有机材料反饱和吸收特性分析

从能级角度出发，结合入射激光脉宽对粒子吸收方面的影响，用速率方程模拟了各能级粒子数的瞬时变化关系，给出了激光脉宽与能级寿命可比拟时反饱和吸收的动态解，表明粒子在能级上的分布情况。用C60和HITCI(1,1′,3,3,3′,3′hexa methyl lindo tricarbocyanine Iodide)的实验参数理论模拟了激发态吸收截面大于基态吸收截面时透射率随光强的变化关系，用以说明大的上能级吸收截面可以抑制光强过大时引起的饱和吸收，增强材料的非线性光限幅特性。     

基于反饱和吸收和自聚集两种效应的光限幅器

用酞菁酮金属有机染料首次演示了基于反饱和吸收和自聚焦两种效应的光限幅器。实验和理论分析表明，这种限幅器的输入阈值功率由反饱和吸收决定，而自聚焦使限幅器的最大限幅输出功率降低，限幅效果显著增强。     

基于反饱和吸收和自聚焦两种效应的光限幅器

用酞菁铜金属有机染料首次演示了基于反饱和吸收和自聚焦两种效应的光限幅器．实验和理论分析表明，这种限幅器的输入阈值功率由反饱和吸收决定，而自聚焦使限幅器的最大限幅输出功率降低，限幅效果显著增强．     

有机材料ZnTBP-CA-PhR的非线性吸收和光学限幅性能

报道了一种新型有机材料ZnTBP-CA-PhR的光学非线性吸收特性，此材料在激光作用下，在可见光区域具有反饱和吸收，再反饱和吸收和饱和吸收效应.同时发现该材料优良的光学限幅性能，不仅光限幅的阈值低，而且限幅前光透射呈线性状态没有光学非线性效应.用5能级结构模型及速率方程模拟了饱和及反饱和的实验曲线，分析了非线性吸收等的物理机理.     

C60介质反饱和吸收动力学

采用速率方程理论研究C₆₀分子实现反饱和吸收的动力学过程,以YAG倍频调Q脉冲激光照射C₆₀甲苯溶液,实验验证了理论模拟的正确性。还分析了分子各能级对反饱和吸收的贡献以及不同激光波长和脉宽对反饱和吸收的影响。 关键词：     

C60／PSt复合材料的反饱和吸收与光限幅特性

报道了Ｃ６０／ＰＳｔ（Ｐｏｌｙｓｔｒｅｎｅ）复合材料的制备，测量了材料的线性吸收光谱，研究了不同线性透射率的Ｃ６０／ＰＳｔ材料的反饱和吸收与光限幅特性．     

有机材料ZnTBP—CA—PhR的非线性吸收和光学限幅性能

报道了一种新型有机材料znTBP—CA—PhR的光学非线性吸收特性，此材料在激光作用下，在可见光区域具有反饱和吸收，再反饱和吸收和饱和吸收效应．同时发现该材料优良的光学限幅性能，不仅光限幅的阈值低，而且限幅前光透射呈线性状态没有光学非线性效应．用5能级结构模型及速率方程模拟了饱和及反饱和的实验曲线，分析了非线性吸收等的物理机理．     

新型卟啉衍生物反饱和吸收研究

利用纳秒脉冲激光下的z扫描方法对两种新型卟啉衍生物在450 nm—490 nm范围内的反饱和吸收进行了研究.通过与四苯基卟啉的比较发现，在Soret和Q吸收带之间，两种新型卟啉衍生物都具有大的反饱和吸收.采用五能级模型对实验结果进行了分析，比较了在不同波长范围内各个样品的优势.实验结果表明，在450 nm—490 nm范围内，两种新型的卟啉衍生物有着比四苯基卟啉更好的光限制应用前景. 关键词： 反饱和吸收 z扫描')" href="#">z扫描 卟啉衍生物     

无反转激光:增益与饱和

在下能级相干的型三能级系统得到了原子密度矩阵方程的严格解。在强相干情形分析了产生无反转激光的抽运条件，并导出了光强饱和项。 关键词：     

C60/PMMA复合材料的反饱和吸收与光限幅特性研究

本文报导C₆₀/PMMA复合材料的制备方法,并采用调QNd:YAG倍频脉冲激光照射C₆₀/PMMA夏合材料,研究了其反饱和吸收与光限幅将性。在线性透射率为46%条件下,光限幅阈值能量密度为65mJ/cm²,材料破坏能量密度阈值为600mJ/cm².与C₆₀甲苯溶液相比具有一定的优点。     

Coherence Time Measurement of Picosecond Pulses Using Reverse Saturable Absorption in Lead Phthalocyanine

ＣｏｈｅｒｅｎｃｅＴｉｍｅＭｅａｓｕｒｅｍｅｎｔｏｆＰｉｃｏｓｅｃｏｎｄＰｕｌｓｅｓＵｓｉｎｇＲｅｖｅｒｓｅＳａｔｕｒａｂｌｅＡｂｓｏｒｐｔｉｏｎｉｎＬｅａｄＰｈｔｈａｌｏｃｙａｎｉｎｅＬＩＦｅｎｇＳＯＮＧＹｉｎｇｌｉｎＹＡＮＧＫｕｎＬＵＩＳｈｕｔｉ...     

一种新型有机金属化合物纳秒时域饱和吸收特性研究

合成了一种新型有机金属配合物Cetyltrimethylammonium-bis(2-thioxo-1,3- dithiole- 4,5-dithiolato)-copper(简称CtCu)材料.采用单光束Z扫描测试技术,在波长为1 053 nm,脉宽为1 ns的条件下研究了该样品的三阶非线性光学性质.研究发现,该材料具有很强的饱和吸收特性,激发态的有效吸收截面为σeff＝1.10×10－19 cm2,与基态吸收截面的比值为1∶484.利用非线性透过率实验验证了材料的饱和吸收特性,并对其产生机理进行了分析.实验结果表明,该材料在近红外波段的激光脉冲压缩方面有潜在的应用前景.     

半导体可饱和吸收镜作为被动调Q吸收体的发展状况

简介了近年来发展起来的若干种新型固体激光器被动调Q用吸收体：掺Cr4+系列，Cr，Nd∶YAG自调Q激光晶体，人眼安全激光器被动调Q用吸收体，GaAs吸收体，半导体可饱和吸收镜。着重介绍了固体激光器和光纤激光器调Q用半导体可饱和吸收镜的原理、研制方法及应用状况。     

Ultrafast Saturable Absorption of Core/Shell Colloidal Quantum Dots

Ultrafast saturable absorption (SA) materials that are capable of blocking the optical absorption under strong excitation have extensive applications in photonic devices. This work presents core/shell colloidal quantum dots (CQDs) which have the quantized energy levels, excellent band gap tunability, and possess significant SA performance. When the band gap is close to the pump pulse energy, the CQDs show significant resonant SA response. At the same excitation conditions, the core/shell CQDs dispersions show better SA response than graphene dispersions, and comparable to the recently reported molybdenum disulfide. The carrier dynamics of the SA of the CQDs is analyzed systematically. The research has also found that the two‐photon absorption of the CQDs show nearly cubic power law of the band gap, while the SA performance keeps almost the same in the nonresonant regime. Further, superior passive Q‐switched laser behavior is observed using the CQDs as a saturable absorber. The results directly reveal the physical processes of this basic problem and broaden the applications of CQDs in photonic devices.     

Nonresonant and Resonant Nonlinear Absorption of CdSe-Based Nanoplatelets

We present a comprehensive understanding of the nonlinear absorption characteristics of CdSe-based nanoplatelets(NPLs) synthesized by the solution-phase method and the colloidal atomic layer deposition approach through Z-scan techniques at 532 nm with picosecond pulses. The CdSe NPLs exhibit strong two-photon induced free carrier absorption(effective three-photon absorption) upon the nonresonant excitation, resulting in a remarkable optical limiting behavior with the limiting threshold of approximately 75 GW/cm~2. A nonlinear optical switching from saturable absorption(SA) to reverse saturable absorption(RSA) with increasing the laser intensity is observed when coating CdSe NPLs with a monolayer of CdS shell to realize the resonant absorption. The SA behavior originates from the ground state bleaching and the RSA behavior is attributed to the free carrier absorption.These findings explicitly demonstrate the potential applications of CdSe-based NPLs in nonlinear optoelectronics such as optical limiting devices, optical pulse compressors and optical switching devices.     

Saturable and reverse saturable absorption in aqueous silver nanoparticles at off-resonant wavelength

Silver nano-colloid was prepared by chemical reduction method and its nonlinear absorption properties were investigated by using open aperture z-scan experiment with nanosecond laser pulses operating at 532?nm. Interestingly, a switch over from saturable absorption to reverse saturable absorption was observed when the input intensity is increased from 28.1 to 175.8?MW/cm². The underlying mechanism responsible for the observed switching behaviour is the interplay between ground state plasmon band bleaching and excited state absorption. Theoretical fitting was done by using a model in which nonlinear absorption coefficient as well as saturation intensity are incorporated.     

Saturable Absorption Enchantment of Au Nanorods Based on Energy Transfer between Longitudinal and Transverse Energy Levels

Four kinds of Au nanorods(NRs)with different aspect ratios are designed to adjust the relationship between resonance energy level of longitudinal(L)and transverse(T)modes.During the femto-second Z-scan experiments,huge saturable absorption phenomena are observed while the energy level T is located between one to two times of the energylevel L.This means that the energy may transfer between longitudinal and transverse energylevels in the same and/or different Au NRs.It effectively depresses the production of revised saturated absorption and increases the saturable absorption efficiency.This method is significant for the preparation of high-efficiency saturable absorption devices.     

Saturable absorption and reverse saturable absorption on silver particles with different shapes

Micro/nanostructured silver particles with different shapes (flower, wire, and rod) have been prepared and characterized. All the open aperture z-scan curves of silver microrods and silver nanoflowers present a typical reverse saturable absorption. With the increase of incident intensity, the nonlinear absorption coefficients and the third-order optical susceptibilities ImX⁽³⁾ of nanoflowers increase, but those of silver microrods decrease. Moreover, the silver nanowires show the conversion from saturable absorption to reverse saturable absorption. There was no definite correlation between incident intensity and nonlinear absorption coefficient (β) under the conditions studied herein. And nonlinear optical properties of micro/nanostructured silver particles are dependent on the particle shape in suspensions at 800 nm.     

Theoretical Analysis of Photon-Mode Super-Resolution Optical Memory Using Saturable Absorption Dye

The possibility of a super-resolution optical memory using a saturable absorption dye mask layer is theoretically discussed. An equation which estimates the transmittance change of the mask layer has been derived. The numerical simulation shows that an efficient super-resolution is performed when the initial optical density of the mask layer is high.