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1.
利用反应显微成像谱仪对70和100keV He2+与He原子碰撞转移电离(TI)过程中不同出射角度的电子能谱进行了测量,观测到出射电子能谱具有如下分布特征:出射电子速度分布介于0和入射离子速度vp之间;在不同出射角度电子能谱分布均有一极大值存在,随着出射角度的增大,能谱分布极大值逐渐减小;当电子出射角度等于45°时,多数电子集中在0eV附近。上述特征可由低能离子-原子碰撞"准分子"模型进行定性解释。在100keV He2+-He转移电离出射电子能谱中有靶电子被俘获至散射离子连续态(electron capture to continuum,简称ECC)电子的贡献,这可看做是动力学两步过程的作用。  相似文献   

2.
利用四体模型计算了100 MeV/amu裸碳碰撞氦原子单电离全微分截面,发现在散射面四体模型和实验结果符合很好,但是在散射平面外与实验数据符合有较大差别. 分析了不同散射振幅对全微分截面的贡献. 结果表明在recoil峰区域附近,由于入射粒子和靶核相互作用的振幅和入射粒子和敲出电子相互作用的振幅之间的干涉所贡献的截面更接近于实验数据,特别是在垂直平面,这两振幅的干涉所形成的截面产生了实验的双峰结构. 然而,总相互作用振幅的干涉并没有呈现这个特征. 四体模型不能给出垂直平面内实验结果的特征是由于三项散射振幅的权重不同.  相似文献   

3.
用3C模型、DS3C模型对1KeV电子入射氦原子(e,2e)反应中的三重微分散射截面进行了计算,并将理论计算结果与实验数据进行了比较,研究了各种屏蔽效应对散射平面内以及垂直平面内三重微分散射截面的影响,并对三重微分散射截面变化规律进行了探讨.结果表明:各种屏蔽效应对散射平面内三重微分散射截面的贡献可以忽略;而在垂直平面内,这些效应对三重微分散射截面结构存在较强影响;另外,末态出射电子与靶核的相互作用直接影响散射平面内和垂直平面内截面的结构及其变化规律.  相似文献   

4.
周丽霞  张燕  燕友果 《物理学报》2017,66(20):203401-203401
采用扭曲波玻恩近似理论计算了共面对称几何条件下类Ne离子2p轨道电子在不同出射电子能量下的(e,2e)反应三重微分截面,出射电子能量分别为3,5,7.5,10,15,20,30和50 eV.计算结果表明,随着出射电子能量的增大和核电荷数Z的增大,三重微分截面的幅度逐渐减小.除Ne以外,对其他离子,在出射电子角度为150?附近出现了一个新的结构,对比不同出射电子能量时的(e,2e)反应三重微分截面,发现这个结构的幅度随着出射电子的能量先增大后减小,文中用一种两次两体碰撞过程对这些现象进行了解释.  相似文献   

5.
在质心参考系中研究了激光场中1 MeV质子对基态氢原子的碰撞电离过程. 靶原子的缀饰波函数由含时间微扰论给出, 末道出射电子态用双中心Coulomb-Volkov波函数描述. 计算表明辐射场使出射电子的双重微分截面变小. 敲出电子的能量越高, 截面减小越明显, 但截面中CTC峰的位置基本不受辐射场的影响.  相似文献   

6.
O5+离子与H原子碰撞时电子俘获概率的计算   总被引:4,自引:0,他引:4       下载免费PDF全文
王利光  王军 《物理学报》2003,52(2):312-315
利用原子轨道作基函数展开系统波函数,附加电子转移因子修正O5+离子和H原子相互作用时的边界条件,计算了初始通道的势能.在得出的理论值与实验值符合很好的情况下,验证了计算参数的可靠性.在碰撞参数b=80a.u.,碰撞速度v=2200a.u.的条件下,利用心核近似方法完成了O5+离子和H原子碰撞过程中8个Σ状态的随时间变化电子俘获概率的理论计算. 关键词: O5+离子 H原子 碰撞 电子俘获  相似文献   

7.
电子原子散射中的S,T,U参数可用来描述散射前后自旋状态的变化,研究精细结构水平上的散射激发振幅之间的关系,进而揭示电子原子碰撞过程中电子自旋-轨道耦合以及电子-电子交换等自旋相关效应.采用扭曲波玻恩近似计算了钠原子受电子散射S→P跃迁中的S,T,U参数,分析了多种入射能(2.2-60 eV)的电子与钠原子激发S→P跃迁过程的S,T,U参数随散射角的分布,其中对10 eV入射能的Sp参数与已报道实验数据符合一致.结果表明,较低能电子入射下的S,T,U参数随散射角的分布幅度和起伏都比较明显,入射能大于40 eV的电子入射,S,T,U参数的散射角分布变化很小.  相似文献   

8.
本文在Coulomb-Volkov近似下,研究了激光场中电子对核的相对论散射.电子出射与入射态分别用Volkov波函数和Coulomb-Volkov波函数来描述.数值计算给出了辐射场修正的散射截面及其对激光强度和频率的依赖关系,并与相应的Born近似结果进行了比较.  相似文献   

9.
牛书通  周旺  潘鹏  朱炳辉  宋涵宇  邵剑雄  陈熙萌 《物理学报》2018,67(17):176102-176102
本文测量了30 keV的He~(2+)入射倾斜角度分别为-0.5~?,-1~?,-1.5~?和-2.5~?的聚碳酸酯纳米微孔膜后,出射粒子角度分布、电荷态分布以及相对穿透率随时间的演化.当微孔膜倾斜角度在-0.5~?,-1~?和-1.5~?时,出射的He~(2+)离子始终保持在入射束流方向,出射的He~0原子出射方向由微孔孔道方向逐渐转移到入射束流方向,在实验过程中观测到明显的电荷交换,这一现象与之前发现的导向效应不同,微孔内部沉积的电荷斑和微孔内表面原子的短程集体散射作用,克服入射离子的横向动量,使入射离子在微孔内表面以上以类似镜面掠射的方式出射,并发生时间演化效应,主要传输机制为电荷斑辅助的表面以上的类似镜面掠射行为.而当倾斜角度在-2.5~?时,出射的He~(2+)离子始终保持在入射束流方向,出射的He~0原子始终保持在微孔孔道方向,沉积的电荷斑很难克服入射离子的横向动量,没有时间演化效应,主要传输机制为微孔内表面以下的多次随机非弹性碰撞过程.这一物理图像使中能离子入射不同倾斜角度的微孔膜物理认识更加深入和完整.  相似文献   

10.
应用经典径迹蒙特卡罗方法研究Si2+离子与氢原子碰撞电离反应过程,计算了随入射离子能量变化的总截面、出射电子随角度和能量变化的一阶、二阶微分截面,及出射电子随入射离子能量变化的平均能量.计算结果展示了软碰撞、电子转移到入射离子连续态、两体相遇碰撞等电离机制.通过计算出射电子到入射离子和靶的距离比的电离电子数分布,研究了不同入射离子能量"鞍点"电离机制的可能性.  相似文献   

11.
ABSTRACT

The reaction dynamics of Penning ionisation of a polycyclic aromatic hydrocarbon (PAH), naphthalene C10H8, in collision with the metastable He*(23S) atom is studied by classical trajectory calculations using an approximate interaction potential energy surface between He* and the molecule, which is constructed based on ab initio calculations for the isovalent Li?+?C10H8 system. The ionisation width (rate) around the molecular surface are obtained from overlap integrals of the He 1s orbital and the molecular orbital. The calculated collision energy dependences of partial Penning ionisation cross sections (CEDPICS) in the range 50–500?meV at 300?K have reproduced the experimental results semi-quantitatively. The opacity functions, which represent the reaction probability with respect to the impact parameter b, are discussed in connection with collision energy, interaction with He* and the exterior electron density of molecular orbitals. They indicate that the collisional ionisations of C10H8 can be classified into three types: π electron ionisations with negative collision energy dependences which are predominantly determined by attractive interaction with He*; σ orbitals ionisations of the hardcore type; σ orbital ionisations which reflect interaction potentials around CH bonds. The critical impact parameters bc become larger with increasing collision energy due to the centrifugal barrier.  相似文献   

12.
Angular distributions of electrons ejected in thermal collisions of He(21 S, 23 S)-metastables with Ar, Kr, Xe, Hg, CO, N2 are measured with respect to the vector of relative velocity of the colliding particles. Except for preliminary results on the He(21S, 23 S)-/Ar-system, these are the first such distributions reported. They are found to be strongly anisotropic and asymmetric in some cases, and approximately isotropic in those cases where the interaction potential between the metastable- and the target particle is strong. For the cases of weak interaction potential, the connection between the “internal” angular distribution in the frame fixed to the internuclear axis and the laboratory angular distribution, has been derived. Calculations of laboratory angular distributions involving an assumed “internal” distribution and the kinematics of a hard core collision show good qualitative agreement with the experimental results.  相似文献   

13.
K M Das  B B Deo 《Pramana》1984,23(1):91-97
A novel method of phase shift analysis for the scattering of charged pion from4He nuclei is proposed. The nuclear amplitudef N (ϑ) has been parametrized in terms of a polynomial expansion in a conformally mapped variable, which is obtained by optimally exploiting the analytic property off N . The method exhibits a significant reduction in the number of free parameters required for the fixed energy phase shift analysis of the differential cross-section data. The nuclear amplitude thus constructed is then used to obtain phase shifts and inelastic parameters of all possible orders. Reliable values of the real and imaginary parts of the forward amplitude are also obtained.  相似文献   

14.
Using LCAO-SCF wave functions on the monomers and a non-empirical Unsöld procedure for the second-order properties we have calculated the (2 l ) multipole moments (up to l=6), the (l,l') multipole polarizabilities (up to l + l' = 6) and the related long-range coefficients describing the electrostatic, induction and dispersion interactions for the different azabenzene molecules. The agreement with available experimental data is good, in particular for the dipole polarizabilities. The anisotropy of the long-range interaction potential is dominated by the electrostatic contributions, although the dispersion terms, especially the mixed-pole terms (ll') for even n (C8, C10), also contribute significantly; the induction energy is rather small. The π contributions to the polarizabilities and the dispersion interactions are found to be larger than earlier estimates. Moreover, it is shown by calculating the dipole polarizabilities of some (aza)naphthalenes and (aza)anthracenes, that a bond polarizability model can be applied effectively only if the delocalized π electrons are considered separately from the σ electrons.  相似文献   

15.
The correlation between the upper critical field H c2 and the residual resistivity ρ of the MgB2 compound is studied in a wide range of ρ values. The slope ?dH c2/dT of the temperature dependence of H c2 near T c is found to increase steadily with increasing residual resistivity to 100 μΩ cm. Over the range from 0 to 50 μΩ cm, the dependence of ?dH c2/dT on ρ is fitted well by a linear function, which is typical of a single-band superconductor. The fit is performed using the electronic parameters of the two bands (π and σ) that form the Fermi surface. The field H c2 is assumed to depend on the electronic parameters of the σ band only. Using this approximation, the following quantities are estimated: the relative contribution of σ electrons to the total conductivity along the boron planes (which turns out to be about 1/2), the ratio of the mean free paths of electrons in the σ and π bands l σ/l π ≈ 1.5, and the ratios between some other parameters describing electron scattering.  相似文献   

16.
解研  罗莹  刘绍军 《物理学报》2008,57(7):4364-4370
通过第一性原理计算研究了垂直于碳纳米管轴向的单向压力对碳纳米管(6,6)晶体电子结构特性的影响.计算研究发现:由碳纳米管(6,6)组成的四方结构晶体(t相)具有金属特性,电子可以沿碳纳米管管壁运动;在单向压力作用下,t相发生结构相变形成非成键相,随着压力的进一步增大,碳纳米管间产生键合,形成了成键相;单向压力对碳纳米管(6,6)晶体的能带结构影响主要表现在π能带和π*能带,伴随着单向压力的增加,碳纳米管晶体的电学性质经历从金属到半导体再到活泼金属的转变;非成键相的电子被局域在碳纳米管附近使晶体具有半导体特性,而成键相的电子不仅可以沿着碳纳米管管壁运动,还可以在碳纳米管之间(即成键方向)运动,从而使成健相晶体具有活泼的金属特性. 关键词: 碳纳米管晶体 第一性原理计算 金属—半导体转变  相似文献   

17.
We have measured energy- and angular distributions of autoionization electrons from Li+/He collisions in coincidence with the scattered Li+ projectiles. The coincident energy spectra do not exhibit the broad structures that are observed in the non coincident spectra and which in the past were attributed to quasimolecular autoionization of the (LiHe)+ system. We show that these broad structures are caused by kinematical shifts of electron spectra from pure atomic autoionization following different scattering events. With an exploitation of published inelastic differential scattering cross sections and with the assumption that the angular electron distribution with respect to the asymptotic internuclear line is nearly independent of the scattering angle we are able to reproduce the non coincident electron spectra satisfactorily.  相似文献   

18.
Summary A complete set of absolute double differential cross-section (DDCS) for electron impact ionization of helium has been measured at an incident energyE 0=500 eV. The angular distributions of the ejected and scattered electrons between 40 and 435.5 eV have been measured over the angular range of (10÷145)o. This work supplements the mapping of DDCS for ejected electron energies close to (E 0IP)/2 (IP is the He 1s ionization energy), a region where the experimental data are fragmentary. The possibility of representing the full Bethe surface with a simple functional form is investigated. To speed up publication, the authors of this paper have agreed to not receive the proofs for correction.  相似文献   

19.
20.
Electron impact double ionization cross-sections of Sc+ions have been calculated in the binary encounter approximation (BEA). Accurate expression of σΔE(cross-section for energy transfer ΔE) and Hartree-Fock velocity distributions for the target electrons have been used throughout the calculations. Direct double ionization from ejection of 3d and 4s electrons has been investigated in the modified double binary encounter model incorporating the focusing action of the target ion on the incident electron. The identification of the 3p shell whose ionization provides a major contribution to double ionization through ionization-autoionization is an interesting aspect of the present investigation. The theoretical results show satisfactory agreement with the experimental observations.  相似文献   

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