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Direct catalytic oxidative conversion of light alkanes to alcohols using molecular oxygen as an oxidant is a challenging and important synthetical goal, which might be met by transition metal porphyrin complexes that are capable of forming active metal oxo intermediates via direct reaction with O2 in the presence of a co-reductant[1]. It was found that iron complexes of halogenated porphyrins were remarkably active catalysts for the hydroxylation of light alkanes by O2 without added co-reductants in an organic solvent such as benzene 相似文献
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