Quadrupole moments of superdeformed bands in 193Tl

Lifetimes of states in the two strongest superdeformed (SD) bands in ¹⁹³Tl were measured using the Doppler-shift attenuation method. The reaction ¹⁷⁶Yb(²³Na,6n)¹⁹³Tl at a beam energy of 129 MeV was used and γ-rays were detected by the Gammasphere array. Quadrupole moments of 18.3(10) eb and 17.4(10) eb were extracted for SD bands 1 and 2, respectively, using the fractional Doppler-shifts of the SD transitions. The previously reported linking transitions of these SD bands to normal deformed near yrast levels could not be confirmed. No other candidates for linking transitions could be established. Received: 27 April 1999     

Pionic degrees of freedom in atomic nuclei and quasielastic knockout of pions by high-energy electrons

The microscopic mechanism of the identical bands in odd-odd nucleus ¹⁹⁴Tl and its neighbor odd-A nuclei ^193,195Tl is investigated using the particle-number-conserving (PNC) method for treating the cranked shell model with monopole and quadrupole pairing interactions. It is found that the blocking effect of the high-j intruder orbital plays an important role in the variation of moments of inertia (J⁽¹⁾ and J⁽²⁾) with rotational frequency for the superdeformed bands and identical bands. The variation of the occupation probability of each cranked orbital and the contributions to moment of inertia from each cranked orbital are presented.     

Nuclear moments and the change in the mean square charge radius of neutron deficient thallium isotopes

The hyperfine structure, isotope and isomeric shifts in the atomic transition 6p ² P _3/2–7s ² S _1/2, =535 nm have been measured for theI=7 andI=2 states of^{190, 192, 194, 196}Tl; theI=1/2 andI=9/2 states of¹⁹¹Tl and the I=7 isomer of¹⁸⁸Tl. The thallium isotopes were prepared as fast atomic beams at the GSI on-line mass separator following fusion reactions and — in some cases — subsequent-decay. The nuclear dipole moments, electric quadrupole moments and the change in the nuclear mean square charge radius are evaluated. Theuu-isotopes show an isomeric shift which changes sign between¹⁹²Tl and¹⁹⁴Tl.Dedicated to P. Armbruster on the occasion of his 60th birthday     

Nuclear structure of 189Tl states studied via \beta^{{+}}_{} /EC decay and laser spectroscopy of 189m+gPb

The /EC decay of ^{189m, g}Pb has been studied at the ISOLDE facility using nuclear spectroscopy and in-source laser spectroscopy. A level scheme of ¹⁸⁹Tl has been built from - coincidence relationships and information on the feeding of some excited levels of ¹⁸⁹Tl provided by the hyperfine spectra obtained from laser ionization. The half-lives of both the 13/2⁺ and 3/2^{- 189}Pb isomers have been estimated to be T _1/2 = 50±3 s and T _1/2 = 39±8 s, respectively. Calculations have been performed for different oblate and prolate nuclear deformations using an axial-rotor coupled to one-quasiparticle model, a structure has been suggested for the low-lying levels of the ¹⁸⁹Tl nucleus.     

The limit of stability of proton-rich thallium isotopes: a search for the decay of177Tl

The fusion reaction⁷⁴Se+¹⁰⁶Cd¹⁸⁰Pb^* at a compound nucleus excitation energy E_x 40 MeV, has been used in a search for the decay of the unknown nucleus¹⁷⁷Tl. Evaporation residues were velocity and mass analysed prior to implantation into a position sensitive silicon surface barrier detector. No evidence was discovered for the proton or alpha-decay of¹⁷⁷Tl for a cross-section > 10 _– ⁵⁺¹⁰ nb. This indicates either that¹⁷⁷Tl decays too rapidly (t_1/2 < 1=">s) by proton emission for the decay to be detected, or that¹⁷⁷Tl is produced with a cross-section less than the limit established in the present experiment. The following nuclear decay half-lives were measured with improved accuracy;¹⁷⁷Hg (t_1/2 = 130±5 ms),¹⁷⁸Hg (t_1/2=250±25 ms) and¹⁷⁷Au (t_1/2=1180±70 ms). The experiment also provided the first direct confirmation of the correct mass assignment of the alpha-decay, E=6.26 MeV, to the decay of¹⁷⁶Au. Two additional halflife measurements of proton-rich Osmium isotopes are also presented from a previous similar experiment;¹⁶⁵Os (t_1/2=73±8 ms) and¹⁶⁶Os (t_1/2 = 194±17 ms).     

Study of superdeformed bands in nuclei withA ∼ 150 by heavy-ion-γ coincidences

Superdeformed (SD) bands in¹⁵²Dy,¹⁵¹Dy and¹⁵¹Tb have been populated via the 5n, 6n and 5np evaporation channels, respectively, with the³³S+¹²⁴Sn reaction at 160 and 170 MeV bombarding energies. Population intensities are in good agreement with existing data for SD bands in^{151, 152}Dy and SD yrast band in¹⁵¹Tb. The excited twin SD band in¹⁵¹Tb with the same-transitions as the band in¹⁵²Dy is populated about 5 times more strongly than by the 6n evaporation channel. This might be explained in terms of competition between proton and emission out of an intermediate, excited superdeformed configuration of¹⁵²Dy.Dedicated to Prof. Dr. P. Kienle on the occasion of his 60th birthday     

High-spin states of odd-odd156Ho

High spin states in the nucleus¹⁵⁶Ho have been studied via the fusion-evaporation reaction¹⁴⁰Ce(¹⁹F,3n)¹⁵⁶Ho at the beam energy of 82 MeV.- coincidences, E, I and excitation functions have been measured. With two rotationally-aligned bands identified as [h_11/2] [i_13/2], we found two new bands with a signature splitting, whose structure is believed to arise from either [h_9/2] or [f_7/2] coupled to [h_11/2]. Our placement of rays belonging to these new bands suggests that the previously known level scheme should be corrected. We also found many new low-energy rays in the low excitation energy. As compared to¹⁵⁴Ho, the present nucleus with two more neutrons becomes more collective, and shows well-observed rotationally-aligned bands with a clear signature splitting.Communicated by B. Herskind     

High spin investigation in 193Pb with EUROGAM 2: coexistence of superdeformed and dipole bands

The nucleus ¹⁹³Pb was populated via the ¹⁶⁸Er(³⁰Si, 5n) reaction at a beam energy of 159 MeV and studied with the EUROGAM II spectrometer. Five new dipole ΔI = 1 cascades have been found. The ¹⁹³Pb dipole bands are discussed in terms of microscopic HF+BCS calculations. The proposed configurations are based on a high-K two-quasiproton excitation coupled to rotation aligned quasineutrons. Parallel to the dipole bands the six superdeformed bands have been discussed in the framework of microscopic mean-field calculations. The bands are interpreted as three pairs of signature partners based on quasineutron excitations. Cross-talk transitions linking two signature partner superdeformed bands have been observed and, for the first time in lead isotopes, a mean B(M1)/B(E2) ratio value of 0.15±0.04 μ _N ² /e^2b2 has been extracted.     

Spectroscopy of alkali atoms and molecules attached to liquid He clusters

Large helium clusters, ranging in size from a few hundred to several thousand atoms, are produced in a nozzle expansion. Combining this source with a pick-up scattering cell in which the clusters can be seeded with chromophores allows us to probe the influence of the helium environment on the atoms and molecules attached to the clusters. Using an alkali as chromophore we recorded laser induced fluorescence spectra of Na atoms and molecules attached to helium clusters. Apart from the spectrum of the Na monomer, we have found spectroscopic bands which can unambiguous be assigned to two bound Na atoms. The first of this bands is due to 1^{1 +} (A) 1¹ _g ⁺ (X) excitations of the covalently bound singlet Na₂ molecule while the second is due to 1³ _g ⁺ 1^{3 +} excitations for the van der Waals bound triplet Na₂ dimer. Both bands have been vibrationally resolved. Furthermore we found very large fluorescence intensities in the region 605–635 nm which are likely due to the excitation of a species containing three Na atoms attached to a helium cluster.     

Experimental investigation of vibrational excitations in230Th

Nuclear levels in²³⁰Th have been investigated in the decay of²³⁰Pa, the²³⁰Th(d, pn) reaction and the²³²Th(p, t) reaction. TheK =0 ₁ ⁺ , 2 ₁ ⁺ , and 2 ₂ ⁺ bands with band heads at 635, 781, and 1010 keV were observed up to the 8⁺, 9⁺, and 7⁺ levels, respectively. A second excited 0⁺ level was identified at 1297 keV which might be interpreted as the usual shape-oscillation. The branching ratios of theE2 transitions from the 0 ₁ ⁺ , 2 ₁ ⁺ , and 2 ₂ ⁺ bands are explained in the framework of the rotational model by taking into account the coupling of these bands with the ground-state band, and the coupling between the 0 ₁ ⁺ and 2 ₁ ⁺ band. A strong enhancement ofE2 transitions from the 2 ₁ ⁺ to the 0 ₁ ⁺ band reported earlier is not confirmed. For the octupole vibrations withK =0^–, 1^–, and 2^– theE1 branching ratios are analyzed in terms of the Coriolis coupling of these bands. An almost complete experimental set ofE1 transition moments from these negative-parity bands to the 0 _g ⁺ , 0 ₁ ⁺ , and 2 ₁ ⁺ bands was obtained. It is suggested that octupole correlations might be important in explaining theseE1 moments.We appreciate the help of Mr. Assmus with the proton irradiations and the financial support of the Kernforschungszentrum Karlsruhe GmbH. This work was supported by the Deutsche Forschungsgemeinschaft (grants Bo 1109/1-1, Gr 894/2-1, Gu 179/3-1 and He 1316/2-3) and by the Volkswagen Stiftung.     

A pair of excited superdeformed bands in196Pb

Two excited superdeformed bands have been found in¹⁹⁶Pb using the GASP-ray spectrometer array. They are signature-partner bands with a small signature splitting developing at higher frequencies, similar to bands 2 and 3 in the isotone¹⁹⁴Hg. The bands are probably built on an excited neutron configuration. They show an unusual incremental alignment of 1/2 with respect to the¹⁹⁴Pb core.Communicated by: B. Herskind     

Superdeformed bands in194Tl

Two superdeformed (SD) bands have been found in¹⁹⁴Tl using the reactions¹⁷⁶Yb(²³Na,5n) and¹⁸¹Ta(¹⁸O,5n). The mass assignments were made from excitation function data. These are the first SD bands found in the mass-190 region that are not in Hg nuclei. The energies of many of the transitions of one of these new SD bands are similar in energy to those in the SD band of¹⁹²Hg.     

The deformedN=60 nucleus 41 101 Nb

The ^– decay of¹⁰¹Zr has been investigated at the fission-product separators JOSEF and LOHENGRIN. The half-life of¹⁰¹Zr has been determined to 2.5(1) s and a level scheme for¹⁰¹Nb has been established from ray singles as well as X/3- and — coincidence measurements. Conversion coefficients for transitions in¹⁰¹Nb and level half-lives between 10 ps and 2 ns have been determined. Three rotational bands are identified among the low-lying levels with band heads at 0 keV, 206 keV and 208 keV. The bands are probably based on the Nilsson configurations [422 5/2⁺], [301 3/2^–] and [303 5/2^–], respectively. The deformation has been determined to _q=0.40(4) and 0.41(8) for the ground state band and the band based on the 206 keV level from the half-lives of the first and second excited members of these bands. This shows that the rapid onset of deformation at N=60 which is typical for the A=100 region of neutron-rich nuclei, takes also place in the Nb isotopes. Nilsson model calculations describe the experimental data well, especially the several determined transition probabilities including those for E1 transitions from the 206 and 208 keV band heads to the ground state.Dedicated to Prof. Dr. P. Armbruster on the occasion of his 60th birthday     

Observation of a πh9/2 ⊗ νi13/2 oblate band in 188Tl

Excited states in ¹⁸⁸Tl have been studied experimentally using the ¹⁵⁷Gd (³⁵Cl, 4n) reaction at a beam energy of 170MeV. A rotational band built on the πh _9/2 ⊗ νi _13/2 configuration with oblate deformation has been established for ¹⁸⁸Tl. Based on the structure systematics of the oblate πh _9/2 ⊗ νi _13/2 bands in the heavier odd-odd Tl nuclei, we have tentatively proposed spin values for the new band in ¹⁸⁸Tl. The πh _9/2 ⊗ νi _13/2 oblate band in ¹⁸⁸Tl shows low-spin signature inversion, and it can be interpreted qualitatively by the two-quasiparticle plus rotor model including a J-dependent p-n residual interaction.     

New combination bands in CCH2 around 0.83 μm recorded using FT-ICLAS

Fourier-transform intracavity laser absorption spectroscopy allowed five ¹²C¹³CH₂ Σ⁺-Σ⁺ bands, all from the ground state, to be identified in the 0.83 μm range. Their rotational analysis was performed and rotational constants are provided. Three of these bands, with origins at 11616.9684(18), 11737.2356(14), and 11761.0322(23) cm⁻¹, have never been reported before. Their upper states are assigned to , respectively.     

Identification and imaging of hot O2 (v″=2, 3, or 4) in hydrogen flames using 193 nm- and 210 nm-range light

Some simple molecules can be excited by light within the tuning ranges of ArF (193–194 nm) and KrF (247.8–248.8 nm) excimer lasers and their fluorescence has been previously used for imaging. Additional wavelength ranges should become available by Raman shifting. As a demonstration, we present excitation and fluorescence spectra from hot O₂ obtained (a) with tunable 193 nm-range light and (b) with that light shifted into the 210 nm range. All measurements are via predissociative upper states. In the 193 nm range, results are compared with those of Andresen's group. In the 210 nm range, the light is tuned to various excitation wavelengths in the (5 3), (8 4), and (7 4) bands of the B–X transition. The (7 4) excitations are well separated and the (7 v) fluoresence spectrum is in accord with Franck-Condon calculations. The wavelengths tend to overlap for the (5 3) and (8 4) excitations and the fluorescence is weaker. State-specific two-dimensional fluorescence images of an H₂-O₂ flame are obtained in both wavelength ranges to illustrate the use of the method.We acknowledge the National Science Foundation and the Donors of the Petroleum Research Fund, administered by the American Chemical Society, for support of this research     

A 3-quasiparticle isomer in neutron-rich <Superscript>183</Superscript>Ta

Excited states in neutron-rich ¹⁸³Ta have been studied using a two-neutron transfer reaction of ¹⁸¹Ta(¹⁸O,¹⁶O) . In-beam -rays were measured in coincidence with scattered ions detected by a high-resolution E -E Si telescope for reaction channel selection. Previously known 1-quasiparticle bands are extended to higher spins, and several levels including a T _1/2 = 0.9(3) μs 3-quasiparticle isomer are identified.     

Energy inversion of thef 7/2 andh 9/2 neutrons in yrast states of154Yb

The N=84 nucleus¹⁵⁴Yb was investigated through the¹⁰⁶Cd(⁵⁴Fe,2p) reaction. We found the 16⁺ yrast level in this nucleus to be formed by the (h_11/2 ² f_7/2h_9/2) configuration, in contrast to the lower-Z isotones where (h_11/2 ² f_7/2 ²)16⁺ is the yrast state. Manybody shell model calculations with empirical two-body interactions support our conclusion.Dedicated to Prof. Dr. O. Schult on the occasion of his 60^th birthday     

Collective structures of the <Superscript>131</Superscript>Cs nucleus

The collective structures of ¹³¹Cs have been investigated by in-beam -ray spectroscopic techniques following the ¹²⁴Sn (^11B , 4n) reaction at a beam energy E_lab = 57MeV. The previously established rotational bands, built on g_7/2, d_5/2 and the unique-parity h_11/2 orbitals, have been extended and evolve into new bands involving rotationally aligned (h_11/2)² and (h_11/2)² quasiparticles. In addition, a new multiquasiparticle band based on the g_7/2 g_7/2 h_11/2 configuration has also been observed. Theoretical interpretations for the assigned configurations are discussed in the framework of Total Routhian Surface (TRS) and Tilted Axis Cranking (TAC) model calculations. TAC model calculations predict a decrease in the B(M1) values with increasing rotational frequency for the g_7/2/d_5/2 (h_11/2)² and h_11/2 (h_11/2)² bands, thus indicating a magnetic rotation character for these bands.