Multiple Coulomb excitation of198Hg and200Hg

Multiple Coulomb excitation measurements on^{198, 200}Hg have been performed with 5MeV/amu²⁰⁸Pb projectiles andB(E2)-values are determined for transitions between states up to spin 8⁺. In¹⁹⁸Hg a reduction of theB(E2)-value for the yrast transition 8⁺→6⁺ by a factor of 3 as compared to the rigid rotor prediction is observed, which supports the earlier proposed idea that the ground state band is crossed between the 6⁺ and 8⁺ state by a weakly interactingvi ₁₃ ^2/2 rotation aligned band. In each of the two nuclei,¹⁹⁸Hg and²⁰⁰Hg, a state with a possibleI ^π=8⁺ assignment is observed, which is tentatively interpreted as the 8⁺ member of the ground state band.     

Rotational band crossings in the actinides

In the actinides bothi _13/2 protons andj _15/2 neutrons are close to the Fermi surface. At rapid rotation these high-j particles will unpair and align their orbital angular momentum along the axis of rotation giving rise tos-bands that cross the ground-state band. Coulomb excitation of the odd nuclei ₂₃₇ ⁹³ Np (established up to the 45/2⁺ state) and ₂₃₅ ⁹² U (established up to the 51/2^? state) provides specific information about these band crossings: From the saturating alignment of the odd high-j particle in both nuclei at intermediate rotational frequencies we find the aligned angular momentum of thei _13/2 protons-band to be 6.6? while the corresponding value for thej _15/2 neutrons-band is 5.5?. At more rapid rotation above ?ω=0.18 MeV we observe additional alignment in²³⁵U. This is ascribed to the interaction of the protons-band. From the gradual onset of the additional alignment we deduce that forZ=92 the protons-band interacts strongly with the ground-state band and from a comparison of the actual amount of alignment with the full value of 6.6? we estimate the crossing to occur around ?gw _c ^p =0.25 MeV.     

Evidence for a 3.6 minute isomeric 12− state of the πh 11 2/−1 vi 13 2/−1 configuration in206Tl and effective two-particle interactions

Using the²⁰⁴Hg(α, pn)-reaction andα-particles of energies 39–55 MeV, we have found an isomeric 3.6 min 12^? state in²⁰⁶Tl at 2,642.9 keV which has the two-hole configurationπh ₁₁ ^2/?1 vi ₁₃ ^2/?1 The 12^? state decays mainly by anE5 transition of energy 1,021.4 keV to a 7⁺ state at 1,621.5 keV whose main configuration isπs ₁ ^2/?1 vi ₁₃ ^2/?1 There is, in addition, evidence for a weak 565 keVM 4 branch to an 8⁺ state at 2,078 keV whose main configuration should beπh ₁₁ ^2/?1 vf ₅ ^2/?1 . The 7⁺ state decays by a stretched cascade ofγ-rays to states of the following values ofJ ^π and excitation energy: 5 _? ⁺ , 1,405.4 keV; 4^?, 952.1 keV; 2^?, 265.8 keV and 0^?, 0 keV. The main configurations of these states areπh ₁₁ ^2/?1 vp ₁ ^2/?1 ,πd ₃ ^2/?1 vf ₅ ^2/?1 ,πd ₃ ^2/?1 vp ₁ ^2/?1 andπs ₁ ^2/?1 vp ₁ ^2/?1 respectively. From the nuclear masses of²⁰⁸Pb,²⁰⁷Pb,²⁰⁷Tl, and²⁰⁶Tl and the experimental excitation energies it is possible to obtain the proton hole-neutron hole interaction in²⁰⁶Tl. This interaction is compared with the calculations of Kuo and Herling and the discrepancies are discussed. The 12^?→8⁺ M4 transition rate is reduced because of destructive interference between the protonh _11/2→d _3/2 and the neutroni _13/2→f _5/2 contributions. The magnitude of the reduction is accurately reproduced by the wave functions of Kuo and Herling. The 12^?→7⁺ E5 transition rate is about twice as large as the single-holeπh ₁₁ ^2/?1 πs ₁ ^2/?1 transition rate. This deviation is fully explained by the configuration admixtures in the 7⁺ state, given by Kuo and Herling.     

The 235 ns 9+ isomer in 63 148 Eu85

From (p, xn) in-beamγ-ray and electron measurements aT _1/2=235(14) ns isomer at 720 keV was identified in ₆₃ ¹⁴⁸ Eu₈₅ and the levels populated in its decay have been characterized. The results determineI ^π=9⁺ for the isomeric state, and we assign it as the (πh _11/2 j ₀ ^?2 ν f ₇ ^2/3 )9⁺ shell model state, analogous to the configuration of the 235 μs isomer in ₆₃ ¹⁴⁶ Eu₈₃.     

A coupled-channel treatment of Cabibbo-angle favoured (D,D s + )→VP decays

We have performed a two-channel calculation of Cabibbo-angle favoured decays,D _s ⁺ →VP. We find a satisfactory fit toS _s ⁺ →φπ ⁺,ρ ⁰ π ⁺ andK ⁺ \(\bar K^{ * 0} \) data from ARGUS and E-691. We have also studied Cabbibo-angle favouredD→VP decays in a coupled channel formalism. We coupleD→K ^*π,K _? and \(\bar K^0 \phi \) channels inI=1/2 state, andK ^*π andK _? channels inI=3/2 state. We leave the two channels, \(\bar K^0 \omega \) and \(\bar K^{ * 0} \eta \) out of our unitarization scheme. Particular attention is paid to the role of the weak annihilation term in these decays.     

Gyromagnetic ratios of 4+ and 6+ states in156Gd and158Gd

The followingg-factors have been derived from time integral measurements of γ-γ angular correlations in the static magnetic hyperfine field of magnetized gadolinium metal probes:¹⁵⁶Gd:g(4 ₁ ⁺ )=+0.310(19)g(6 ₁ ⁺ )=+0.25(21)g(4 ₃ ⁺ , 1511 keV)=+0.809(27)¹⁵⁸Gd:g(4 ₁ ⁺ )=+0.409(15). The 5.35d ¹⁵⁶Tb sources were produced by the reaction¹⁵⁶Gd(d, 2n)¹⁵⁶Tb in our cyclotron. A carrier-free 150y ¹⁵⁸Tb source was obtained from ISOLDE/CERN. In comparison with the precisely knowng-factors of the 2 ₁ ⁺ states,g(2 ₁ ^su+ ,¹⁵⁶Gd) =+0.386(4) andg(2 ₁ ⁺ ,¹⁵⁸Gd)=0.381(4), we observe a large reduction for the¹⁵⁶Gd 4 ₁ ⁺ state whereasg increases slightly for¹⁵⁸Gd. The half-life of the 4 ₁ ⁺ state of¹⁵⁸Gd was remeasured as¹⁵⁸Gd:T _1/2(4 ₁ ⁺ )=148(2) ps. A measurement of the rotation in the 4 ₃ ⁺ state of¹⁵⁶Gd in external magnetic fields of various strengths up toB _ext=9.5 T did not confirm the anomalous dependence of the magnetic hyperfine field in gadolinium metal on the external field, which has been reported by Persson et al. [29].     

On the yrast levels in204Pb

High-spin states in²⁰⁴Pb were populated in the²⁰⁴Hg(α,4n) reaction using α-particles in the energy region 42–51 MeV. Prompt and delayedγ-rays as well as conversion electrons were studied in addition to excitation functions, angular distributions andγ-γ coincidences. In this way a stretched cascade ofγ-rays from a level at 8125.9 keV was found to feed the previously known isomeric 9^? level at 2185.7 keV. Spins and parities were established for levels up to and including a 19^? level at 6098.0 keV. The levels with c= 17^2212; and 19^? at excitation energies of 5664.3 and 6098.0 keV are likely to be due to the simplep ₁ ^2/s-1 i ₁₃ ^2/?3 andf ₅ ^2/?1 i ₁₃ ^2/?3 configurations. The agreement between calculated and experimental energies for all observed levels in the regionJ=9–19 is very good in cases where the empirical two-particle interactions used are satisfactorily well known. Above the 19^? level there are three weakly populated levels at 7402.1, 7849.2 and 8125.9 keV, which are likely to haveJ≥20. None of these energies agrees with the calculated value 7695±20 keV for the 20⁺ state of thei ₁₃ ^2/?4 configuration which has the highest angular momentum produced by the four valence neutron holes. This apparent anomaly can be understood if the yrast levels withJ≥20 have angular momentum contribution from the core. It seems likely that the states at 7402.1, 7849.2 and 8125.9 keV are due to proton core excited states of the typeπh _9/2 h ₁₁ ^2/?1 ×νp ₁ ^2/?2 i ₁₃ ^2/?2 withJ ^π=20⁺ andJ ^π=21⁺ andπh _9/2 h ₁₁ ^2/?1 ×νp ₁ ^2/?1 f ₅ ^2?1 i ₁₃ ^2/?2 withJ ^π=22⁺ or 23⁺, respectively. The state at 8126 keV has the highest energy so far directly observed in a stretched cascade ofγ-rays from the decay of a heavy nucleus produced in (α, xn) reactions.     

Excitation of bands of the first negative system of the N 2 + ion in collisions of N+ and O+ ions with N2 molecules

Absolute values of the excitation cross sections of the (0,0) bands [for O⁺(⁴ S), O⁺(² P)-N₂ pairs] and the (0,0), (0,1), (1,2), and (2,3) bands [for N⁺(³ P)-N₂ pairs] of the first negative system of the N ₂ ⁺ ion have been measured in collisions with nitrogen molecules of nitrogen and oxygen ions in the ground state and in a metastable state in the interval of ion energies 1–10 keV. The process of excitation of the (0,0) band of the first negative system of the N ₂ ⁺ ion by oxygen ions in the metastable ² P state is of a quasi-resonant character. The presence in the beam of ions in metastable states was monitored by measuring the excitation efficiency of the (0,0) band λ3914 Å of the N ₂ ⁺ ion in different operating regimes of the highfrequency ion source. For N⁺ ions in the ³ P ground state, as the collision frequency is decreased the relative vibrational population of the v′=1 and v′=2 levels of the B ²Σ _u ⁺ state of the N ₂ ⁺ ion is observed to deviate strongly from the value calculated in the Franck-Condon model.     

An ESR study of NH 3 + , al center and HO2 · radical in alkali feldspars

Paramagnetic centers of NH ₃ ⁺ , Al, and HO₂ · have been observed in alkali feldspars from Aichi prefecture, Japan. The quartet signal has been tentatively ascribed to NH ₃ ⁺ rather than to ·CH₃, although the hyperfine splitting by¹⁴N (I=1) was not observed. The averageg- andA-valuesg _av=2.0033 andA _av ^H =2.45 mT, respectively, were attributed to hydrogen. The powder spectra of Al centers stable up to 400 K were simulated by the anisotropicg factors ofg _zz =2.060,g _xx =2.0014,g _yy=2.0021 andA=0.9 mT. Newly discovered HO₂ · is stable up to 570 K. The intensities of the spectra from NH ₃ ⁺ and Al centers were enhanced by gamma-ray irradiation, while that of HO₂ · was not enhanced. Production efficiency,G-value (radical/100 eV) of NH ₃ ⁺ has been obtained to beG=0.01. These results suggest that ESR dating of feldspars is possible.     

Pion photoproduction on197Au to ground and isomeric states in197Hg

The lifetime of the 331.3 keV 0 ₂ ⁺ state in¹⁰⁰Zr has been measured at the gas-filled recoil separator for fission products JOSEF. By observing the delayed coincidences between theβ-particles populating the level and theE0 conversion electrons from its decay into the ground state, a half-life of 3.37±0.30 ns has been obtained. From the measured lifetime and the relative intensities of the 0 ₂ ⁺ →0 ₁ ⁺ and 0 ₂ ⁺ →2 ₁ ⁺ transitions, values of 0.493±0.015 for theE0 strength parameterρ, and of 16 single particle units forB(E2,2 ₁ ⁺ → 0 ₂ ⁺ ) have been deduced. The enhanced nature of theE0 transitions suggests mixing of the 0 ₁ ⁺ and 0 ₂ ⁺ states which may be estimated by comparing the experimentalB(E2) values for the 2 ₁ ⁺ →0 ₁ ⁺ and 2 ₁ ⁺ →0 ₂ ⁺ transitions with the predictions of the asymmetric VMI model.     

g-factor of the second 4+ state in24Mg

The transient field technique has been used to determine theg-factor of the 4 ₂ ⁺ state at 6.010MeV excitation in²⁴Mg. The deduced value ofg=+0.5(4) is consistent with collective model expectations. Further, the equality within experimental accuracies, of the g-factors of the 2 ₁ ⁺ , 2 ₂ ⁺ , 4 ₁ ⁺ and 4 ₂ ⁺ states agrees with theoretical predictions for thisT=0 self-conjugate nucleus, in contrast to the results for²⁰Ne.     

In-beam study of the doubly-odd nucleus 61 140 Pm79 above the 8− β +-decaying isomer

An in-beamγ-ray study performed with the¹¹⁴Cd(³⁰Si,p 3n) reaction has established the structure of theN=79 nucleus¹⁴⁰Pm. States up toI=(20)? and 5.5 MeV excitation energy have been recognized above the 5.95 m isomeric state which we identify, from the GT decay to¹⁴⁰Nd, as the 8^? member of the (πd ₅ ^2/?1 vh ₁₁ ^2/?1 ) multiplet, changing the present 7^? assignment. The low energy part of the level scheme is discussed in terms of the coupling of the valence holes in respect to theZ=64,N=82 shell closure. A new 8⁺ isomeric state witht _1/2=1 _?0.5 ⁺¹ ns has been observed, having most likely a (πh _11/2 vh _11/2 ^-1 )₈ configuration.     

E2 andE3 transition strengths in some rare-earth nuclei

Coulomb excitation byα-particles of vibrational-like states in even-mass rare-earth nuclei is used to determine the reduced transition probabilitiesB(E2; 0 _gs ⁺ →2 _γ ⁺ ),B(E2; 0 _gs ⁺ →2 _β ⁺ ),B(E2; 2 _gs ⁺ →0 _β ⁺ ) andB(E2; 0 _gs ⁺ →3 _oct ^? ) in¹⁵⁰Nd,^{152, 154}Sm,^{154, 158}Gd,¹⁶⁴Dy and¹⁶⁶Er. TheB(Eλ; 0 _gs ⁺ →I=λ)-values range from 2.4 to 6.5 single-particle units for transitions to the 2 _γ ⁺ -states, 0.8 single-particle units for the 2 _β ⁺ -states and from 14.1 to 21.7 single-particle units for the 3^?-states.     

Microscopic foundation of the interacting boson model in thes d-shell nuclei

Starting from an isospin invariant shell-model hamiltonian, we describe a method for deriving microscopically the IBM-hamiltonian appropriate to lights d-shell nuclei. The key ingredients of our approach are:a) the Belyaev-Zelevinsky-Marshalek (BZM) bosonization procedure;b) two successive unitary transformations that extract the “maximally decoupled” collective bosons with angular momentaJ=0(s _ππ ⁺ ,s _νν ⁺ ,s _πν ⁺ ) andJ =2(d _ππ ⁺ ,d _νν ⁺ ,d _πν ⁺ (T=0),d _πν ⁺ (T=1)). The method is applied to obtain the low-energy spectra and the electron scattering form factors for the 0 ₁ ⁺ →2 ₁ ⁺ transitions in²⁰Ne and²⁴Mg. Good agreement with the exact shell-model results is achieved. The inclusion of proton-neutron bosons (s _πν ⁺ ,d _πν ⁺ (T=1),d _πν ⁺ (T=0)), as well as the renormalization of boson parameters due to the non-collective degrees of freedom, are shown to play a crucial role.     

Production and loss of N 2 + , Ne+ and Ne 2 + during the decay period of plasmas produced in neon-nitrogen mixtures

Studies of the time dependencies of the number density of N ₂ ⁺ , Ne⁺ and Ne ₂ ⁺ ions have been made during the decay period of plasmas produced in neon containing various concentrations of nitrogen molecules. Reaction rate constants were obtained for N ₂ ⁺ +N₂+Ne→N ₄ ⁺ +Ne((1.2±0.2)×10^?29 cm⁶ sec^?1) and Ne⁺+N₂→N ₂ ⁺ + Ne ((2.9±0.3) × 10^?12 cm³ sec^?1). The ambipolar diffusion coefficient of N ₂ ⁺ in neon was found to beD _a p _o =350±20 cm² sec^?1 Torr.     

Symmetric charge-exchange reactions of N 2 + -ions investigated by laser-induced fluorescence

The symmetric charge-exchange reaction of fast N ₂ ⁺ ions (U _ion=800 eV) has been investigated by the method of laser-induced fluorescence. The distinction between the primary N ₂ ⁺ ion beam and the N ₂ ⁺ ions formed by charge-exchange was possible because of the different velocities of the two species which resulted in two spectral distributions separated by the Doppler-shift. Simulation techniques have been used in order to obtain rotation-vibration distributions for both the inelastically scattered fast ions and the charge-exchange products. The rotation distributions could be described by a temperature of 1,000 K for the inelastic and 300 K for the charge-exchange process. The latter process exhibits, however, a significant vibrational excitation which is attributed to the existence of a stable intermediate complex of N ₄ ⁺ . The preferred geometry for the intermediate collision complex is assumed to be non-planar.     

Electronic color centers in SrF2-Na crystals

It was shown that optical bleaching of M _A ⁺ color centers at 80 K in SrF₂-Na crystals causes the core of an M _A ⁺ -center to transform into the V _a ⁺ Me ⁺ V _a ⁺ configuration, in which all three point defects are arranged diagnonally in the cube cell. Reirradiation of an optically bleached crystal by x-rays generates F _D centers in it: V _a ⁺ Me ⁺ V _a ⁺ + e ^? → V _a ⁰ Me ⁺ V _a ⁺ ≡ F _D. The F _D → M _A ⁺ transformation in SrF₂-Na crystals proceeds at T = 135 K, in contrast to the F _A → M _A ⁺ transformations, which take place at T > 200 K.     

A new many-body solution of the Friedel resonance problem

It is numerically shown that the groundstate of the Friedel problem (consisting of a conduction band and a dresonance), occupied with (n+ 1) electrons, can be written as Ψ = (A a ₀ ^* +Bd*) Π _v=1 ⁿ a _v ^* Φ₀, where a ₀ ^* represents a localized conduction electron state, d* is the Friedel resonance state and Π _v=1 ⁿ a _v ⁸ Φ₀ is a Slater determinant of n single electron states a _t ^* , (Φ₀ is the vacuum state). The a _i ^* together with a ₀ ^* are part of a full ortho-normalized basis of the conductions band.     

Magnetic moments of the 2 1 + states in102, 104Mo

Theg factors of the first excited 2⁺ levels in the neutron-rich nuclei¹⁰²Mo and¹⁰⁴Mo have been studied through the measurement of the perturbed angular correlations for theγ-γ cascades between the 0 ₂ ⁺ -2 ₁ ⁺ -0 ₁ ⁺ level sequences. The results of g=0.42±0.07 for¹⁰²Mo and ofg= _?0.11 ^+0.12 for¹⁰⁴Mo agree with the prediction of the vibrational-rotational model. In terms of IBA, with the assumption ofN _π=3 for the Mo isotopes which takes into consideration a two particle, two-hole excitation across the Z=40 subshell, the proton-bosong factor is deduced to beg _π=1.00±0.23. It is shown that this value provides evidence for subshell effects in¹⁰⁰Zr.