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1.
The rotation of a spin subject to an on-resonance soft pulse and simultaneously to a soft pulse at a nearby frequency may strongly deviate from the desired rotation expected for a single on-resonance pulse. The deviation is the result of transient frequency shifts of the spin caused by the off-resonance irradiation. We show that the resulting error can be corrected by shifting the frequency of the on-resonance pulse in such a way that it tracks the shift of the spin frequency. Experimentally, the effectiveness of this simple and intuitive method is demonstrated for simultaneous inversions at nearby frequencies in the case of both coupled and uncoupled spins. Simulations predict that the correction technique is effective for arbitrary pulse shapes and tip angles and is particularly useful when the frequency window of the shaped pulse is two to eight times the frequency separation between the chemical shifts of the two spins.  相似文献   

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3.
The operator formalism of quantum mechanics is applied to the problem of reflection and transmission of non-relativistic spin particles at stratified media. Two basic numerical methods in optics of stratified media, the matrix method of Abeles and the formalism of Airy, have been thus generalized for non-relativistic spin particles. Such an approach provides numerical solution of the problem of interaction of a spin particle in an arbitrary state with a spin-dependent one-dimensional potential. Application of the generalized Airy's formalism to neutrons in magnetically non-collinear stratified media has been considered as an example.  相似文献   

4.
For a model molecular system with one vibrational degree of freedom and three electronic states coupled by pump and probe laser pulses in a condensed medium, the response signal in a femtosecond pump-probe experiment is calculated. The potential curves of all three states are described by the Morse potential. Calculations are performed using two qualitatively different approaches to describing the medium-induced relaxation: with memory of the relaxation process and without memory (Markovian approximation). The temporal evolution of the vibrational wave packet in the intermediate electronically excited state is described using a master equation for the density matrix of the molecular system, which is derived within the framework of the Nakajima-Zwanzig formalism. It is demonstrated that, at short delay times, when the proposed approach is applicable, taking into account memory effects can substantially change the form of the pump-probe experiment signal in comparison with the signal calculated in the Markovian approximation.  相似文献   

5.
Paul J  Lee MW  Shore KA 《Optics letters》2004,29(21):2497-2499
An experimental demonstration of the effect of chaos pass filtering on high-frequency message transmission in the complete synchronization regime is reported. The opportunity for chaotic message decoding at frequencies up to 6 GHz is shown.  相似文献   

6.
A formalism is proposed to study the electronic and transport properties of graphene sheets with corrugations as the one recently synthesized. The formalism is based on coupling the Dirac equation that models the low energy electronic excitations of clean flat graphene samples to a curved space. A cosmic string analogy allows to treat an arbitrary number of topological defects located at arbitrary positions on the graphene plane. The usual defects that will always be present in any graphene sample as pentagon–heptagon pairs and Stone–Wales defects are studied as an example. The local density of states around the defects acquires characteristic modulations that could be observed in scanning tunnel and transmission electron microscopy.  相似文献   

7.
The generalized version of the Montroll-Weiss formalism for continuous-time random walks is employed to show that some of the asymptotic results for large times appropriate to the ordinary walk become exact when the start of the observations is arbitrary.  相似文献   

8.
The reflection, transmission, and absorption of a symmetric electromagnetic pulse are calculated. The carrier frequency of the pulse is close to the frequency of direct interband transitions in a quantum well (QW). The QW energy levels are assumed to be discrete, with two closely spaced excited levels being taken into account. The QW width is assumed to be sufficiently large and comparable to the light wavelength corresponding to the pulse carrier frequency. In this case, the dependence of the momentum matrix element for the interband transition on the light wave vector should be taken into account. The refractive indices of the QW and barriers are assumed to be equal. The problem is solved for an arbitrary relation between the radiative and non-radiative lifetimes of the excited electronic states. It is shown that spatial dispersion considerably affects the shapes of the reflected and transmitted pulses. The greatest changes occur in the case where the inverse radiative lifetime is close to the difference between the frequencies of the interband transitions considered.  相似文献   

9.
The scattered wave formalism is developed for a quantum subsystem interacting with the external environment through open boundaries. The total wave function is divided into incident and scattered components and Markovian outgoing wave boundary conditions are applied to the scattered wave function. This formalism significantly reduces the computational effort relative to other methods which rely on Green functions and memory kernels. The method is applied to one-dimensional barrier scattering and to a three-dimensional model for the field effect transistor.  相似文献   

10.
The common matrix formalism for multi-layer systems is generalized to describe the optical field propagation along an arbitrary cascade of step discontinuities in a planar dielectric waveguide. The reflection and transmission properties of the step cascade are modelled by rigorous operator relations in a Hilbert-space calculus. In this way the complete propagation problem is reduced to two basic transformations. TE- and TM-polarized fields are treated simultaneously.  相似文献   

11.
In this Letter we propose a new formalism to map history-dependent metadynamics in a Markovian process. We apply this formalism to model Langevin dynamics and determine the equilibrium distribution of a collection of simulations. We demonstrate that the reconstructed free energy is an unbiased estimate of the underlying free energy and analytically derive an expression for the error. The present results can be applied to other history-dependent stochastic processes, such as Wang-Landau sampling.  相似文献   

12.
We present the experimental realization of a method to generate predetermined, arbitrary pulse shapes after transmission through an optical fiber in the nonlinear regime. The method is based on simulating the reverse propagation of the desired pulse shape in the fiber. First, linear and nonlinear parameters of a single-mode step-index fiber required for the simulation are determined. The calculated pulse shapes are then generated in a pulse shaper.  相似文献   

13.
Using pulsed-field-gradient (PFG) experiments, the sizes of the pores in ordered porous media can be estimated from the "diffraction" pattern that the signal attenuation curves exhibit. A different diffraction pattern is observed when the experiment is extended to a larger number (N) of diffusion gradient pulse pairs. Simulations to calculate signal values from arbitrary gradient waveforms are performed for diffusion in restricted geometries using a matrix operator formalism. The simulations suggest that the differences in the characteristics of the attenuation curves are expected to make it possible to measure smaller pore sizes, to improve the accuracy of pore size measurements and potentially to distinguish different pore shapes using the N-PFG technique. Moreover, when an even number of PFG pairs is used, it is possible to observe the diffraction pattern at shorter diffusion times and measure an approximation to the average pore size even when the sample contains pores with a broad distribution of sizes.  相似文献   

14.
By using tailored pulse sequences from a novel, 1.5-microm direct space-to-time pulse shaper driving a high-speed photodetector, we have achieved, for the first time to our knowledge, millimeter-wave arbitrary waveform generation at center frequencies approaching 50 GHz. By appropriately designing the driving optical pulse sequences, we demonstrate the ability to synthesize strongly phase- and frequency-modulated millimeter-wave electrical signals on a cycle-by-cycle basis.  相似文献   

15.
The surface plasmon dispersion relation for a two component degenerate plasma system is obtained in spherical geometry, using the hydrodynamical model. The general solution for arbitrary value of angular quantum number l has been shown to have two branches, one of higher frequency and another of lower frequency. The formalism is explicitly applied to the case of electron-hole droplets (EHD) in silicon and germanium, and the normal mode frequencies have been computed for l = O, 1 and 2 values  相似文献   

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17.
We present an investigation of the optical properties of semiconductors, which are excited by a strong laser pulse. On the basis of a nonequilibrium Green's function technique (Keldysh formalism) we study the system of electrons and holes, interacting among themselves and with the exciting pulse. A set of coupled equations for the one-particle Green's function and the transverse and longitudinal polarizability is derived, which is valid for arbitrary excitation conditions. For an initially prepared state, which is not too far from a quasiequilibrium state of the excited system, the theory is elaborated in detail, using a screened Hartree-Fock approximation scheme. Within this approximation earlier results of various theoretical approaches are found to be special cases of the equilibrium limit of the present theory.  相似文献   

18.
It is a significant subject to explore effective quantum communication protocol and enhance the efficiency of the transmission process in noisy environments. In this paper, we investigate the bidirectional controlled remote preparation of an arbitrary single-qubit state in the presence of dissipative environments by using two EPR states as the entanglement source. We first construct the quantum circuit of our scheme by means of unitary matrix decomposition procedure, then the effects of the Markovian and non-Markovian environmental noises acting on the EPR states are considered through the analytical derivation and numerical calculations of the corresponding average fidelity. Moreover, we adopt two methods of weak measurement reversal (WMR) and detuning modulation to improve the average fidelity. Our results show that the average fidelity can be remarkably enhanced under appropriate conditions of the WMR strength and the detuning. Compared with the average fidelity behaviors in dissipative environments, it is also shown that the two methods for fidelity improvement are more efficient in the non-Markovian regime than in the Markovian regime.  相似文献   

19.
Defects play a key role in the electronic structure of graphene layers flat or curved. Topological defects in which an hexagon is replaced by an n-sided polygon generate long range interactions that make them different from vacancies or other potential defects. In this work we review previous models for topological defects in graphene. A formalism is proposed to study the electronic and transport properties of graphene sheets with corrugations as the one recently synthesized. The formalism is based on coupling the Dirac equation that models the low energy electronic excitations of clean flat graphene samples to a curved space. A cosmic string analogy allows to treat an arbitrary number of topological defects located at arbitrary positions on the graphene plane. The usual defects that will always be present in any graphene sample as pentagon–heptagon pairs and Stone-Wales defects are studied as an example. The local density of states around the defects acquires characteristic modulations that could be observed in scanning tunnel and transmission electron microscopy.  相似文献   

20.
本文提出了用量子力学的空间转动变换算符描述特形脉冲的方法。它把任意的特形脉冲用三个欧拉角来表示,并且使得在特形脉冲下的相干演化可以很容易地利用多极NMR理论,张量算符理论或者积算符理论来分析,作为例子,用数值方法计算了高斯脉冲的三个参数。  相似文献   

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