Molecular structure of nuclei

Cluster structures of nuclei are discussed, with emphasis on nuclear clustering in unstable nuclei. The subjects we discuss are alpha condensed states, clustering in Be and B isotopes, and clustering in ³²Mg and ³⁰Ne. The subject of alpha cluster condensation comes from the clustering nature of dilute nuclear matter. We discuss that recent heavy-ion central collision experiments give us nice evidence of the clustering in dilute nuclear matter. We then present a new prediction of the existence of the “alpha cluster condensed states” in the self-conjugate 4n nuclei around the breakup threshold energy into n alpha-particles. As for the clustering in neutron-rich Be, we discuss the comparison between the antisymmetrized molecular-dynamics results and the recent experimental data, which shows that the clustering feature manifests itself very clearly in neutron-rich Be isotopes both in the ground and excited states. Clustering in Be isotopes near neutron dripline is intimately related to the breaking of the neutron magic number N = 8. We report our recent study about the possible relationship between the clustering and the breaking of the neutron magic number N = 20 in ³²Mg and ³⁰Ne. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: horiuchi@ruby.scphys.kyoto-u.ac.jp     

Reactions with fast radioactive beams of neutron-rich nuclei

The neutron dripline has presently been reached only for the lightest nuclei up to the element oxygen. In this region of light neutron-rich nuclei, scattering experiments are feasible even for dripline nuclei by utilizing high-energy secondary beams produced by fragmentation. In the present article, reactions of high-energy radioactive beams will be exemplified using recent experimental results mainly derived from measurements of breakup reactions performed at the LAND and FRS facilities at GSI and at the S800 spectrometer at the NSCL. Nuclear and electromagnetically induced reactions allow probing different aspects of nuclear structure at the limits of stability related to the neutron-proton asymmetry and the weak binding close to the dripline. Properties of the valence-neutron wave functions are studied in the one-neutron knockout reaction, revealing the changes of shell structure when going from the beta-stability line to more asymmetric loosely bound neutron-rich systems. The vanishing of the N = 8 shell gap for neutron-rich systems like ¹¹Li and ¹²Be, or the new closed N = 14, 16 shells for the oxygen isotopes are examples. The continuum of weakly bound nuclei and halo states can be studied by inelastic scattering. The dipole response, for instance, is found to change dramatically when going away from the valley of stability. A redistribution of the dipole strength towards lower excitation energies is observed for neutron-rich nuclei, which partly might be due to a new collective excitation mode related to the neutron-proton asymmetry. Halo nuclei, in particular, show strong dipole transitions to the continuum at the threshold, being directly related to the ground-state properties of the projectile. Finally, an outlook on future experimental prospects is given.     

Clustering in neutron-rich nuclei

Clustering in nuclei is discussed putting emphasis on the investigation of the role of nuclear clustering in neutron-rich nuclei. The subjects we discuss include clustering in neutron-rich Be, B and C isotopes, clustering in the island of inversion around N = 20, and clustering in the region with A ≈ 40. Be isotopes present us typical examples of clustering in neutron-rich nuclei not only in their ground band states but also in their excited band states, for which we show the analyses based on antisymmetrized molecular dynamics (AMD). Clustering in Be isotopes near neutron dripline is intimately related to the breaking of the neutron magic number N = 8. In this connection we report our study about the possible relation of the clustering with the breaking of the neutron magic number N = 20 in the island of inversion including ³²Mg and ³⁰Ne. Our discussion is not only about the positive parity states but also about negative parity states. Recently in the latter half of sd shell and in the pf shell many excited rotational bands with large deformation have been found to exist. Since the first excited K ^π = 0⁺ and K ^π = 0^- bands in ⁴⁰Ca have been regarded as constituting inversion doublet bands having the ³⁶Ar + α structure, and since the first excited K ^π = 0^- band in ⁴⁴Ti has been concluded to have ⁴⁰Ca + α structure through the α transfer reaction and by using the unique α optical potential on ⁴⁰Ca, it is important to investigate the role of α clustering in these newly-found rotational bands with large deformation. We will report the AMD study about this problem.     

Cluster structures in light nuclei

Clustering in light stable and unstable nuclei is discussed. After a brief review of the clustering in stable nuclei, we make a new prediction of the existence of the alpha cluster condensed states in ¹²C and ¹⁶O. Discussions of clustering in light unstable nuclei are made in the cases of Be and B isotopes up to the neutron dripline. Received: 1 May 2001 / Accepted: 4 December 2001     

Triton-emission cross sections with 30 MeV d(Be) break-up neutrons

Triton-emission cross sections were measured for Al, Ti, V, Cr, Mn, Fe, Co, Ni, Cu, Nb, Mo, Ag, Ta, Tl, Pb and Bi with a 30 MeV d(Be) break-up neutron spectrum characterized by a multiple-foil activation technique. The accumulated tritium was separated by vacuum extraction and measured by low-level gas-phase β^? counting. The systematic trend in the cross sections is somewhat similar to that in the 53 MeV d(Be) break-up neutron spectrum; apart from some initial decrease as a function of Z, the cross section is almost constant over the entire range of Z = 22 to 83. The magnitudes of the cross sections lie between those with 14 MeV neutrons and 53 MeV d(Be) break-up neutrons. Hauser-Feshbach calculations show that the statistical model describes the triton-emission cross sections for nuclei in the (2s, ld) shell within a factor of 2; for the heavier nuclei, however, the calculated cross sections are much smaller than the experimental values.     

Rearrangements in neutron shell closures far from stability

A survey of experimental results obtained at GANIL (Caen, Prance) on the study of the properties of very neutron-rich nuclei (Z = 6–20, A = 20–60) near the neutron drip line and resulting in an appearance of further evidence for the new magic number N = 16 is presented. Very recent data on mass measurements of neutron-rich nuclei at GANIL and some characteristics of binding energies in this region are discussed. Nuclear binding energies are very sensitive to the existence of nuclear shells and together with the measurements of instability of doubly magic nuclei ¹⁰He and ²⁸0 they provide information on changes in neutron shell closures of very neutron-rich isotopes. The behaviour of the two-neutron separation energies S_2n derived from mass measurements gives a very clear evidence for the existence of the new shell closure N = 16 for Z = 9 and 10 appearing between 2s_1/2 and ld_3/2 orbitals. This fact, strongly supported by the instability of C, N and O isotopes with N > 16, confirms the magic character of N = 16 for the region from carbon up to neon while the shell closure at N = 20 tends to disappear for Z ≤ 13. Decay studies of these hardly accessible short-lived neutron-rich nuclei from oxygen to silicon using the in-beam γ-ray spectroscopy are also reported.     

Nuclear structure near the drip line studied by RNB

The use of radioactive nuclear beams (RNB) has provided an opportunity to study nuclei far from the stability line. Reaction studies using intermediate and high-energy (30–1000 AMeV) radioactive beams have revealed new structures of nuclei that are not seen in nuclei near to the stability line [1]. One such new structure is the neutron halo, a long low-density tail of the neutron distribution [2]. It has been observed in neutron drip-line nuclei, such as⁶He,¹¹Li and¹¹Be. The neutron halo has put light on many new structure problems. Among those, recent studies of a softE1 mode, a low-frequency oscillation of halo neutrons against the core, are discussed in the following section in connection with a recent (p, p′) reaction measurement [3]. Also, the effect of changes in single-particle orbitals on halo formation is discussed [4]. Another new finding is the formation of neutron skins in neutron-rich unstable nuclei [5]. The relation between the equation-of-state (EOS) of asymmetric nuclear matter and the neutron-skin thickness as well as the density distribution of nuclei far from the stability line is discussed in the last section.     

β-delayed neutron decay of drip line nuclei 11Li and 14Be

Experimental studies of β-decay measurements of the neutron drip line nuclei ¹¹Li and ¹⁴Be are presented. β- decay schemes of these nuclei are determined by measuring β-rays, delayed neutrons and γ-rays in triple coincidence. The decay schemes of both ¹¹Li and ¹⁴Be associated with single neutron emission are unambiguously determined. New levels in their daughter nuclei, ¹¹Be and ¹⁴B, are found. In addition, the deduced level scheme of 14B indicates the lowering of 2s _1/2 single neutron orbital with respect to 1p _1/2 orbital in the N=9 isotones. Such behavior is known to exist in N=7.     

Pionic 3d → 2p X-ray measurements in 50,52,54Cr, 45Sc, 51V, 55Mn and Fe

We report the measurement of the strong interaction shifts and widths of the pionic 3d → 2p transitions in separated isotopes of ^50,52,54Cr and natural Sc, V, Mn, and Fe. Using these new data in combination with earlier low-Z pionic data (6 ? Z ? 20) we have studied the phenomenological pion-nuclear potential. Employing nuclear structure information from measured charge densities and Hartree-Fock calculations, we have fitted the pion-nuclear potential parameters to the pionic-atom data. We have explored the sensitivity of these data to the value of the Lorentz-Lorenz parameter ξ. The addition of an isovector dependence to the s- and p-wave two-nucleon terms is shown to be unnecessary at the present level of experimental accuracy. We have used the deduced optical potentials to determine the neutron radii of the nuclei 20 ? Z ? 26 and find reasonable agreement with Hartree-Fock predictions and with the results of other hadronic probes for 20 ? Z ? 23 but poor agreement for 24 ? Z ? 26.     

Neutron halos in hypernuclei

Properties of single- Λ and double- Λ hypernuclei for even-N Ca isotopes ranging from the proton dripline to the neutron dripline are studied using the relativistic continuum Hartree-Bogoliubov theory with a zero-range pairing interaction. Compared with ordinary nuclei, the addition of one or two Λ-hyperons lowers the Fermi level. The predicted neutron dripline nuclei are, respectively, ⁷⁵ _ΛCa and ⁷⁶ _2ΛCa, as the additional attractive force provided by the Λ-N interaction shifts nuclei from outside to inside the dripline. Therefore, the last bound hypernuclei have two more neutrons than the corresponding ordinary nuclei. Based on the analysis of two-neutron separation energies, neutron single-particle energy levels, the contribution of continuum and nucleon density distribution, giant halo phenomena due to the pairing correlation, and the contribution from the continuum are suggested to exist in Ca hypernuclei similar to those that appear in ordinary Ca isotopes. Received: 21 October 2002 / Accepted: 11 January 2003 / Published online: 8 April 2003     

Atomic masses above146Gd derived from a shell model analysis of high spin states

From a shell model analysis of high-spin states in neutron deficient nuclei above¹⁴⁶Gd we have derived the ground state masses of theN=82 and 83 isotones of Eu, Tb, Dy, Ho, and Er. The results can be used to calculate the energies of aligned multiparticle yrast configurations. They also link ten α-decay chains to the nuclei with known masses, providing many new absolute mass values which are compared with predictions. An examination of the two-proton separation energies atN=82 shows an 0.5 MeV break in the nuclear mass surface atZ=64.     

β delayed emission of a proton by a one-neutron halo nucleus

Some one-neutron halo nuclei can emit a proton in a β decay of the halo neutron. The branching ratio towards this rare decay mode is calculated within a two-body potential model of the initial core + neutron bound state and final core + proton scattering states. The decay probability per second is evaluated for the ¹¹Be, ¹⁹C and ³¹Ne one-neutron halo nuclei. It is very sensitive to the neutron separation energy.     

Core-breakup reactions of the halo nuclei 11Be and 11Li: momentum distributions and shadow effects

The halo nuclei ¹¹Be and ¹¹Li have been studied in core-breakup reactions where the halo neutrons are expected to be released without a major distortion due to the reaction. The widths of the halo-neutron momentum distributions have been extracted in coincidence with He fragments, Γ = 32 ± 4 MeV/c, and Li fragments, Γ = 42 ± 4 MeV/c for ¹¹Be and with He fragments, Γ = 42 ± 6 MeV/c for ¹¹Li. The ¹¹Be breakup gives a very low neutron multiplicity of 0.38±0.09 which is a manifestation of the shadowing of the neutron in the core-breakup reaction. This value can be understood from a simple theoretical calculation, which also accounts for the observed transverse momentum widths at small angles.     

Topology of “white stars” in the relativistic fragmentation of light nuclei

Experimental observations of the multifragmentation of relativistic light nuclei by means of emulsions are surveyed. Events that belong to the type of “white stars” and in which the dissociation of relativistic nuclei is not accompanied by the production of mesons and target-nucleus fragments are considered. An almost complete suppression of the binary splitting of nuclei to fragments of charge in excess of two, Z > 2, is a feature peculiar to charge topology in the dissociation of Ne, Mg, Si, and S nuclei. An increase in the degree of nuclear fragmentation manifests itself in the growth of the multiplicity of singly and doubly charged fragments (Z = 1, 2) as the charge of the unexcited fragmenting-nucleus part (which is the main part) decreases. Features of the production of systems formed by extremely light nuclei α, d, and t are studied in the dissociation of the stable isotopes of Li, Be, B, C, N, and O to charged fragments. Manifestations of ³He clustering can be observed in “white stars” in the dissociation of neutron-deficient isotopes of Be, B, C, and N.     

Gas-cell-based setup for the production and study of neutron rich heavy nuclei

The present limits of the upper part of the nuclear map are very close to stability while the unexplored area of heavy neutron-rich nuclides along the neutron closed shell N = 126 is extremely important for nuclear astrophysics investigations and, in particular, for the understanding of the r-process of astrophysical nucleosynthesis. This area of the nuclear map can be reached neither in fusion–fission reactions nor in fragmentation processes widely used nowadays for the production of exotic nuclei. A new way was recently proposed for the production of these nuclei via low-energy multi-nucleon transfer reactions. The estimated yields of neutron-rich nuclei are found to be significantly high in such reactions and several tens of new nuclides can be produced, for example, in the near-barrier collision of ¹³⁶Xe with ²⁰⁸Pb. A new setup is proposed to produce and study heavy neutron-rich nuclei located along the neutron closed shell N = 126.     

New neutron magic number <Emphasis Type="Italic">N</Emphasis> = 16 for neutron-rich nuclei

A survey of experimental results obtained at GANIL (Caen, France) on the study of the properties of very neutron-rich nuclei (Z=6–20, A=20–60) near the neutron drip line and resulting in an appearance of further evidence for the new magic number N=16 is presented. Very recent data on mass measurements of neutron-rich nuclei at GANIL and some characteristics of binding energies in this region are discussed. Nuclear binding energies are very sensitive to the existence of nuclear shells, and together with the measurements of instability of doubly magic nuclei ¹⁰He and ²⁸O, they provide information on changes in neutron shell closures of very neutron-rich isotopes. The behavior of the two-neutron separation energies S_2n derived from mass measurements gives very clear evidence for the existence of the new shell closure N=16 for Z=9 and 10 appearing between the 2s_1/2 and 1d_3/2 orbitals. This fact, strongly supported by the instability of C, N, and O isotopes with N>16, confirms the magic character of N=16 for the region from carbon up to neon, while the shell closure at N=20 tends to disappear for Z≤13. Decay studies of these hardly accessible short-lived neutron-rich nuclei from oxygen to silicon using in-beam γ-ray spectroscopy are also reported.     

Fusion-fission of heavy and superheavy nuclei

The process of fusion-fission of heavy and superheavy nuclei (SHE) with Z=82–122 formed in the reactions with ⁴⁸Ca and ⁵⁸Fe ions at energies near and below the Coulomb barrier has been studied. The experiments were carried out at the U-400 accelerator of the Flerov Laboratory of Nuclear Reactions (JINR) and at the XTU Tandem accelerator of the National Laboratory of Legnaro (LNL) using the time-of-flight spectrometer of fission fragments CORSET and the neutron multidetector DEMON. As a result of the experiments, mass and energy distributions (MED) of fission fragments; fission, quasifission, and evaporation residue cross sections; and multiplicities of neutrons and γ-quanta and their dependences on the mechanism of formation and decay of compound systems have been studied.     

Shell effects in fusion-fission of heavy and superheavy nuclei

The process of fusion-fission of heavy and superheavy nuclei (SHE) with Z=82?122 formed in the reactions with ⁴⁸Ca and ⁵⁸Fe ions at energies near and below the Coulomb barrier has been studied. The experiments were carried out at the U-400 accelerator of the Flerov Laboratory of Nuclear Reactions (JINR) and at the XTU Tandem accelerator of the National Laboratory of Legnaro (LNL) using the time-of-flight spectrometer of fission fragments CORSET and the neutron multi-detector DEMON. As a result of the experiments, mass and energy distributions (MED) of fission fragments, fission, quasi-fission and evaporation residues cross sections, multiplicities of neutrons and γ quanta and their dependence on the mechanism of formation and decay of compound systems have been studied.     

Research program for the radioactive beams of the ACCULINNA-2 separator

The ACCULINNA-2 separator is intended to provide beams of exotic nuclei with Z = 1?30, energies of 10?C50 MeV/amu, and intensities that allow one to study excitation spectra and decay dynamics of neutron- and proton-drip nuclei. Examples from studies of the ¹⁰He and ⁶Be nuclei are presented.     

Investigation of the neutron shell structure of the even-even isotopes <Superscript>40–56</Superscript>Ca within the dispersive optical model

Within the method of matching experimental data obtained in the neutron-stripping and neutron-pickup reactions on ^{40,42,44,46,48}Ca isotopes, the single-particle energies and probabilities that neutron states are filled are obtained for the even-even calcium isotopes. These data are analyzed within the dispersive optical model, and good agreement between the calculated and experimental values of the energies of states is obtained. The dispersive optical potential is extrapolated to the region of the unstable ^50,52,54,56Ca nuclei. The calculated single-particle energies of bound states in these isotopes are compared with the results of the calculations within the multiparticle shell model, the latter predicting a new magic number N = 34 for Z = 20 nuclei.