纳米流体液滴撞击壁面铺展动力学特性研究

纳米流体液滴撞击固体壁面的铺展动力学特性是基于液滴沉积实现高效传热传质过程的关键因素,然而由于纳米流体的非牛顿流变特性及液滴内微流动与纳米颗粒的耦合作用,目前对纳米流体液滴撞击固体壁面的铺展动力学行为缺乏足够的认识.本研究利用了两步法分别配制了分散有3种纳米颗粒的均匀稳定纳米流体(碳纳米管、石墨烯、纳米石墨粉),并对流体的流变特性进行了测量分析.利用显微高速数码摄像技术捕捉了液滴撞击固体壁面的动态过程,通过图像处理技术分析铺展过程中液滴的无量纲高度、铺展因子及动态接触角,探究了液滴在韦伯数约为200及800时撞击壁面后铺展沉积形态的演变规律.研究表明,3种不同纳米颗粒的加入均使基液表现出明显的剪切变稀特性,在液滴撞击壁面的铺展过程中,流体的剪切黏度起重要作用,液滴的无量纲高度和铺展因子的变化幅度随着纳米流体剪切黏度的增大而减小.纳米流体液滴撞击疏水表面时能更快的达到平衡状态,液滴的惯性力主导着液滴的初始铺展阶段,液滴的铺展范围和速度随撞击速度的增大而增大.开展该研究能够为基于液滴沉积的增益冷却技术以及微型高导热及导电材料的制造提供理论依据和技术指导.     

剪切变稀流体液滴撞击疏水表面回弹现象及最大铺展的研究

非牛顿流体液滴撞击固体表面的行为广泛存在于多种工农业生产中, 然而目前相关研究主要关注牛顿流体, 非牛顿流变特性对液滴撞击动力学的影响机制还有待探索. 本文研究了纯剪切变稀流体(质量分数≤ 0.03%的黄原胶水溶液)液滴撞击疏水表面后的最大铺展及回弹行为. 通过高速摄像技术捕获液滴撞击疏水表面的运动过程及形态变化, 研究了液滴的铺展回缩过程. 实验结果表明, 在相同We下, 剪切变稀特性对液滴撞击疏水表面后的铺展阶段影响很小, 但对回缩阶段影响很大. 黄原胶浓度增加使得液滴依次表现出部分回弹、完全回弹和表面沉积三种不同的回弹行为. 利用能量守恒定律推导出了液滴能在疏水表面上回弹的临界无量纲高度ξ_c理论值. 发现牛顿流体与非牛顿流体液滴最大无量纲高度ξ_max均符合标度律ξ_max ~ αWe斜率随黄原胶浓度增大而减小. 基于有效雷诺数Re_eff, 提出了一种有效黏度μ_eff表达式, 并据此建立了剪切变稀流体的最大无量纲直径β_max预测模型. 该模型在较广We区间与实验测量值取得了良好一致.      

强磁场影响下镓液滴撞击固壁的实验研究

在材料的电磁冶金过程及磁约束核聚变装置中, 金属液滴在磁场和壁面温度影响下的撞击过程表现出复杂的动力学特性. 本文对水平磁场作用下液态镓(Ga)液滴撞击等温和过冷壁面的铺展和回弹特性进行了实验研究. 采用高速相机拍摄液滴撞击过程中轮廓的变化, 通过图像处理获得不同磁场强度、不同撞击速度和不同底板温度下的最大铺展因子、回弹过程中的最大高度以及产生的二次液滴的半径和速度. 碰撞速度由0.45 ~ 1.8 m/s, 磁场强度从0 ~ 1.6 T, 底板温度为30 °C, ?20 °C和?10 °C. 基于实验结果分析了磁场和壁面温度对液滴铺展和回弹的影响规律. 实验结果表明, 液滴撞击等温壁面和过冷壁面的最大铺展因子随We的变化均与理论预测关系式一致. 液滴撞击等温壁面的情况下, 不同的We下, 出现不同的回弹现象. 磁场抑制了平行于磁场方向的液滴铺展和回弹过程中二次液滴的产生, 而对回弹过程中的液滴在平行磁场方向上有拉伸作用. 液滴撞击过冷壁面时, 在一定的We值范围内, 同样会出现二次液滴分离现象, 此时产生的二次液滴的速度较小. 磁场的增强和We的增大都会导致液滴在高度方向的振荡减弱, 加速凝固过程.      

不同壁面条件下液滴撞击铺展特性的模拟研究

液滴撞击不同润湿性壁面的传热流动问题在自然界和工业生产中广泛存在。研究采用CLSVOF方法,引入描述壁面润湿特性的动态接触角,并考虑液滴物性参数随温度的变化,建立液滴撞壁模型,模拟研究液滴撞击流动行为,通过与实验对比验证,确定模型有效性。在此基础上,对传热作用下考虑壁面润湿性的液滴撞击问题展开研究,探讨壁面传热作用对液滴撞击铺展特性的影响。研究表明,在撞击过程中,液滴先铺展后逐渐收缩,与静态接触角模型相比,采用动态接触角模型所得的液滴流动特性与实验结果更加吻合;随着接触角增大,液滴在撞壁初期不易铺展,随后则易于收缩;虽然固液传热作用会影响液滴铺展直径,但不改变液滴的运动趋势。     

非等温粗糙表面液滴撞击特性试验与仿真研究

非等温固体表面液滴碰撞现象广泛存在于航空航天领域机械零部件中，液滴碰撞动力学行为的研究对提升机械零部件传热换热以及润滑性能具有重要意义.为获得液滴在非等温粗糙表面的撞击特性，研究了硅油在金属表面撞击、铺展和回缩的动力学行为，并着重分析了硅油黏度、撞击速度、油滴初始直径、金属表面粗糙度及温度对硅油撞击特性的影响.结果表明，在等温表面，液滴最大铺展直径与撞击速度、基体表面温度及液滴初始直径正相关，与基体表面粗糙度、硅油黏度负相关；当表面粗糙度介于6.3～25μm时，其对液滴最大铺展直径影响较小；在非等温表面，液滴回缩过程中少量液体残留并形成尾迹，且残留尾迹随基体温度升高而愈发明显；随后数值模拟了硅油在非等温粗糙表面的碰撞过程，并揭示了基体温度和表面粗糙度的影响机制.本文中研究成果为理解非等温粗糙金属表面液滴的撞击行为提供了丰富的理论和试验依据.     

镓铟锡液滴撞击泡沫金属表面的运动学特性研究

常温下为液态的镓铟锡合金以其优异的导热性能在具有特殊要求的传热领域有着重要的应用价值,与传统流动介质相比较大的表面张力使得其产生的流动现象必有所区别.本文研究镓铟锡所形成的液滴撞击泡沫金属表面后所产生的铺展、回缩及回弹现象.采用高速相机拍摄液滴投影轮廓随液滴运动的变化过程,并通过图像处理获得不同撞击速度、底板表面孔径下的液滴铺展系数、中心位置轮廓高度以及液滴回弹后在空中的振动特性.研究结果表明:具有较高表面张力的镓铟锡液滴的铺展系数随无量纲时间的变化在铺展初始阶段仍满足常规流体的1/2次幂关系,只在铺展后期与底板的无量纲孔径有关系;液滴的最大铺展系数在较小无量纲孔径底板大于在光滑镍板,且随底板无量纲孔径增大而逐渐减小;在回弹过程,由于底板孔隙结构的存在使得液滴回弹后在空中的振动呈现3种形态:规则的横向和纵向振动、带旋转的横向和纵向振动以及旋转振动;最后,通过对振动频率的拟合和分析,进一步拓展了传统振动频率理论公式在非规则振动过程预测中的应用.      

镓铟锡液滴撞击泡沫金属表面的运动学特性研究

常温下为液态的镓铟锡合金以其优异的导热性能在具有特殊要求的传热领域有着重要的应用价值,与传统流动介质相比较大的表面张力使得其产生的流动现象必有所区别.本文研究镓铟锡所形成的液滴撞击泡沫金属表面后所产生的铺展、回缩及回弹现象.采用高速相机拍摄液滴投影轮廓随液滴运动的变化过程,并通过图像处理获得不同撞击速度、底板表面孔径下的液滴铺展系数、中心位置轮廓高度以及液滴回弹后在空中的振动特性.研究结果表明:具有较高表面张力的镓铟锡液滴的铺展系数随无量纲时间的变化在铺展初始阶段仍满足常规流体的1/2次幂关系,只在铺展后期与底板的无量纲孔径有关系;液滴的最大铺展系数在较小无量纲孔径底板大于在光滑镍板,且随底板无量纲孔径增大而逐渐减小;在回弹过程,由于底板孔隙结构的存在使得液滴回弹后在空中的振动呈现3种形态:规则的横向和纵向振动、带旋转的横向和纵向振动以及旋转振动;最后,通过对振动频率的拟合和分析,进一步拓展了传统振动频率理论公式在非规则振动过程预测中的应用.     

液滴撞击具有浸润性分布的倾斜固壁铺展行为的格子Boltzmann研究

采用基于单组分多相伪势模型的格子Boltzmann方法,模拟了三维液滴撞击左右两侧浸润性不同的倾斜固壁的铺展过程,获得了液滴在壁面两侧的铺展因子、相对铺展宽度、相对高度和液滴运动速度随时间的变化情况,研究了壁面浸润性分布和壁面倾斜角度对液滴铺展过程的影响．结果表明,液滴在倾斜壁面的铺展过程受到重力和表面力的综合作用,重力影响液滴的铺展和沿壁面向下的滑动,壁面浸润性分布影响液滴向壁面亲水侧横向移动．     

平壁液滴静态铺展影响因素的研究

通过建立液滴撞击固体平壁的静态铺展力学平衡的数学模型,从理论上得到了静态铺展半径与液滴物性参数、以及液滴与固体壁面接触角之间关系的数学表达式,将理论结果与数值模拟的结果进行了比较,两者吻合较好.比较了不同条件下液滴的静态铺展半径的变化规律,分别得到了液滴密度、体积、表面张力和接触角等因素对液滴静态铺展半径的影响规律.      

基于SPH方法的湿润性固壁边界条件模拟研究

固体壁面由于表面特殊结构和材料属性,时常表现出对交界面上水体的吸附作用,而这一特征对微小水体作用尤为明显。本文提出了一种湿润性固壁边界条件的计算方法,即假设壁面粒子的亲水性以及毛细吸附作用统一表现为对支持域内流体粒子的吸附力。基于光滑粒子流体动力学（SPH）方法,模拟了静态液滴在不同湿润性壁面上的变形至稳定过程。模拟了液滴撞击疏水壁面的过程,将液滴的运动过程分为碰撞、铺展、回缩和回弹四个阶段,分析各阶段壁面受力分布情况。研究表明：根据模拟液滴静态接触角的变化特点,本文湿润性固壁边界条件可以较好的反映出壁面湿润性;液滴撞击输水表面的模拟数据与试验结果趋势上吻合良好;壁面压力波伴随着液滴的铺展和回缩传播并衰减;只有在回弹后期液滴即将脱离壁面时壁面拉力起主导作用,其余各时刻壁面均以压力为主。     

Viscosity of alumina nanoparticles dispersed in car engine coolant

The present paper, describes our experimental results on the viscosity of the nanofluid prepared by dispersing alumina nanoparticles (<50 nm) in commercial car coolant. The nanofluid prepared with calculated amount of oleic acid (surfactant) was tested to be stable for more than 80 days. The viscosity of the nanofluids is measured both as a function of alumina volume fraction and temperature between 10 and 50 °C. While the pure base fluid display Newtonian behavior over the measured temperature, it transforms to a non-Newtonian fluid with addition of a small amount of alumina nanoparticles. Our results show that viscosity of the nanofluid increases with increasing nanoparticle concentration and decreases with increase in temperature. Most of the frequently used classical models severely under predict the measured viscosity. Volume fraction dependence of the nanofluid viscosity, however, is predicted fairly well on the basis of a recently reported theoretical model for nanofluids that takes into account the effect of Brownian motion of nanoparticles in the nanofluid. The temperature dependence of the viscosity of engine coolant based alumina nanofluids obeys the empirical correlation of the type: log (μ_nf) = A exp(BT), proposed earlier by Namburu et al.     

Particle velocimetry inside Newtonian and non-Newtonian droplets impacting a hydrophobic surface

A particle velocimetry technique is described which enables the measurement of the fluid velocity inside impacting drops. Using high speed photography of 2 μm fluorescent tracer particles suspended in the fluid, the velocity field was measured as a function of time and radial position. The potential of the technique is illustrated using velocimetry measurements of drops of pure water and aqueous solutions of 200 ppm poly-(ethylene oxide) (PEO). Dilute solutions of PEO have been known for some time to suppress the rebound of water from hydrophobic surfaces. The dissipation has traditionally been attributed to an increased extensional viscosity as the polymers stretch in the extensional flow of the droplet. Our results enable us to infer that the extensional viscosity of PEO drops, during both the spreading and retraction phase, is similar to that of pure water. The data suggest that the true source of dissipation lies at the droplet edge. We also show, by analysing the spreading of water drops, that the Roisman-Yarin theory for a droplet spreading on a surface is valid in the bulk of the droplet prior to the final stages of spreading.     

Free Convection of Non-Newtonian Nanofluids in Porous media with Gyrotactic Microorganisms

The free convection of non-Newtonian nanofluids along a vertical plate in porous medium is investigated numerically. It is assumed that the medium contains gyrotactic microorganisms along with nanoparticles and the plate is subjected to prescribed temperature, concentration of nanoparticles and density of motile microorganisms. It is further assumed that the plate is impermeable. The governing partial differential equations are reduced to nonlinear ordinary differential equations using similarity transformations. The nonlinear ordinary differential equations are then solved by a finite difference numerical method. The effects of controlling parameters on several dimensionless quantities and numbers of our interest are investigated. The numerical results are compared with the published data and an excellent agreement has been found. It is found that nanofluid and bioconvection parameters have strong effects on local Nusselt, Sherwood and density numbers.     

Analytical considerations of flow/thermal coupling of nanofluids in foam metals with local thermal non-equilibrium (LTNE) phenomena and inhomogeneous nanoparticle distribution

Foam metals with micro pores own excellent thermal performance, however, poor heat conductive ability of most heat-transfer fluids restricts further heat transfer improvement. Combination of foam metal and nanofluid with highly conductive nanoparticles is a promising solution. Convective thermal characteristics of nanofluids in porous foams are theoretically investigated in this work. Effects of Brownian motion and thermophoretic diffusion of nanoparticles in the base fluid on thermal performance are considered. The nanoparticle and the base-fluid are considered to be in thermal equilibrium and the temperature difference between the nanofluid and foam ligaments is especially considered. Compared with the base-fluid flow in a duct, the velocity distribution for the nanofluid flow in a porous foam is more uniform with a decreased dimensionless temperature. The pressure drop of the nanofluid increases with an increase in the concentration of the nanoparticles. By employing foam metals and nanofluid, the cross-sectional temperature becomes closer to the wall temperature. Simultaneously, notable difference between solid and fluid temperatures can be observed, revealing the LTNE effect of the nanofluid on the porous foam. It is found that the Nusselt number first increases and then decreases with an increase in nanoparticle concentration. Furthermore, the Nusselt number decreases with an increase in the foam porosity. It is found that the thermal performance of a nanofluid in a plain tube is different from that in the foam metals.     

润滑力学中非牛顿流动的普遍Reynolds方程

本文导出了润滑力学中关于非牛顿流动的普遍 Reynolds 方程。这一方程适用于多种非牛顿流动模型,可以用于解算热流体动力润滑或热弹性流体动力润滑膜的压力分布。本文给出了一种同时求出剪应力、剪切率、速度和等效粘度的解法,并以两种润滑力学中常用的流变模型为例,应用这一方程得到了线接触热弹性流体动力润滑问题的数值解。     

Measurement of temperature-dependent thermal conductivity and viscosity of TiO2-water nanofluids

Nanofluid is an innovative heat transfer fluid with superior potential for enhancing the heat transfer performance of conventional fluids. Many attempts have been made to investigate its thermal conductivity and viscosity, which are important thermophysical properties. No definitive agreements have emerged, however, about these properties. This article reports the thermal conductivity and dynamic viscosity of nanofluids experimentally. TiO₂ nanoparticles dispersed in water with volume concentration of 0.2–2 vol.% are used in the present study. A transient hot-wire apparatus is used for measuring the thermal conductivity of nanofluids whereas the Bohlin rotational rheometer (Malvern Instrument) is used to measure the viscosity of nanofluids. The data are collected for temperatures ranging from 15 °C to 35 °C. The results show that the measured viscosity and thermal conductivity of nanofluids increased as the particle concentrations increased and are higher than the values of the base liquids. Furthermore, thermal conductivity of nanofluids increased with increasing nanofluid temperatures and, conversely, the viscosity of nanofluids decreased with increasing temperature of nanofluids. Moreover, the measured thermal conductivity and viscosity of nanofluids are quite different from the predicted values from the existing correlations and the data reported by other researchers. Finally, new thermophysical correlations are proposed for predicting the thermal conductivity and viscosity of nanofluids.     

Multiphysics of multifunctional nanofluids based on different oxides nanoparticles and glycerol fluid

Nanofluid (NF) materials consisting of glycerol (Gly) and different inorganic nano oxides (TiO₂, ZnO, Al₂O₃, and SiO₂ for the oxides concentration of 0.01 wt% to the weight of Gly base fluid) were prepared by a two-step method through ultrasonic cavitation process. These nanofluids were investigated by employing an X-ray diffractometer (XRD), ultraviolet–visible (UV–Vis) spectrophotometer, 20 Hz to 1 MHz frequency range dielectric relaxation spectroscopy (DRS), ultrasonic interferometer, and rotational viscometer. The multiphysics of these nanofluids includes structural and optical properties, dielectric permittivity, electrical conductivity, conductivity relaxation, ultrasound velocity, adiabatic compressibility, acoustic impedance, viscosity, density, thermal conductivity, and viscoacoustic relaxation were characterized. The XRD patterns identified monodispersed and stable suspensions of these different characteristic nanoparticles in the hydrogen-bonded 3D supramolecular structure of ultra-high viscous glycerol fluid which were supported by their UV–Vis absorbance analyses. The energy band gap values of the TiO₂ and ZnO containing nanofluids were found primarily ruled by the characteristic optical properties of these oxides nanomaterials. The complex dielectric and various electrical functions studied at 25 °C revealed that the suspension of different oxide nanoparticles in the glycerol fluid increased the static permittivity whereas reduced the direct current electrical conductivity which showed strong conductivity relaxation process dependence. The rheological measurements of the formulated nanofluids were performed over a shear rate range of 0.4–40 s⁻¹ at temperatures of 25–55 °C. The linear relationship between shear rate and shear stress and also the shear rate-independent viscosity revealed the Newtonian behaviour of these nanofluids. The shear viscosity non-linearly decreased with the increase of temperature and exhibited the Arrhenius behaviour for all different oxides containing Gly-based nanofluids. The acoustic parameters of the nanofluids were altered unevenly with types of nano oxides and inferred some structure-property correlations. The promising technologically useable properties of these nanofluids were expected to impact their potential applications in optoelectronics, UV-blocking, sensing, nanodielectrics, energy storing and electric insulation, heat transfer systems, and also in materials processing for the development of innovative soft condensed devices.