Directional correlations of gamma cascades in153Gd

TheEC-decay of¹⁵³Tb to the levels of¹⁵³Gd has been studied in singles and coincidence mode using high resolution x-ray andγ-ray Ge(Li) detectors. The results, in general, are in agreement with the recent findings of Tuurnalaet al. showing a very high density of low-spin states in¹⁵³Gd. The results of theγγ directional correlation experiment using two Ge(Li) detectors together with the I.C.C. data have been used in assigning the spin and parity of 5/2^?, 5/2^?, 3/2^?, 3/2⁺, 5/2⁺, 3/2⁺ and 3/2⁺ to the 41.6, 109.8, 129.1, 212.0, 303.5, 945.6 and 1102.0 keV states respectively. Multipolarity assignments to majority of theγ-transitions have been made from the I.C.C. data obtained through the knowledge of ourγ-ray intensities and the published conversion-electron intensities. From the multipole characters of theγ-transitions, parity assignments have been made to seven states in¹⁵³Gd. Our results have been discussed and compared with that of Tuurnalaet al.     

Negative-parity bands in the 88-neutron nuclei153Tb and155Ho

Bands of negative-parity levels have been observed in in-beam studies of¹⁵³Tb and¹⁵⁵Ho. The data are qualitatively accounted for in the rotation-alignment model as decoupled bands based on the h_11/2 proton orbital. Nuclear Reactions:¹⁵³Eu(α, 4nγ)¹⁵³Tb,E=45–55 MeV;¹⁵⁰Sm(¹⁰B, 5nγ)¹⁵⁵Ho,E=60–70 MeV; measuredE _γ,I _γ (0), γ ? γ coinc.,E _e, I _e ^K ,¹⁵³Tb and¹⁵⁵Ho deduced levels,J, π. Ge(Li) and Si(Li) detectors. Enriched targets.     

Level structure of the 89-neutron nucleus 153Gd: (I). Levels and gamma-transitions in 153Gd excited in the decay of 153Tb

Investigations of the properties of ¹⁵³Gd excited states populated in ¹⁵³Tb decay were continued. The following measurements were performed: coincidence spectra e^?γ with L41, K93 + L52, K110, K129 + L87 + L88 and K195 + L152 keV conversion electron lines, angular correlations of high energy γ-cascades going through the 109.7 keV level, delayed e^?γ and e^?e^? coincidence spectra to determine the half-lives of 41.5, 93.3, 109.7, 129.1,183.5, 212.0 and 216.1 keV states, R(135°, ± B) parameters of IPAC for the 102–110 and 83–129 keV cascades using ¹⁵³Tb sources implanted into Fe foil.A decay scheme of ¹⁵³Tb containing 50 excited levels is proposed. Their spins, parities, $\text{log}\text{?t}$ and, for low-lying levels, also the mean half-lives have been determined. An estimation of the g-factors of the 109.7 and 129.1 keV levels has been given. On the basis of half-lives of investigated states absolute values of reduced γ-transition probabilities for these states have been calculated. The structure of the ground state of ¹⁵³Gd is discussed.     

Study of low-lying states in151Eu via (n,n′γ) reaction

The levels of¹⁵¹Eu have been investigated in the (n,n′γ) reaction using nuclear reactor fast neutrons. The energies, intensities and angular distributions of theγ-rays have been measured with the Ge(Li) spectrometer. Four rotational bands with the following band heads and Nilsson configurations have been identified: ground state band, 5/2⁺ [402]; 21.5 keV, 7/2⁺[404]; 196.5 keV, 3/2⁺[411]; 260.5 keV, 5/2⁺[413]. The low spin states at 332.2 and 336.2 keV have been tentatively assigned to the l/2⁺[411] Nilsson orbital, but 522.8, 580.0 and 587.0 keV states to the 1/2⁺[420] Nilsson orbital. The negative parity levels at 353.7, 522.1 and probably 546.2 keV have been proposed basing on theh _11/2 proton state.     

Studies on the energy levels of153Eu following the β−-decay of153Sm

The level scheme of¹⁵³Eu was investigated by observing the gamma-rays following theβ ^?-decay of the 47 h¹⁵³Sm using a high purity Ge(HPGe) detector and a Ge(Li)-Nal(Tl) fast-slow coincidence spectrometer. The energies and relative intensities of about fifty six gamma-ray transitions were determined. Five of them at energies of 124.91, 431.65, 443.24, 487.75 and 623.73 keV were observed and confirmed for the first time in the present singles and/or gamma-gamma coincidence measurements. These new transitions could be fitted into a proposed level scheme of¹⁵³Eu. Theβ ^?-decay branching ratios as well as the log (ft) values were obtained.     

Microscopic structures of parity doublets in the151Pm,153Eu and155Eu nuclei

Microscopic structures of the proposed parity doublet bands in the odd-proton Z=61¹⁵¹Pm and Z=63^{153, 155}Eu nuclei are examined using the quasiparticle phonon nuclear model Hamiltonian including the residual pairing and multipole-multipole interactions. Octupole correlations between intrinsic nonrotational states are studied to check the suggested assignments of parity doublet partners in these nuclei. We conclude significant octupole correlations between a pair ofK ^π = 1/2^± doublets in each of these nuclei, with somewhat weaker correlations betweenK ^π = 3/2^± bands in both the Eu isotopes. No octupole connection between the lowestK ^π = 5/2^± bands is found; however, significant octupole collectivity, built on the low-lying 5/2^? bands, is predicted in the higher-lying 5/2⁺ bands which contain the 5/2⁺ [402] fragmented strength.     

High spin states in153Er

High spin states in¹⁵³Er have been populated in the¹⁴⁴Sm(¹²C, 3n)¹³³Er reaction. Excitation functions, lifetimes, angular distributions,γ-γ coincidences and internal conversion coefficients were measured. Three isomeric states at 2.75 MeV (T _1/2=400 ns), 2.95 MeV (T _1/2～10 ns) and 5.2 MeV (T _1/2=200 ns) have been observed. A fourth isomer seems to be weakly excited above 6.8 MeV. The level scheme proposed is discussed in term of the nuclear shell model.     

Der Zerfall des163Tb

The beta and gamma radiations of¹⁶³Tb have been investigated employing scintillation and semiconductor spectrometers and coincidence techniques. The sources were produced by the¹⁶³Dy(n,p)¹⁶³Tb reaction. A half-life of 19.5 min has been measured without evidence for an isomeric state in the half-life range of 2 sec to 7 d; especially a 6.5 h activity previously assigned to¹⁶³Tb could not be confirmed. 76 of the total of 82 gamma-ray transitions, representing 99.6% of the gamma-ray intensity, could be assigned to 23 levels in¹⁶³Dy. From beta and beta-gamma coincidence measurements aQβ-value of 1.7 ± 0.1 MeV has been determined. Spin and parity of 3/2⁺ are deduced for the ground state of¹⁶³Tb with the Nilsson configuration [411↑]. The level at 884 keV is interpreted as aJ ^π=1/2⁺ state with a high contribution of the three-quasiparticle configurationp[411↑]-p[523↑]-n[523↓] because of an allowed unhindered beta-ray transition to this level.     

Levels in152Gd and152Sm populated by the decay of152Eu

The energy level schemes of¹⁵²Gd and¹⁵²Sm have been established on the basis of singlesγ-spectra, andγ- γ coincidence measurements. Ge(Li) detectors were used to study the gamma spectra produced in the EC/β⁺ and β^? decays of¹⁵²Eu to¹⁵²Sm and¹⁵²Gd, respectively. Thirteen new transitions are reported and data from eleven coincidence gates enabled five new levels to be suggested. Relative intensities and logf t values were calculated and spin/parities deduced. Comparisons are made with new predictions of the Interacting Boson Model.     

High spin states in103Rh

High spin states in¹⁰³Rh have been studied using the¹⁰⁰Mo(⁷Li, 4n) reaction. Standard in-beam measurements involving singlesγ-ray,γ-γ-t coincidences, angular distribution and linear polarization measurements have been performed. A perturbed band based on a 9/2⁺ state is interpreted as ag _9/2 coupled band. A sequence built on a 1/2^? state is related to thep _1/2 state. At higher excitation energy, in the range 2.2–3.7 MeV, the strongΔI=1 cascade observed, connecting negative parity levels, probably arises from states including three quasi-particle configurations.     

Decay energies of the low-spin states of147Tb and148Tb

Using¹¹²Cd(⁴⁰Ar,pxn) reactions andγ-ray spectroscopy, the EC/β ⁺ and EC(K)/β ⁺ probability ratios were determined for individualβ-transitions in the¹⁴⁷Tb(1.6 h)→¹⁴⁷Gd and¹⁴⁸Tb(60 min)→¹⁴⁸Gd decays. Under assumption of applicability of theoretical ratios for allowedβ-decays on the first-forbidden nonunique transitions studied here, the experimental ratios were converted into information on decay energies. Combining the results with the known masses of^147,148Gd andQ _α values of neutron-deficient holmium-to-lutetium isotopes, mass excesses could be determined for¹⁴⁷Tb,¹⁴⁸Tb, low-spin¹⁵¹Ho, low-spin¹⁵²Ho,¹⁵⁵Tm,¹⁵⁶Tm and¹⁵⁹Lu.     

In-beam γ-ray studies of complex band structures and of isomeric states in 152, 153Dy nuclei

The high-spin level structures of ¹⁵²Dy and ¹⁵³Dy were studied experimentally with ^{154, 155}Gd(α xnγ) in-beam reactions, and for ¹⁵²Dy also with ${}^{\mathrm{144,\; 146}}\text{Nd}\text{(}{}^{12}\text{C, x}\text{n}\text{γ)}$ reactions. The experiments included measurements of singles γ-ray and conversion-electron spectra, γ-ray angular distributions and E_γ-t and E_γ-E_γ-t coincidences. A multiplicity filter set-up was used to study the feeding and decay of isomeric states in ¹⁵²Dy. In ¹⁵²Dy about twenty so far unknown levels were found, including two high-spin isomeric states with $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{≈ 60}\text{and}\text{≈ 13}\text{ns}$ at excitation energies E_x ≈ 5.04 and 6.08 MeV, respectively. These states are compared with recent calculations on yrast traps. The level scheme of ¹⁵³Dy contains 28 levels up to E_x = 4.1 MeV and $\text{J}{}^{\mathrm{\pi }}\text{= (}\text{37}\text{2}{}^{\mathrm{+}}\text{)}$. Band structures in both nuclei are discussed in comparison with other N = 86 and N = 87 isotones.     

Lifetimes of a dipole cascade in 192Hg

The β-spectrum of the 3^?-2⁺ transition in the decay of¹⁴⁶Pm has been investigated with a 4π-Si(Li)-semiconductor spectrometer in a β-γ-coincidence experiment for the first time. The shape factor has been determined: C(W)=1?0.394W}-0.275/W+0.044 W². The spin and parity of the ground state of¹⁴⁶Pm can be determined to be 3^?. The shape of this non-allowed spectrum indicates the existence of the “cancellation” or “selection rule” effect.     

Precise atomic masses of147Eu,147Gd,and151Tb derived from their decay properties

Theβ-decay energies of¹⁴⁷Eu,¹⁴⁷Gd, and¹⁵¹Tb were determined by usingγ-spectroscopical methods. The comparison of experimental with calculatedK-capture probabilities yielded theQ _EC values 1.690( _?16 ⁺²¹ )MeV and 2.203( _?13 ⁺¹⁹ )MeV for¹⁴⁷Eu and¹⁴⁷Gd, respectively. By measuring the ratio of positron decay to electron capture for two branches in¹⁴⁷Eu decay, the decay energiesQ _EC=1.702(13) MeV andQ _EC=1.709(18)MeV were derived. Also fromEC/β ⁺ ratios the valuesQ _EC=2.225(75) MeV for¹⁴⁷Gd, andQ _EC=2.566(12)MeV for¹⁵¹Tb were obtained. Earlier discrepancies in the mass adjustment of these isotopes were removed. In course of the present studiesγ-decay properties of¹⁴⁷Eu and¹⁴⁷Gd were reinvestigated.     

Ground state properties and β-decay half-lives near 132Sn in a self-consistent theory

The level scheme of⁹⁵Tc has been investigated with Ge(Li)-detectors by observing the γ-rays after the decay of 1.65 h⁹⁵Ru. The energies and intensities of theγtransitions were extracted fromγ-singles andγγ-coincidence spectra. In the decay of⁹⁵Ru 88γ-transitions were observed; a scheme of⁹⁵Tc with 25 levels is proposed into which 86 transitions could be accomodated. Spin and parity assignments were made from log (ft) values andγ-ray branching ratios. The level structure of⁹⁵Tc is compared with that of the other odd Tc isotopes.     

The decay of83gSe and83mSe

The decay of the isomeric pair^83gSe (T1/2=22.6 min,I ^α = 9/2⁺) and^83mSe (T1/2=70 s,I ^α = 1/2^?) has been reinvestigated using straight Ge(Li) (^83gSe and^83mSe) and Ge(Li)-Ge(Li) coincidence spectrometry (^83gSe). Both decays populate entirely different⁸³Br levels, 11 of them being previously unreported. Fromγ-ray unbalances and from the known isomeric cross-section ratio of⁸²Se, β^?-branchings have been obtained, including a 34% branching of^83mSe to the ground state of⁸³Br. Logft-values are deduced, spin and parity values proposed and discussed.     

On the decay of73Ga to levels in73Ge

Theγ-radiation following the β^? decay of⁷³Ga has been studied. Singlesγ andγγ coincidence spectra were recorded with Ge(Li)-detectors. 17γ-rays were assigned to transitions in⁷³Ge, where 11 excited levels are proposed. From logft values based onγ-transition intensities, spin and parity assignments for the levels were deduced. The half-life of⁷³Ga was measured to (4.86±0.03) h. From allowedβ-transitions the ground state of⁷³Ga was assigned 3/2^?.     

Radioactive decay of 1.7-h149Nd to levels of transitional149Pm

Sources of¹⁴⁹Nd were produced by thermal-neutron irradiation of enriched¹⁴⁸Nd. High resolution Ge(Li) spectrometers were used to collect gamma-ray singles and coincidence spectra in the study of the decay of 1.7-h¹⁴⁹Nd. A total of 214 gamma rays have been assigned to the decay of¹⁴⁹Nd, and 201 of these transitions have been placed in a level scheme of¹⁴⁹Pm involving 42 excited states. Absolute values for the beta-group intensities were determined for transitions to the¹⁴⁹Pm levels, and spin and parity assignments were made for many of the observed states. The experimentally determined level structure of¹⁴⁹Pm was compared with corresponding levels in other odd-mass Pm and Eu nuclides. Interpretations were made in terms of the core-coupling model. Radioactive decay¹⁴⁸Nd(n, γ)¹⁴⁹Nd; measuredE _γ,I _γ,γ-γ coinc.¹⁴⁹Pm deduced levels,J,π. Compton-suppression. Ge(Li) detector. Enriched targets.     

Low-lying excited states of106Ag studied with the103Rh (α,nγ)106Ag and104Pd (α,pnγ)106Ag Reactions

The level scheme of¹⁰⁶Ag has been studied using the¹⁰³Rh(α,nγ)¹⁰⁶Ag and¹⁰⁴Pd(α,pnγ)¹⁰⁶Ag Reactions. The experimental information is taken fromγ-ray coincidence data using Ge(Li)-Ge(Li) and HPGe-planar Ge(Li) configurations andγ-ray angular distributions. With these measurements 126 γ rays have been assigned to¹⁰⁶Ag with 116 deexciting 78 states below 2.26 MeV in excitation. The location of the 8.4-day 6⁺ isomer is established at 89.63±0.09 keV. Many of the low-lying states are interpreted in terms of a slightly deformed rotor model.