Hollow particle tracks in AgCI-detectors

In selected Cd-doped monocristalline silverchloride detectors we observe developed tracks from particles at LET values > 300 keV/μm AgCl and charge state values > 9, without a visible central region: the “hollow track”. The microdensitometric lateral profile shows a density decrease near the track axis, up to a radial extension of some microns from highly charged particles as Fe or U-ions of several MeV/u; the tracks of fast U- or Fe-projectiles, moreover, represent an entanglement of delta-electron tracks only. A recent reanalysis of this “hollow track”-effect is suggested to be caused by recombination effects and structural distortions. They occure in areas of high delta-electron density; together with the characteristic process of track formation in crystalline AgCl/Cd they enable us to vizualise and to measure the radial range of distortion and to evaluate the threshold of the energy density above which the destruction occurs.     

Differentiation between tracks and damages in SSNTD under the atomic force microscope

We have observed three-dimensional sponge-like structures as well as strips of connecting pits on the surface of the LR 115 detector after etching, which can be confused with the small tracks formed after short etching time. We have employed an atomic force microscope (AFM) to study these “damages” as well as genuine alpha tracks for short etching time. It was found that while the track and damage openings could be similar in size and shape, the depths for the damages were consistently smaller. Therefore, the depth of the pits will serve as a clear criterion to differentiate between tracks and other damages. The ability to discriminate between genuine tracks from other damages is most important for etching for short time intervals.     

The state-of-the-art in electrochemical etching of charged particle track detectors

The state-of-the-art in the electrochemical etching (ECE) amplification of charged particle tracks in polymeric detectors and its applications in particular in radiation dosimetry are presented and discussed in this paper. During the past quarter of century, extensive efforts have been made on research and development in the world as well as at NRPD in AEOI on production of high voltage generators, construction of ECE chamber systems, optimization of ECE conditions, development of detectors, studies on basic physical and chemical phenomena, promotion of large-scale applications, etc. Quality high voltage generators can now be home made or are commercially available. The ECE chamber systems are advanced for special purposes as well as for large-scale applications (e.g. pressure chamber, triplet ECE or TECE chamber, etc. from NRPD). Many parameters have been optimized and new parameters such as internal heating, pressure, detector dimensions, etchant volume, chamber insulation, etc. have been recently discovered. Lexan polycarbonates (PC) and CR-39 have been shown to be the most successful detectors for ECE, while other detectors were also applied. The fundamental phenomena including “dielectric breakdown”, “dielectric loss”, “electro-osmosis”, “dielectrophoresis”, “electrostriction”, etc. although primarily proved to exist and studied, need to be further studied. The novel triplet ECE (TECE) method has provided a new approach for track amplification, firing tree production, fractal tree generation, etc. Also the novel dyed ECE track (DYECET) method enables one to study in more detail the structure of tracks, cracks, fractals, etc. Large-scale radon monitoring indoors and outdoors, large-scale neutron personnel dosimetry, low level radionuclide determination in environmental samples, autoradiography, beam profile determination, etc. are considered some successful applications. In this paper, the above were explored with emphasis on recent discoveries and inventions at NRPD in AEOI.     

Cosmic history of the Bragin pallasite: evidence from the fission-track analysis

Chronology is rather a weak point in the investigation of pallasites, the stony-iron meteorites. No chronological data are known for the Bragin pallasite. Our attempt to reconstruct its cosmic history was based on the interpretation of fission-track analysis data. To apply this method only uranium-rich phosphates can be used. Extremely rare grains of stanfieldite were extracted from the silicate sawing residue and from the pallasite sample directly.

The researches pursued by us made it possible to find two populations of fossil tracks in stanfieldite grains. The tracks of these populations strongly differed both in size, shape and character of distribution. The first population, consisting of short (L2–6 μm instead of L8–12 μm for induced fission tracks), round-shaped tracks irregularly distributed, as we suppose, suffered an intense heating process, which caused a significant amount of partial annealing. The second population, consisting of longer (L8–12 μm), rhombic-shaped tracks homogeneously distributed, occurred after this thermal event. Only the second population track density was used for the fission-track age calculation.

After correction of the fossil track density, consisting of the second population tracks, for other possible track sources, the revealed tracks were unequivocally identified as those due to the spontaneous fission of ²⁴⁴Pu and ²³⁸U. The largest part of them was attributed to the spontaneous fission of ²⁴⁴Pu; ρ_Pu/ρ_U≈3. The model fission-track age of the studied pallasite turned out to be 4.20 Gyr. This value fix the time of the last shock/thermal event in the cosmic history of the Bragin pallasite, which had caused the partial annealing of tracks presented to that time and “fission-track clock” reset.     

Investigation of nuclear reaction products by atomic force microscopy

The use of Atomic Force Microscope (AFM, from Corporate Head, Santa Clara, California, USA) opened a new way to study latent nuclear tracks. In our experiments we used plastic track detectors of the type CR-39 (Columbia Resin No. 39) Impinging ions with energy above a threshold of 180 keV can alter the molecular structure forming latent tracks. Since nuclear latent tracks have diameters in the range of 10 to 1000 nm, they can be visualized by AFM with a slight chemical etching (6 min in 6 n NaOH solution at 70 °C). These tracks are significant for the energy, momentum and the mass of the incoming particles. In our study, passive CR-39 detectors were irradiated by secondary particles produced bombarding ¹⁰³Rh by ¹⁶O and ¹²C in a wide range of energy (1 MeV/amu to 33 MeV/amu) at the MP Tandem generator of the Laboratorio Nazionale del Sud in Catania, Italy. The experiment was carried out in order to identify the secondary particles and to determine their density and the spatial distribution.     

Alternative procedure for LR 115 chemical etching and alpha tracks counting

An improved procedure for etching and analysis of alpha tracks induced in LR-115 detectors is proposed with the advantages of simplicity and its relatively low cost. A new type of detector holder was designed to etch and rinse efficiently up to 100 detectors. We develop a simple and reliable methodology with a semiautomatic track count using a Nikon digital camera coupled to a PC and employing software “SCION” freely available on the Internet. Track images are binarized prior the application of software “SCION” so that original track shapes are not distorted, space resolution is improved and track counting has low dependence on focus and illumination level. High discrimination for tracks is achieved when marks and rips perturb the detector surface. An image generator of nuclear tracks is included to study the effect of track overlapping effect on counting.     

Low-threshold-current CW injection lasers

In this paper we report on the properties and structure of oxide-defined stripe-geometry lasers with cw threshold currents as low as 27mA at room temperature. These results have been obtained by the addition pf a dielectric facet reflector and use of a thin “cap” structure that limits the current spreading. These devices are capable of output powers up to 60mW from one facet with power conversion efficiencies up to 14%.     

Watching at the correlation between the specific track-etch rate and the primary physical parameters of the swift ion interaction with the CR-39

Analysis of etched nuclear tracks in CR-39 solid state nuclear track detectors has recently been made possible by the confocal microscope. This recent innovation has opened up some particularly interesting perspectives. The main originality of this microscopy technique is that it makes it possible to work on numerical, three-dimensional images of chemically etched nuclear tracks in the CR-39. We have studied the performances of this new approach for light ions (H, He, Li and C) with kinetic energies typically of the order of the MeV per nucleus. First, we determined the response functions of the CR-39 for these ions. We were then able to show that aside from decreasing the analysis time of traditional methods, the confocal microscope greatly increases the sensibility of the detection. The aim of this study was to find a correlation between the response functions and the primary physical parameters of the interaction between the ion and the material, such as the linear energy transfer (LET), the restricted energy transfer (REL_ω0), the integrated radial dose or the rate of ionization. Although these parameters presented a strong resemblance to the experimental response functions (they are all “Bragg” curves), none of them were correlated to the response function in an unambiguous way.     

Acoustic Analyses of Developmental Changes and Emotional Expression in the Preverbal Vocalizations of Infants

The nonverbal vocal utterances of seven normally hearing infants were studied within their first year of life with respect to age- and emotion-related changes. Supported by a multiparametric acoustic analysis it was possible to distinguish one inspiratory and eleven expiratory call types. Most of the call types appeared within the first two months; some emerged in the majority of infants not until the 5th (“laugh”) or 7th month (“babble”). Age-related changes in acoustic structure were found in only 4 call types (“discomfort cry,” “short discomfort cry,” “wail,” “moan”). The acoustic changes were characterized mainly by an increase in harmonic-to-noise ratio and homogeneity of the call, a decrease in frequency range and a downward shift of acoustic energy from higher to lower frequencies. Emotion-related differences were found in the acoustic structure of single call types as well as in the frequency of occurrence of different call types. A change from positive to negative emotional state was accompanied by an increase in call duration, frequency range, and peak frequency (frequency with the highest amplitude within the power spectrum). Negative emotions, in addition, were characterized by a significantly higher rate of “crying,” “hic” and “ingressive vocalizations” than positive emotions, while positive emotions showed a significantly higher rate of “babble,” “laugh,” and “raspberry.”     

Methane activation over Ag-exchanged ZSM-5 zeolites: A theoretical study

Methane activation catalyzed over Ag-exchanged ZSM-5 zeolites was investigated by using the density functional theory (DFT) with a cluster model. Two different pathways were taken into account in this work: the “alkyl” and the “carbenium” pathways. The activation barriers obtained are 34.09 and 66.63 kcal/mol for the “alkyl” and the “carbenium” pathway, respectively. The calculated results show that the activation barrier of the “alkyl” pathway is smaller than that of “carbenium” pathway. Consequently, the “alkyl” pathway is the preferential reaction pathway. A new mechanism of methane conversion in the presence of ethene was proposed. In the catalytic cycle, the initial step of methane activation proceeds with the “alkyl” pathway and the Ag⁺ cation acts as an acceptor of the methyl group, then ethene reacts with the Ag⁺CH₃⁻ group to form propene. In addition, it is found that the Ag⁺ cations play an important role in the methane activation, compared with the reaction of methane activation over H-ZSM-5.     

Thermal spike analysis of low energy ion tracks

The theoretical track diameter of low energy ions in organic materials is usually estimated through the model of dose deposition by delta rays, with results remarkably lower than the experimental values obtained via a replica method and electron microscopy. The track detector used here is Makrofol-E and the ions studied have specific energies between 1.4 and 100 keV/n. To evaluate the problem from another point of view, thermal effects for track formation, a modified version of the “liquid drop model” for insulators was applied. The electronic as well as nuclear energy deposition by an individual ion are considered and the thermal spike evolution is studied. The model allows for the formation of ion tracks in a range of energies previously considered as “forbidden”. There still exists a discrepancy between the experimental data and the track diameters predicted by the model, and although this difference is smaller than the obtained with previous calculations, it suggests the necessity of further adjustments.     

Four decades of nuclear tracks research in India

The science of solid state nuclear track detectors (SSNTDs)—“Trackology”—developed by R.L. Fleischer, P.B. Price and R.M. Walker in the early 1960s of the last century is an interesting and potentially useful concept with something to offer to almost all branches of science and technology. In fact nuclear tracks find applications wherever solid state damage occurs. Apart from the direct applications of far reaching consequences in nuclear physics, other areas as diverse as bio-medical sciences, cosmic rays and space physics, environmental research, geological sciences, material science, microanalysis, mine safety, nuclear technology, uranium prospecting, etc. have been greatly influenced by SSNTDs.

In this presentation, we attempt to provide an overview of the growth of nuclear tracks research in India over the last four decades and the contributions of various groups from Universities, Institutes, Nuclear Track Society of India and the Department of Atomic Energy in nurturing nuclear track research in the country. Finally, a summary of the significant contributions made by Indian scientists is also presented in this paper along with the overall impact it has made at the national and international level in many areas of basic and applied sciences such as cosmic rays and space physics, fusion–fission and particle evaporation, heavy ion ranges and energy-loss measurements, country-wide indoor radon–thoron survey, geochronology, environmental sciences, track-etch membranes and ion tracks technology, material science, physics and chemistry of fission, etc.     

Nuclear tracks in solids: registration physics and the compound spike

Observations of GeV heavy ion and MeV cluster-ion tracks in crystalline solids give us new insight into registration physics. Thermal and ion explosion spikes no longer compete; a ‘compound spike’ accounts for both. Ion explosion dominates for surface tracks (electronic sputtering). And there can also be transient plasma stopping in the bulk. For clusters there are ‘vicinage effects’—both electronic and nuclear—which can influence track dimensions and structure. Displacement cascades in large energetic clusters may lead to projectile “fission” and coherent flow into sub-tracks. The absence of tracks in certain targets, and their size/structure in others, leads to a model of projectile assisted prompt anneal (PAPA) in 10⁻¹¹s, either partial or complete, often by swift epitaxy, on elemental lattices (e.g. silicon) or on compound sublattices (e.g. fluorite). Phase transformations are important, but simple target amorphization is rare—the exception, not the rule. For many targets the thermal spike (macroscopic) fails, since ‘point’ defects (atomistic) characteristic of the target, their motion, and the electronic band structure, determine latent track detail. Circumstances in which the Bragg Rule of Additivity fails completely are revealed, and the kinetic threshold for constructive phase transitions in tracks described. This same track physics applies generally also to geothermometry—the opposite time extremum (10⁺¹¹s)—where annealing is due to defect assisted delayed anneal (DADA). Differences between etching rates of induced and spontaneous fission tracks can be explained. The geothermobarometric “Wendt/Vidal effect” (2002)—combined pressure, temperature and stress (with time) influences on fission track annealing (in e.g. apatite)—is briefly discussed.     

Track detectors in radiation monitoring of the sunken submarine “Komsomolets”

Track method (using the CN and CR-39 detectors, spark couner of tracks as well as selective sorbents for plutonium and uranium) is applied in 1994 and 1995 together with many other methods in radioecological monitoring of water in the region of the sunken nuclear submarine (NS) “Komsomolets”. The detection assembles were installed with the help of the submersibles MIR. The results obtained inside the NS and on its surface as well as near and on the remote buoy station do not contradict the data obtained by other methods confirming the absence of the plutonium leakage outside of the submarine.     

Completeness of “good” Bethe ansatz solutions of a quantum-group-invariant Heisenberg model

The sl_q(2) quantum-group-invariant Heisenberg model with open boundary conditions is investigated by means of the Bethe ansatz. As is well known, quantum groups for q equal to a root of unity possess a finite number of “good” representations with non-zero q-dimension and “bad” ones with vanishing q-dimension. Correspondingly, the state space of an invariant Heisenberg chain decomposes into “good” and “bad” states. A “good” state may be described by a path of only “good” representations. It is shown that the “good” states are given by all “good” Bethe ansatz solutions with roots restricted to the first periodicity strip, i.e. only positive-parity strings (in the language of Takahashi) are allowed. Applying Bethe's string-counting technique completeness of the “good” Bethe states is proven, i.e. the same number of states is found as the number of all restricted paths on the sl_q(2) Bratteli diagram. It is the first time that a “completeness” proof for an anisotropic quantum-invariant reduced Heisenberg model is performed.     

Discrete gauge symmetry anomalies

It has been recently argued that quantum gravity effects strongly violate all non-gauge symmetries. This would suggest that all low energy discrete symmetries should be gauge symmetries, either continuous or discrete. Acceptable continuous gauge symmetries are constrained by the condition they should be anomaly free. We show here that any discrete gauge symmetry should also obey certain “discrete anomaly cancellation” conditions. These conditions strongly constrains the massles fermion content of the theory and follow from the “parent” cancellation of the usual continuous gauge anomalies. They have interesting applications in model building. As an example we consider the constraints on the Z_N “generalized matter parities” of the supersymmetric standard model. We show that only a few (including the standard R-parity) are “discrete anomaly free” unless the fermion content of the minimal supersymmetric standard model is enlarged.     

Functional Characteristics of a New Electrolarynx “Evada” Having a Force Sensing Resistor Sensor

Electrolarynxes have been used as one of the rehabilitation methods for laryngectomees. Earlier electrolarynxes could not alter frequency and intensity simultaneously during conversation. Recently, we developed an electrolarynx named “Evada” (prototype so far) using a force sensing resistor (FSR) sensor that can control both frequency and intensity simultaneously during conversation. Employing three types of electrolarynxes (Evada, Servox-inton, Nu-vois), this study was undertaken to examine the functional characteristics of Evada for the normal control group and for laryngectomess. Five laryngectomees and five normal adults were asked to express three sentences (declarative sentence, “You stay here.”, interrogative sentence, “You stay here?”, and imperative sentence, “You! Stay here.”) using three types of electrolarynxes. Frequency and intensity changes between the first and last vowels in the three sentences were calculated and analyzed statistically by paired t test. The frequency changes in the interrogative and imperative sentences were more prominent in Evada than in Servox-inton and Nu-vois. The intensity changes in the interrogative and imperative sentences were also more prominent in Evada than in Servox-inton and Nu-vois. Evada controls frequency and/or intensity by having the subject press the control button(s). Therefore, Evada appears to be better at producing intonation and contrastive stress than Nu-vois and Servox-inton.     

Order parameters and boundary effects in U(1) lattice gauge theory

We show that, independently of the boundary conditions, the two phases of the 4-dimensional compact U(1) lattice gauge theory can be characterized by the presence or absence of an “infinite” current network, with an appropriate definition of “infinite” network takes values 0 or 1 in the cold and hot phase, respectively. It thus constitutes a very efficient order parameter, which allows one to determine the transition region at low computational cost. In addition, for open and fixed boundary conditions we address the question of the impact of inhomogeneities and give examples of the reappearance of an energy gap already at moderate lattice sizes.     

Interfacial waves with free-surface boundary conditions: an approach via a model equation

In a two-fluid system where the lower fluid is bounded below by a rigid bottom and the upper fluid is bounded above by a free surface, two kinds of solitary waves can propagate along the interface and the free surface: classical solitary waves characterized by a solitary pulse or generalized solitary waves with nondecaying oscillations in their tails in addition to the solitary pulse. The classical solitary waves move faster than the generalized solitary waves. The origin of the nonlocal solitary waves can be understood from a physical point of view. The dispersion relation for the above system shows that short waves can propagate at the same speed as a “slow” solitary wave. The interaction between the solitary wave and the short waves creates a nonlocal solitary wave. In this paper, the interfacial-wave problem is reduced to a system of ordinary differential equations by using a classical perturbation method, which takes into consideration the possible resonance between short waves and “slow” solitary waves. In the past, classical Korteweg–de Vries type models have been derived but cannot deal with the resonance. All solutions of the new system of model equations, including classical as well as generalized solitary waves, are constructed. The domain of validity of the model is discussed as well. It is also shown that fronts connecting two conjugate states cannot occur for “fast” waves. For “slow” waves, fronts exist but they have ripples in their tails.