
47.
Hikaru Aramoto Motofumi Osaki Subaru Konishi Chiharu Ueda Yuichiro Kobayashi Yoshinori Takashima Akira Harada Hiroyasu Yamaguchi 《Chemical science》2020,11(17):4322
Stimuli-responsive hydrogels have attracted attention as soft actuators that act similarly to muscles. In this work, hydrogel actuators controlled by host–guest interactions have been developed. The introduction of a 1:1 inclusion complex into a hydrogel is a popular design for achieving a change in cross-linking density. To realize faster and larger deformation properties, the introduction of a 1:2 inclusion complex is effective because the alteration in cross-linking density in a hydrogel with 1:2 complexes is larger than that in a hydrogel with 1:1 complexes. A redox-responsive hydrogel actuator cross-linked with 1:2 inclusion complexes is designed, where γ-cyclodextrin (γCD) and viologens modified with an alkyl chain derivative (VC11) were employed as the host and guest units, respectively. γCD includes two VC11 molecules in its cavity. The obtained γCD–VC11 hydrogel cross-linked with the 1:2 complex showed faster and larger deformation behaviour than the αCD–VC11 and the βCD–VC11 hydrogels cross-linked with a 1:1 complex. The deformation ratio and response speed of the γCD–VC11 hydrogel, which forms a supramolecular cross-linking structure by stimuli, are 3 and 11 times larger, respectively, than those of our previous hydrogel consisting of a βCD/ferrocene 1:1 inclusion complex.A hydrogel actuator with a 1:2 host–guest complex controlled by redox stimuli has been developed to realize faster and larger deformation. 相似文献
48.
Tohyama M. Takahara S. Schuck P. 《The European Physical Journal A - Hadrons and Nuclei》2004,21(2):217-225
We propose a time-independent method for finding a correlated ground state of an extended time-dependent Hartree-Fock theory, known as the time-dependent density matrix theory (TDDM). The correlated ground state is used to formulate the small amplitude limit of TDDM (STDDM) which is a version of extended RPA theories with ground-state correlations. To demonstrate the feasibility of the method, we calculate the ground state of 22
O and study the first 2 + state and its two-phonon states using STDDM.Received: 7 November 2003, Published online: 10 August 2004PACS:
21.10.Re Collective levels - 21.60.Jz Hartree-Fock and random-phase approximations - 27.30. + t
相似文献
49.
Ishii K Tsutsui K Endoh Y Tohyama T Kuzushita K Inami T Ohwada K Maekawa S Masui T Tajima S Murakami Y Mizuki J 《Physical review letters》2005,94(18):187002
Mott gap excitations in the optimally doped high-T(c) superconductor YBa(2)Cu(3)O(7-delta) (T(c)=93 K) have been studied by the resonant inelastic x-ray scattering method. Anisotropic spectra in the ab plane are observed in a twin-free crystal. The excitation from the one-dimensional CuO chain is enhanced at 2 eV near the zone boundary of the b* direction, while the excitation from the CuO2 plane is broad at 1.5-4 eV and almost independent of the momentum transfer. Theoretical calculations based on the one-dimensional and two-dimensional Hubbard model reproduces the observed spectra when different values of the on-site Coulomb energy are assumed. The Mott gap of the CuO chain site is found to be much smaller than that of the CuO2 plane site. 相似文献
50.